Articles | Volume 14, issue 9
Biogeosciences, 14, 2441–2468, 2017
Biogeosciences, 14, 2441–2468, 2017

Research article 15 May 2017

Research article | 15 May 2017

Air–water CO2 evasion from US East Coast estuaries

Goulven Gildas Laruelle1, Nicolas Goossens1, Sandra Arndt1,2, Wei-Jun Cai3, and Pierre Regnier1 Goulven Gildas Laruelle et al.
  • 1Department Geosciences, Environment and Society, Université Libre de Bruxelles, Brussels, Belgium
  • 2School of Geographical Sciences, University of Bristol, Bristol, UK
  • 3School of Marine Science and Policy, University of Delaware, Newark, Delaware, USA

Abstract. This study presents the first regional-scale assessment of estuarine CO2 evasion along the US East Coast (25–45° N). The focus is on 42 tidal estuaries, which together drain a catchment of 697 000 km2 or 76 % of the total area within this latitudinal band. The approach is based on the Carbon–Generic Estuary Model (C-GEM) that allows the simulation of hydrodynamics, transport, and biogeochemistry for a wide range of estuarine systems using readily available geometric parameters and global databases of seasonal climatic, hydraulic, and riverine biogeochemical information. Our simulations, performed using conditions representative of the year 2000, suggest that, together, US East Coast estuaries emit 1.9 Tg C yr−1 in the form of CO2, which corresponds to about 40 % of the carbon inputs from rivers, marshes, and mangroves. Carbon removal within estuaries results from a combination of physical (outgassing of supersaturated riverine waters) and biogeochemical processes (net heterotrophy and nitrification). The CO2 evasion and its underlying drivers show important variations across individual systems, but reveal a clear latitudinal pattern characterized by a decrease in the relative importance of physical over biogeochemical processes along a north–south gradient. Finally, the results reveal that the ratio of estuarine surface area to the river discharge, SQ (which has a scale of per meter discharged water per year), could be used as a predictor of the estuarine carbon processing in future regional- and global-scale assessments.

Short summary
The C-GEM generic reactive-transport model is applied to each tidal estuary of the US East Coast. Seasonal simulations are performed, which allows the understanding and quantification of the effect of the estuarine filter on the lateral fluxes of carbon coming from rivers.
Final-revised paper