Articles | Volume 15, issue 13
https://doi.org/10.5194/bg-15-4087-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/bg-15-4087-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Technical note
| 
04 Jul 2018
Technical note |
| 04 Jul 2018
| 04 Jul 2018
Technical note: In situ measurement of flux and isotopic composition of CO2 released during oxidative weathering of sedimentary rocks
Guillaume Soulet
CORRESPONDING AUTHOR
Department of Geography, Durham University, South Road, Durham DH1
3LE, UK
Robert G. Hilton
Department of Geography, Durham University, South Road, Durham DH1
3LE, UK
Mark H. Garnett
NERC Radiocarbon Facility, Rankine Avenue, East Kilbride, Glasgow G75
0QF, UK
Mathieu Dellinger
Department of Geography, Durham University, South Road, Durham DH1
3LE, UK
Thomas Croissant
Department of Geography, Durham University, South Road, Durham DH1
3LE, UK
Mateja Ogrič
Department of Geography, Durham University, South Road, Durham DH1
3LE, UK
Sébastien Klotz
IRSTEA Grenoble, 2 rue de la papeterie, BP 76, 38402
Saint-Martin-d'Hères, Cedex, France
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Cited
18 citations as recorded by crossref.
- Concentration‐Discharge Relationships of Dissolved Rhenium in Alpine Catchments Reveal Its Use as a Tracer of Oxidative Weathering R. Hilton et al. 10.1029/2021WR029844
- A high-frequency, long-term data set of hydrology and sediment yield: the alpine badland catchments of Draix-Bléone Observatory S. Klotz et al. 10.5194/essd-15-4371-2023
- Net effect of chemical erosion in a tropical basin on carbon cycle: Constraints from elemental and sulfur isotopic composition of the Mahanadi river water R. Rout & G. Tripathy 10.1016/j.chemgeo.2023.121859
- Carbon Dioxide Production in Bedrock Beneath Soils Substantially Contributes to Forest Carbon Cycling A. Tune et al. 10.1029/2020JG005795
- Validating the rhenium proxy for rock organic carbon oxidation using weathering profiles K. Grant et al. 10.1016/j.chemgeo.2024.122464
- High-temporal-resolution of lithium isotopes in Yangtze River headwater: Hydrological control on weathering in high-relief catchments T. Ma et al. 10.1016/j.scitotenv.2023.163214
- Temperature control on CO2 emissions from the weathering of sedimentary rocks G. Soulet et al. 10.1038/s41561-021-00805-1
- Ideas and perspectives: Emerging contours of a dynamic exogenous kerogen cycle T. Blattmann 10.5194/bg-19-359-2022
- Biomineral deposits and coatings on stone monuments as biodeterioration fingerprints J. Sanjurjo-Sánchez et al. 10.1016/j.scitotenv.2023.168846
- Biodeterioration of stone and metal — Fundamental microbial cycling processes with spatial and temporal scale differences C. Gaylarde & B. Little 10.1016/j.scitotenv.2022.153193
- Deep root activity overprints weathering of petrogenic organic carbon in shale A. Tune et al. 10.1016/j.epsl.2023.118048
- Probing the exchange of CO2 and O2 in the shallow critical zone during weathering of marl and black shale T. Roylands et al. 10.5194/esurf-12-271-2024
- Mountains, erosion and the carbon cycle R. Hilton & A. West 10.1038/s43017-020-0058-6
- Geogenic organic carbon in terrestrial sediments and its contribution to total soil carbon F. Kalks et al. 10.5194/soil-7-347-2021
- Fractionation of rhenium isotopes in the Mackenzie River basin during oxidative weathering M. Dellinger et al. 10.1016/j.epsl.2021.117131
- Origin of dissolved gas (CO2, O2, N2, alkanes) in pore waters of a clay formation in the critical zone (Tégulines Clay, France) C. Lerouge et al. 10.1016/j.apgeochem.2020.104573
- Experimental investigation of the influence of sequential water-rock reactions on the mineral alterations and porosity evolution of shale Q. Li et al. 10.1016/j.conbuildmat.2021.125859
- Capturing the short-term variability of carbon dioxide emissions from sedimentary rock weathering in a remote mountainous catchment, New Zealand T. Roylands et al. 10.1016/j.chemgeo.2022.121024
18 citations as recorded by crossref.
- Concentration‐Discharge Relationships of Dissolved Rhenium in Alpine Catchments Reveal Its Use as a Tracer of Oxidative Weathering R. Hilton et al. 10.1029/2021WR029844
- A high-frequency, long-term data set of hydrology and sediment yield: the alpine badland catchments of Draix-Bléone Observatory S. Klotz et al. 10.5194/essd-15-4371-2023
- Net effect of chemical erosion in a tropical basin on carbon cycle: Constraints from elemental and sulfur isotopic composition of the Mahanadi river water R. Rout & G. Tripathy 10.1016/j.chemgeo.2023.121859
- Carbon Dioxide Production in Bedrock Beneath Soils Substantially Contributes to Forest Carbon Cycling A. Tune et al. 10.1029/2020JG005795
- Validating the rhenium proxy for rock organic carbon oxidation using weathering profiles K. Grant et al. 10.1016/j.chemgeo.2024.122464
- High-temporal-resolution of lithium isotopes in Yangtze River headwater: Hydrological control on weathering in high-relief catchments T. Ma et al. 10.1016/j.scitotenv.2023.163214
- Temperature control on CO2 emissions from the weathering of sedimentary rocks G. Soulet et al. 10.1038/s41561-021-00805-1
- Ideas and perspectives: Emerging contours of a dynamic exogenous kerogen cycle T. Blattmann 10.5194/bg-19-359-2022
- Biomineral deposits and coatings on stone monuments as biodeterioration fingerprints J. Sanjurjo-Sánchez et al. 10.1016/j.scitotenv.2023.168846
- Biodeterioration of stone and metal — Fundamental microbial cycling processes with spatial and temporal scale differences C. Gaylarde & B. Little 10.1016/j.scitotenv.2022.153193
- Deep root activity overprints weathering of petrogenic organic carbon in shale A. Tune et al. 10.1016/j.epsl.2023.118048
- Probing the exchange of CO2 and O2 in the shallow critical zone during weathering of marl and black shale T. Roylands et al. 10.5194/esurf-12-271-2024
- Mountains, erosion and the carbon cycle R. Hilton & A. West 10.1038/s43017-020-0058-6
- Geogenic organic carbon in terrestrial sediments and its contribution to total soil carbon F. Kalks et al. 10.5194/soil-7-347-2021
- Fractionation of rhenium isotopes in the Mackenzie River basin during oxidative weathering M. Dellinger et al. 10.1016/j.epsl.2021.117131
- Origin of dissolved gas (CO2, O2, N2, alkanes) in pore waters of a clay formation in the critical zone (Tégulines Clay, France) C. Lerouge et al. 10.1016/j.apgeochem.2020.104573
- Experimental investigation of the influence of sequential water-rock reactions on the mineral alterations and porosity evolution of shale Q. Li et al. 10.1016/j.conbuildmat.2021.125859
- Capturing the short-term variability of carbon dioxide emissions from sedimentary rock weathering in a remote mountainous catchment, New Zealand T. Roylands et al. 10.1016/j.chemgeo.2022.121024
Latest update: 23 Nov 2024
Short summary
Oxidative weathering of sedimentary rocks can release carbon dioxide to the atmosphere. Here, we designed a chamber-based method to measure these CO2 emissions directly for the first time. The chamber is drilled in the rock and allows us to collect the CO2 to fingerprint its source using carbon isotopes. We tested our method in Draix (France). The measured CO2 fluxes were substantial, with ~20% originating from oxidation of the rock organic matter and ~80% from dissolution of carbonate minerals.
Oxidative weathering of sedimentary rocks can release carbon dioxide to the atmosphere. Here, we...
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