Articles | Volume 18, issue 9
https://doi.org/10.5194/bg-18-2843-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/bg-18-2843-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
10 May 2021
Research article |
| 10 May 2021
| 10 May 2021
Sun-induced fluorescence and near-infrared reflectance of vegetation track the seasonal dynamics of gross primary production over Africa
Anteneh Getachew Mengistu
CORRESPONDING AUTHOR
Department of Physics, Addis Ababa University, Addis Ababa, Ethiopia
Royal Netherlands Meteorological Institute, De Bilt, The Netherlands
Gizaw Mengistu Tsidu
Department of Physics, Addis Ababa University, Addis Ababa, Ethiopia
Department of Earth and Environmental Sciences, Botswana International University of Science and Technology, Palapye, Botswana
Gerbrand Koren
Meteorology and Air Quality Group, Wageningen University, Wageningen, the Netherlands
Maurits L. Kooreman
Royal Netherlands Meteorological Institute, De Bilt, The Netherlands
K. Folkert Boersma
Meteorology and Air Quality Group, Wageningen University, Wageningen, the Netherlands
Royal Netherlands Meteorological Institute, De Bilt, The Netherlands
Torbern Tagesson
Department of Physical Geography and Ecosystem Science, Lund University, Lund, Sweden
Department of Geosciences and Natural Resource Management, University of Copenhagen, Copenhagen, Denmark
Jonas Ardö
Department of Physical Geography and Ecosystem Science, Lund University, Lund, Sweden
Yann Nouvellon
Eco&Sols, Univ Montpellier, CIRAD, INRA, IRD, Montpellier SupAgro, 34060 Montpellier, France
CIRAD, UMR Eco&Sols, 34060 Montpellier, France
Wouter Peters
Meteorology and Air Quality Group, Wageningen University, Wageningen, the Netherlands
Centre for Isotope Research, University of Groningen, Groningen, the Netherlands
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Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2025-561, https://doi.org/10.5194/essd-2025-561, 2025
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Earth Syst. Sci. Data, 17, 6129–6147, https://doi.org/10.5194/essd-17-6129-2025, https://doi.org/10.5194/essd-17-6129-2025, 2025
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This study describes a unique large-scale isotope dataset to study water dynamics in European forests. Researchers collected data from 40 beech and spruce forest sites in spring and summer 2023, using a standardized method to ensure consistency. The results show that water sources for trees change between seasons and vary by tree species. This large dataset offers valuable information for understanding plant water use, improving ecohydrological models, and mapping water cycles across Europe.
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Hong Zhao, Han Dolman, Jan Elbers, Wilma Jans, Bart Kruijt, Eddy Moors, Henk Snellen, Jordi Vila-Guerau de Arellano, Wouter Peters, Maarten Krol, Ronald Hutjes, and Michiel van der Molen
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Blanca Ayarzagüena, Amy H. Butler, Peter Hitchcock, Chaim I. Garfinkel, Zac D. Lawrence, Wuhan Ning, Philip Rupp, Zheng Wu, Hilla Afargan-Gerstman, Natalia Calvo, Álvaro de la Cámara, Martin Jucker, Gerbrand Koren, Daniel De Maeseneire, Gloria L. Manney, Marisol Osman, Masakazu Taguchi, Cory Barton, Dong-Chang Hong, Yu-Kyung Hyun, Hera Kim, Jeff Knight, Piero Malguzzi, Daniele Mastrangelo, Jiyoung Oh, Inna Polichtchouk, Jadwiga H. Richter, Isla R. Simpson, Seok-Woo Son, Damien Specq, and Tim Stockdale
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Sudden Stratospheric Warmings (SSWs) are known to follow a sustained wave dissipation in the stratosphere, which depends on both the tropospheric and stratospheric states. However, the relative role of each state is still unclear. Using a new set of subseasonal to seasonal forecasts, we show that the stratospheric state does not drastically affect the precursors of three recent SSWs, but modulates the stratospheric wave activity, with impacts depending on SSW features.
Daniel Epron, Rawiwan Chotiphan, Zixiao Wang, Ornuma Duangngam, Makoto Shibata, Sumonta Kumar Paul, Takumi Mochidome, Jate Sathornkich, Wakana A. Azuma, Jun Murase, Yann Nouvellon, Poonpipope Kasemsap, and Kannika Sajjaphan
Biogeosciences, 22, 4013–4033, https://doi.org/10.5194/bg-22-4013-2025, https://doi.org/10.5194/bg-22-4013-2025, 2025
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The rapid expansion of rubber cultivation constitutes a significant land-use change in Southeast Asia. Despite fertilization being a common practice in rubber plantations, its impact on soil methane (CH4) dynamics has remained poorly understood. Our study demonstrates that fertilization not only reduces soil CH4 consumption but also increases CH4 production, transforming rubber plantations from a net CH4 sink to a source. Implementing rational fertilization could enhance atmospheric CH4 removal.
Suvarna Fadnavis, Yasin Elshorbany, Jerald Ziemke, Brice Barret, Alexandru Rap, P. R. Satheesh Chandran, Richard J. Pope, Vijay Sagar, Domenico Taraborrelli, Eric Le Flochmoen, Juan Cuesta, Catherine Wespes, Folkert Boersma, Isolde Glissenaar, Isabelle De Smedt, Michel Van Roozendael, Hervé Petetin, and Isidora Anglou
Atmos. Chem. Phys., 25, 8229–8254, https://doi.org/10.5194/acp-25-8229-2025, https://doi.org/10.5194/acp-25-8229-2025, 2025
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Satellites and model simulations show enhancement in tropospheric ozone, which is highly impacted by human-produced nitrous oxides compared to volatile organic compounds. The increased amount of ozone enhances ozone radiative forcing. The ozone enhancement and associated radiative forcing are the highest over South and East Asia. The emissions of nitrous oxides show a higher influence on shifting ozone photochemical regimes than volatile organic compounds.
Theertha Kariyathan, Ana Bastos, Markus Reichstein, Wouter Peters, and Julia Marshall
Atmos. Chem. Phys., 25, 7863–7878, https://doi.org/10.5194/acp-25-7863-2025, https://doi.org/10.5194/acp-25-7863-2025, 2025
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The carbon uptake period (CUP) is the time period when land absorbs more CO2 than it emits. While atmospheric CO2 mole fraction measurements can be used to assess CUP changes, atmospheric transport and asynchronous timing across regions reduce the accuracy of the estimates. Forward model experiments show that only ~ 50 % of prescribed shifts in CUP timing applied to surface fluxes (ΔCUPNEE) are captured in simulated CO2 mole fraction data at monitoring sites like the Barrow Atmospheric Baseline Observatory.
Santiago Botía, Saqr Munassar, Thomas Koch, Danilo Custodio, Luana S. Basso, Shujiro Komiya, Jost V. Lavric, David Walter, Manuel Gloor, Giordane Martins, Stijn Naus, Gerbrand Koren, Ingrid T. Luijkx, Stijn Hantson, John B. Miller, Wouter Peters, Christian Rödenbeck, and Christoph Gerbig
Atmos. Chem. Phys., 25, 6219–6255, https://doi.org/10.5194/acp-25-6219-2025, https://doi.org/10.5194/acp-25-6219-2025, 2025
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This study uses dry CO2 mole fractions from the Amazon Tall Tower Observatory together with airborne profiles to estimate net carbon exchange in tropical South America. We found that the biogeographic Amazon is a net carbon sink, while the Cerrado and Caatinga biomes are net carbon sources, resulting in an overall neutral balance. Finally, to further reduce the uncertainty in our estimates we call for an expansion of the monitoring capacity, especially in the Amazon–Andes foothills.
Getachew Agmuas Adnew, Gerbrand Koren, Neha Mehendale, Sergey Gromov, Maarten Krol, and Thomas Röckmann
Atmos. Meas. Tech., 18, 2701–2719, https://doi.org/10.5194/amt-18-2701-2025, https://doi.org/10.5194/amt-18-2701-2025, 2025
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This study presents high-precision measurements of ∆′17O(CO2). Key findings include the extension of the N2O–∆′17O correlation to the upper troposphere and the identification of significant differences in the N2O–∆′17O slope in StratoClim samples. Additionally, the ∆′17O measurements are used to estimate global stratospheric production and surface removal of ∆′17O, providing an independent estimate of global vegetation CO2 exchange.
Cynthia H. Whaley, Tim Butler, Jose A. Adame, Rupal Ambulkar, Steve R. Arnold, Rebecca R. Buchholz, Benjamin Gaubert, Douglas S. Hamilton, Min Huang, Hayley Hung, Johannes W. Kaiser, Jacek W. Kaminski, Christoph Knote, Gerbrand Koren, Jean-Luc Kouassi, Meiyun Lin, Tianjia Liu, Jianmin Ma, Kasemsan Manomaiphiboon, Elisa Bergas Masso, Jessica L. McCarty, Mariano Mertens, Mark Parrington, Helene Peiro, Pallavi Saxena, Saurabh Sonwani, Vanisa Surapipith, Damaris Y. T. Tan, Wenfu Tang, Veerachai Tanpipat, Kostas Tsigaridis, Christine Wiedinmyer, Oliver Wild, Yuanyu Xie, and Paquita Zuidema
Geosci. Model Dev., 18, 3265–3309, https://doi.org/10.5194/gmd-18-3265-2025, https://doi.org/10.5194/gmd-18-3265-2025, 2025
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The multi-model experiment design of the HTAP3 Fires project takes a multi-pollutant approach to improving our understanding of transboundary transport of wildland fire and agricultural burning emissions and their impacts. The experiments are designed with the goal of answering science policy questions related to fires. The options for the multi-model approach, including inputs, outputs, and model setup, are discussed, and the official recommendations for the project are presented.
Gezahegn Sufa Daba and Gizaw Mengistu Tsidu
EGUsphere, https://doi.org/10.5194/egusphere-2025-2232, https://doi.org/10.5194/egusphere-2025-2232, 2025
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This study investigates non-ideal instrumental effects that could degrade the performance of a high-resolution infrared spectrometer. By using standard gas cell measurement, it identifies key sources of modulation loss and spectral artifacts. The results help improve understanding of instrumental stability and support more accurate use of the spectrometer in long-term scientific applications.
Samuel Upton, Markus Reichstein, Wouter Peters, Santiago Botía, Jacob A. Nelson, Sophia Walther, Martin Jung, Fabian Gans, László Haszpra, and Ana Bastos
EGUsphere, https://doi.org/10.5194/egusphere-2025-2097, https://doi.org/10.5194/egusphere-2025-2097, 2025
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We create a hybrid ecosystem-level carbon flux model using both eddy-covariance observations and observations of the atmospheric mole fraction of CO2 at three tall-tower observatories. Our study uses an atmospheric transport model (STILT) to connect the atmospheric signal to the ecosystem-level model. We show that this inclusion of atmospheric information meaningfully improves the model's representation of the interannual variability of the global net flux of CO2.
Juliëtte C. S. Anema, K. Folkert Boersma, Lieuwe G. Tilstra, Olaf N. E. Tuinder, and Willem W. Verstraeten
Atmos. Meas. Tech., 18, 1961–1979, https://doi.org/10.5194/amt-18-1961-2025, https://doi.org/10.5194/amt-18-1961-2025, 2025
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Long-term records of plant fluorescence offer vital insights into changing vegetation activity. The GOME-2A sensor provides extensive global observations but suffers from calibration and instrument degradation, which affects data consistency. This study presents the SIFTER v3 algorithm, which effectively resolves these issues and includes other improvements, resulting in robust, accurate, and consistent GOME-2A fluorescence measurements from 2007 to 2017.
Qianqian Zhang, K. Folkert Boersma, Chiel van der Laan, Alba Mols, Bin Zhao, Shengyue Li, and Yuepeng Pan
Atmos. Chem. Phys., 25, 3313–3326, https://doi.org/10.5194/acp-25-3313-2025, https://doi.org/10.5194/acp-25-3313-2025, 2025
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Accurate NOx emission estimates are required to better understand air pollution. This study investigates and demonstrates the ability of the superposition column model in combination with TROPOMI tropospheric NO2 column data to estimate city-scale NOx emissions and lifetimes and their variabilities. The results of this work nevertheless confirm the strength of the superposition column model in estimating urban NOx emissions with reasonable accuracy.
Zhu Deng, Philippe Ciais, Liting Hu, Adrien Martinez, Marielle Saunois, Rona L. Thompson, Kushal Tibrewal, Wouter Peters, Brendan Byrne, Giacomo Grassi, Paul I. Palmer, Ingrid T. Luijkx, Zhu Liu, Junjie Liu, Xuekun Fang, Tengjiao Wang, Hanqin Tian, Katsumasa Tanaka, Ana Bastos, Stephen Sitch, Benjamin Poulter, Clément Albergel, Aki Tsuruta, Shamil Maksyutov, Rajesh Janardanan, Yosuke Niwa, Bo Zheng, Joël Thanwerdas, Dmitry Belikov, Arjo Segers, and Frédéric Chevallier
Earth Syst. Sci. Data, 17, 1121–1152, https://doi.org/10.5194/essd-17-1121-2025, https://doi.org/10.5194/essd-17-1121-2025, 2025
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This study reconciles national greenhouse gas (GHG) inventories with updated atmospheric inversion results to evaluate discrepancies for three principal GHG fluxes at the national level. Compared to our previous study, new satellite-based CO2 inversions were included and an updated mask of managed lands was used, improving agreement for Brazil and Canada. The proposed methodology can be regularly applied as a check to assess the gap between top-down inversions and bottom-up inventories.
Pierre Friedlingstein, Michael O'Sullivan, Matthew W. Jones, Robbie M. Andrew, Judith Hauck, Peter Landschützer, Corinne Le Quéré, Hongmei Li, Ingrid T. Luijkx, Are Olsen, Glen P. Peters, Wouter Peters, Julia Pongratz, Clemens Schwingshackl, Stephen Sitch, Josep G. Canadell, Philippe Ciais, Robert B. Jackson, Simone R. Alin, Almut Arneth, Vivek Arora, Nicholas R. Bates, Meike Becker, Nicolas Bellouin, Carla F. Berghoff, Henry C. Bittig, Laurent Bopp, Patricia Cadule, Katie Campbell, Matthew A. Chamberlain, Naveen Chandra, Frédéric Chevallier, Louise P. Chini, Thomas Colligan, Jeanne Decayeux, Laique M. Djeutchouang, Xinyu Dou, Carolina Duran Rojas, Kazutaka Enyo, Wiley Evans, Amanda R. Fay, Richard A. Feely, Daniel J. Ford, Adrianna Foster, Thomas Gasser, Marion Gehlen, Thanos Gkritzalis, Giacomo Grassi, Luke Gregor, Nicolas Gruber, Özgür Gürses, Ian Harris, Matthew Hefner, Jens Heinke, George C. Hurtt, Yosuke Iida, Tatiana Ilyina, Andrew R. Jacobson, Atul K. Jain, Tereza Jarníková, Annika Jersild, Fei Jiang, Zhe Jin, Etsushi Kato, Ralph F. Keeling, Kees Klein Goldewijk, Jürgen Knauer, Jan Ivar Korsbakken, Xin Lan, Siv K. Lauvset, Nathalie Lefèvre, Zhu Liu, Junjie Liu, Lei Ma, Shamil Maksyutov, Gregg Marland, Nicolas Mayot, Patrick C. McGuire, Nicolas Metzl, Natalie M. Monacci, Eric J. Morgan, Shin-Ichiro Nakaoka, Craig Neill, Yosuke Niwa, Tobias Nützel, Lea Olivier, Tsuneo Ono, Paul I. Palmer, Denis Pierrot, Zhangcai Qin, Laure Resplandy, Alizée Roobaert, Thais M. Rosan, Christian Rödenbeck, Jörg Schwinger, T. Luke Smallman, Stephen M. Smith, Reinel Sospedra-Alfonso, Tobias Steinhoff, Qing Sun, Adrienne J. Sutton, Roland Séférian, Shintaro Takao, Hiroaki Tatebe, Hanqin Tian, Bronte Tilbrook, Olivier Torres, Etienne Tourigny, Hiroyuki Tsujino, Francesco Tubiello, Guido van der Werf, Rik Wanninkhof, Xuhui Wang, Dongxu Yang, Xiaojuan Yang, Zhen Yu, Wenping Yuan, Xu Yue, Sönke Zaehle, Ning Zeng, and Jiye Zeng
Earth Syst. Sci. Data, 17, 965–1039, https://doi.org/10.5194/essd-17-965-2025, https://doi.org/10.5194/essd-17-965-2025, 2025
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The Global Carbon Budget 2024 describes the methodology, main results, and datasets used to quantify the anthropogenic emissions of carbon dioxide (CO2) and their partitioning among the atmosphere, land ecosystems, and the ocean over the historical period (1750–2024). These living datasets are updated every year to provide the highest transparency and traceability in the reporting of CO2, the key driver of climate change.
Takashi Sekiya, Emanuele Emili, Kazuyuki Miyazaki, Antje Inness, Zhen Qu, R. Bradley Pierce, Dylan Jones, Helen Worden, William Y. Y. Cheng, Vincent Huijnen, and Gerbrand Koren
Atmos. Chem. Phys., 25, 2243–2268, https://doi.org/10.5194/acp-25-2243-2025, https://doi.org/10.5194/acp-25-2243-2025, 2025
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Five global chemical reanalysis datasets were used to assess the relative impacts of assimilating satellite ozone and its precursor measurements on tropospheric ozone analyses for 2010. The multiple reanalysis system comparison allows an evaluation of the dependency of the impacts on different reanalysis systems. The results suggested the importance of satellite ozone and its precursor measurements for improving ozone analysis in the whole troposphere, with varying magnitudes among the systems.
Chaim I. Garfinkel, Zachary D. Lawrence, Amy H. Butler, Etienne Dunn-Sigouin, Irene Erner, Alexey Y. Karpechko, Gerbrand Koren, Marta Abalos, Blanca Ayarzagüena, David Barriopedro, Natalia Calvo, Alvaro de la Cámara, Andrew Charlton-Perez, Judah Cohen, Daniela I. V. Domeisen, Javier García-Serrano, Neil P. Hindley, Martin Jucker, Hera Kim, Robert W. Lee, Simon H. Lee, Marisol Osman, Froila M. Palmeiro, Inna Polichtchouk, Jian Rao, Jadwiga H. Richter, Chen Schwartz, Seok-Woo Son, Masakazu Taguchi, Nicholas L. Tyrrell, Corwin J. Wright, and Rachel W.-Y. Wu
Weather Clim. Dynam., 6, 171–195, https://doi.org/10.5194/wcd-6-171-2025, https://doi.org/10.5194/wcd-6-171-2025, 2025
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Variability in the extratropical stratosphere and troposphere is coupled, and because of the longer timescales characteristic of the stratosphere, this allows for a window of opportunity for surface prediction. This paper assesses whether models used for operational prediction capture these coupling processes accurately. We find that most processes are too weak; however downward coupling from the lower stratosphere to the near surface is too strong.
Felipe Cifuentes, Henk Eskes, Enrico Dammers, Charlotte Bryan, and Folkert Boersma
Geosci. Model Dev., 18, 621–649, https://doi.org/10.5194/gmd-18-621-2025, https://doi.org/10.5194/gmd-18-621-2025, 2025
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We tested the capability of the flux divergence approach (FDA) to reproduce known NOx emissions using synthetic NO2 satellite column retrievals from high-resolution model simulations. The FDA accurately reproduced NOx emissions when column observations were limited to the boundary layer and when the variability of the NO2 lifetime, the NOx : NO2 ratio, and NO2 profile shapes were correctly modeled. This introduces strong model dependency, reducing the simplicity of the original FDA formulation.
Pieter Rijsdijk, Henk Eskes, Arlene Dingemans, K. Folkert Boersma, Takashi Sekiya, Kazuyuki Miyazaki, and Sander Houweling
Geosci. Model Dev., 18, 483–509, https://doi.org/10.5194/gmd-18-483-2025, https://doi.org/10.5194/gmd-18-483-2025, 2025
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Clustering high-resolution satellite observations into superobservations improves model validation and data assimilation applications. In our paper, we derive quantitative uncertainties for satellite NO2 column observations based on knowledge of the retrievals, including a detailed analysis of spatial error correlations and representativity errors. The superobservations and uncertainty estimates are tested in a global chemical data assimilation system and are found to improve the forecasts.
Alba Mols, Klaas Folkert Boersma, Hugo Denier van der Gon, and Maarten Krol
EGUsphere, https://doi.org/10.5194/egusphere-2025-49, https://doi.org/10.5194/egusphere-2025-49, 2025
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We created a new method to estimate city air pollution (NOx emissions) using satellite data. Testing showed our approach works well to track how pollution spreads in urban areas. By combining observations with prior knowledge, we improved the accuracy of emission estimates. Applying this method in Paris, we found emissions were 9 % lower than expected and dropped significantly during COVID-19 lockdowns. Our method offers a reliable way to monitor pollution and support environmental policies.
Dylan Jones, Lucas Prates, Zhen Qu, William Cheng, Kazuyuki Miyazaki, Takashi Sekiya, Antje Inness, Rajesh Kumar, Xiao Tang, Helen Worden, Gerbrand Koren, and Vincent Huijen
EGUsphere, https://doi.org/10.5194/egusphere-2024-3759, https://doi.org/10.5194/egusphere-2024-3759, 2025
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We evaluate five chemical reanalysis products to assess their potential to provide useful information on tropospheric ozone variability. We find that the reanalyses produce consistent information on ozone variations in the free troposphere, but have large discrepancies at the surface. The results suggests that improvements in the reanalyses are needed to better exploit the assimilated observations to enhance the utility of the reanalysis products at the surface.
Jacob A. Nelson, Sophia Walther, Fabian Gans, Basil Kraft, Ulrich Weber, Kimberly Novick, Nina Buchmann, Mirco Migliavacca, Georg Wohlfahrt, Ladislav Šigut, Andreas Ibrom, Dario Papale, Mathias Göckede, Gregory Duveiller, Alexander Knohl, Lukas Hörtnagl, Russell L. Scott, Jiří Dušek, Weijie Zhang, Zayd Mahmoud Hamdi, Markus Reichstein, Sergio Aranda-Barranco, Jonas Ardö, Maarten Op de Beeck, Dave Billesbach, David Bowling, Rosvel Bracho, Christian Brümmer, Gustau Camps-Valls, Shiping Chen, Jamie Rose Cleverly, Ankur Desai, Gang Dong, Tarek S. El-Madany, Eugenie Susanne Euskirchen, Iris Feigenwinter, Marta Galvagno, Giacomo A. Gerosa, Bert Gielen, Ignacio Goded, Sarah Goslee, Christopher Michael Gough, Bernard Heinesch, Kazuhito Ichii, Marcin Antoni Jackowicz-Korczynski, Anne Klosterhalfen, Sara Knox, Hideki Kobayashi, Kukka-Maaria Kohonen, Mika Korkiakoski, Ivan Mammarella, Mana Gharun, Riccardo Marzuoli, Roser Matamala, Stefan Metzger, Leonardo Montagnani, Giacomo Nicolini, Thomas O'Halloran, Jean-Marc Ourcival, Matthias Peichl, Elise Pendall, Borja Ruiz Reverter, Marilyn Roland, Simone Sabbatini, Torsten Sachs, Marius Schmidt, Christopher R. Schwalm, Ankit Shekhar, Richard Silberstein, Maria Lucia Silveira, Donatella Spano, Torbern Tagesson, Gianluca Tramontana, Carlo Trotta, Fabio Turco, Timo Vesala, Caroline Vincke, Domenico Vitale, Enrique R. Vivoni, Yi Wang, William Woodgate, Enrico A. Yepez, Junhui Zhang, Donatella Zona, and Martin Jung
Biogeosciences, 21, 5079–5115, https://doi.org/10.5194/bg-21-5079-2024, https://doi.org/10.5194/bg-21-5079-2024, 2024
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The movement of water, carbon, and energy from the Earth's surface to the atmosphere, or flux, is an important process to understand because it impacts our lives. Here, we outline a method called FLUXCOM-X to estimate global water and CO2 fluxes based on direct measurements from sites around the world. We go on to demonstrate how these new estimates of net CO2 uptake/loss, gross CO2 uptake, total water evaporation, and transpiration from plants compare to previous and independent estimates.
Pharahilda M. Steur, Hubertus A. Scheeren, Gerbrand Koren, Getachew A. Adnew, Wouter Peters, and Harro A. J. Meijer
Atmos. Chem. Phys., 24, 11005–11027, https://doi.org/10.5194/acp-24-11005-2024, https://doi.org/10.5194/acp-24-11005-2024, 2024
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We present records of the triple oxygen isotope signature (Δ(17O)) of atmospheric CO2 obtained with laser absorption spectroscopy from two mid-latitude stations. Significant interannual variability is observed in both records. A model sensitivity study suggests that stratosphere–troposphere exchange, which carries high-Δ(17O) CO2 from the stratosphere into the troposphere, causes most of the variability. This makes Δ(17O) a potential tracer for stratospheric intrusions into the troposphere.
Pierluigi Renan Guaita, Riccardo Marzuoli, Leiming Zhang, Steven Turnock, Gerbrand Koren, Oliver Wild, Paola Crippa, and Giacomo Alessandro Gerosa
EGUsphere, https://doi.org/10.5194/egusphere-2024-2573, https://doi.org/10.5194/egusphere-2024-2573, 2024
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This study assesses the global impact of tropospheric ozone on wheat crops in the 21st century under various climate scenarios. The research highlights that ozone damage to wheat varies by region and depends on both ozone levels and climate. Vulnerable regions include East Asia, Northern Europe, and the Southern and Eastern edges of the Tibetan Plateau. Our results emphasize the need of policies to reduce ozone levels and mitigate climate change to protect global food security.
Tong Sha, Siyu Yang, Qingcai Chen, Liangqing Li, Xiaoyan Ma, Yan-Lin Zhang, Zhaozhong Feng, K. Folkert Boersma, and Jun Wang
Atmos. Chem. Phys., 24, 8441–8455, https://doi.org/10.5194/acp-24-8441-2024, https://doi.org/10.5194/acp-24-8441-2024, 2024
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Using an updated soil reactive nitrogen emission scheme in the Unified Inputs for Weather Research and Forecasting coupled with Chemistry (UI-WRF-Chem) model, we investigate the role of soil NO and HONO (Nr) emissions in air quality and temperature in North China. Contributions of soil Nr emissions to O3 and secondary pollutants are revealed, exceeding effects of soil NOx or HONO emission. Soil Nr emissions play an important role in mitigating O3 pollution and addressing climate change.
Maarten Krol, Bart van Stratum, Isidora Anglou, and Klaas Folkert Boersma
Atmos. Chem. Phys., 24, 8243–8262, https://doi.org/10.5194/acp-24-8243-2024, https://doi.org/10.5194/acp-24-8243-2024, 2024
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This paper presents detailed plume simulations of nitrogen oxides and carbon dioxide that are emitted from four large industrial facilities world-wide. Results from the high-resolution simulations that include atmospheric chemistry are compared to nitrogen dioxide observations from satellites. We find good performance of the model and show that common assumptions that are used in simplified models need revision. This work is important for the monitoring of emissions using satellite data.
Kim A. P. Faassen, Jordi Vilà-Guerau de Arellano, Raquel González-Armas, Bert G. Heusinkveld, Ivan Mammarella, Wouter Peters, and Ingrid T. Luijkx
Biogeosciences, 21, 3015–3039, https://doi.org/10.5194/bg-21-3015-2024, https://doi.org/10.5194/bg-21-3015-2024, 2024
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The ratio between atmospheric O2 and CO2 can be used to characterize the carbon balance at the surface. By combining a model and observations from the Hyytiälä forest (Finland), we show that using atmospheric O2 and CO2 measurements from a single height provides a weak constraint on the surface CO2 exchange because large-scale processes such as entrainment confound this signal. We therefore recommend always using multiple heights of O2 and CO2 measurements to study surface CO2 exchange.
Juliëtte C. S. Anema, Klaas Folkert Boersma, Piet Stammes, Gerbrand Koren, William Woodgate, Philipp Köhler, Christian Frankenberg, and Jacqui Stol
Biogeosciences, 21, 2297–2311, https://doi.org/10.5194/bg-21-2297-2024, https://doi.org/10.5194/bg-21-2297-2024, 2024
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To keep the Paris agreement goals within reach, negative emissions are necessary. They can be achieved with mitigation techniques, such as reforestation, which remove CO2 from the atmosphere. While governments have pinned their hopes on them, there is not yet a good set of tools to objectively determine whether negative emissions do what they promise. Here we show how satellite measurements of plant fluorescence are useful in detecting carbon uptake due to reforestation and vegetation regrowth.
Michael Steiner, Wouter Peters, Ingrid Luijkx, Stephan Henne, Huilin Chen, Samuel Hammer, and Dominik Brunner
Atmos. Chem. Phys., 24, 2759–2782, https://doi.org/10.5194/acp-24-2759-2024, https://doi.org/10.5194/acp-24-2759-2024, 2024
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The Paris Agreement increased interest in estimating greenhouse gas (GHG) emissions of individual countries, but top-down emission estimation is not yet considered policy-relevant. It is therefore paramount to reduce large errors and to build systems that are based on the newest atmospheric transport models. In this study, we present the first application of ICON-ART in the inverse modeling of GHG fluxes with an ensemble Kalman filter and present our results for European CH4 emissions.
Samuel Upton, Markus Reichstein, Fabian Gans, Wouter Peters, Basil Kraft, and Ana Bastos
Atmos. Chem. Phys., 24, 2555–2582, https://doi.org/10.5194/acp-24-2555-2024, https://doi.org/10.5194/acp-24-2555-2024, 2024
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Data-driven eddy-covariance upscaled estimates of the global land–atmosphere net CO2 exchange (NEE) show important mismatches with regional and global estimates based on atmospheric information. To address this, we create a model with a dual constraint based on bottom-up eddy-covariance data and top-down atmospheric inversion data. Our model overcomes shortcomings of each approach, producing improved NEE estimates from local to global scale, helping to reduce uncertainty in the carbon budget.
Zhendong Wu, Alex Vermeulen, Yousuke Sawa, Ute Karstens, Wouter Peters, Remco de Kok, Xin Lan, Yasuyuki Nagai, Akinori Ogi, and Oksana Tarasova
Atmos. Chem. Phys., 24, 1249–1264, https://doi.org/10.5194/acp-24-1249-2024, https://doi.org/10.5194/acp-24-1249-2024, 2024
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This study focuses on exploring the differences in calculating global surface CO2 and its growth rate, considering the impact of analysis methodologies and site selection. Our study reveals that the current global CO2 network has a good capacity to represent global surface CO2 and its growth rate, as well as trends in atmospheric CO2 mass changes. However, small differences exist in different analyses due to the impact of methodology and site selection.
Lammert Kooistra, Katja Berger, Benjamin Brede, Lukas Valentin Graf, Helge Aasen, Jean-Louis Roujean, Miriam Machwitz, Martin Schlerf, Clement Atzberger, Egor Prikaziuk, Dessislava Ganeva, Enrico Tomelleri, Holly Croft, Pablo Reyes Muñoz, Virginia Garcia Millan, Roshanak Darvishzadeh, Gerbrand Koren, Ittai Herrmann, Offer Rozenstein, Santiago Belda, Miina Rautiainen, Stein Rune Karlsen, Cláudio Figueira Silva, Sofia Cerasoli, Jon Pierre, Emine Tanır Kayıkçı, Andrej Halabuk, Esra Tunc Gormus, Frank Fluit, Zhanzhang Cai, Marlena Kycko, Thomas Udelhoven, and Jochem Verrelst
Biogeosciences, 21, 473–511, https://doi.org/10.5194/bg-21-473-2024, https://doi.org/10.5194/bg-21-473-2024, 2024
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We reviewed optical remote sensing time series (TS) studies for monitoring vegetation productivity across ecosystems. Methods were categorized into trend analysis, land surface phenology, and assimilation into statistical or dynamic vegetation models. Due to progress in machine learning, TS processing methods will diversify, while modelling strategies will advance towards holistic processing. We propose integrating methods into a digital twin to improve the understanding of vegetation dynamics.
Pierre Friedlingstein, Michael O'Sullivan, Matthew W. Jones, Robbie M. Andrew, Dorothee C. E. Bakker, Judith Hauck, Peter Landschützer, Corinne Le Quéré, Ingrid T. Luijkx, Glen P. Peters, Wouter Peters, Julia Pongratz, Clemens Schwingshackl, Stephen Sitch, Josep G. Canadell, Philippe Ciais, Robert B. Jackson, Simone R. Alin, Peter Anthoni, Leticia Barbero, Nicholas R. Bates, Meike Becker, Nicolas Bellouin, Bertrand Decharme, Laurent Bopp, Ida Bagus Mandhara Brasika, Patricia Cadule, Matthew A. Chamberlain, Naveen Chandra, Thi-Tuyet-Trang Chau, Frédéric Chevallier, Louise P. Chini, Margot Cronin, Xinyu Dou, Kazutaka Enyo, Wiley Evans, Stefanie Falk, Richard A. Feely, Liang Feng, Daniel J. Ford, Thomas Gasser, Josefine Ghattas, Thanos Gkritzalis, Giacomo Grassi, Luke Gregor, Nicolas Gruber, Özgür Gürses, Ian Harris, Matthew Hefner, Jens Heinke, Richard A. Houghton, George C. Hurtt, Yosuke Iida, Tatiana Ilyina, Andrew R. Jacobson, Atul Jain, Tereza Jarníková, Annika Jersild, Fei Jiang, Zhe Jin, Fortunat Joos, Etsushi Kato, Ralph F. Keeling, Daniel Kennedy, Kees Klein Goldewijk, Jürgen Knauer, Jan Ivar Korsbakken, Arne Körtzinger, Xin Lan, Nathalie Lefèvre, Hongmei Li, Junjie Liu, Zhiqiang Liu, Lei Ma, Greg Marland, Nicolas Mayot, Patrick C. McGuire, Galen A. McKinley, Gesa Meyer, Eric J. Morgan, David R. Munro, Shin-Ichiro Nakaoka, Yosuke Niwa, Kevin M. O'Brien, Are Olsen, Abdirahman M. Omar, Tsuneo Ono, Melf Paulsen, Denis Pierrot, Katie Pocock, Benjamin Poulter, Carter M. Powis, Gregor Rehder, Laure Resplandy, Eddy Robertson, Christian Rödenbeck, Thais M. Rosan, Jörg Schwinger, Roland Séférian, T. Luke Smallman, Stephen M. Smith, Reinel Sospedra-Alfonso, Qing Sun, Adrienne J. Sutton, Colm Sweeney, Shintaro Takao, Pieter P. Tans, Hanqin Tian, Bronte Tilbrook, Hiroyuki Tsujino, Francesco Tubiello, Guido R. van der Werf, Erik van Ooijen, Rik Wanninkhof, Michio Watanabe, Cathy Wimart-Rousseau, Dongxu Yang, Xiaojuan Yang, Wenping Yuan, Xu Yue, Sönke Zaehle, Jiye Zeng, and Bo Zheng
Earth Syst. Sci. Data, 15, 5301–5369, https://doi.org/10.5194/essd-15-5301-2023, https://doi.org/10.5194/essd-15-5301-2023, 2023
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The Global Carbon Budget 2023 describes the methodology, main results, and data sets used to quantify the anthropogenic emissions of carbon dioxide (CO2) and their partitioning among the atmosphere, land ecosystems, and the ocean over the historical period (1750–2023). These living datasets are updated every year to provide the highest transparency and traceability in the reporting of CO2, the key driver of climate change.
Tobias Christoph Valentin Werner Riess, Klaas Folkert Boersma, Ward Van Roy, Jos de Laat, Enrico Dammers, and Jasper van Vliet
Atmos. Meas. Tech., 16, 5287–5304, https://doi.org/10.5194/amt-16-5287-2023, https://doi.org/10.5194/amt-16-5287-2023, 2023
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Satellite retrievals of trace gases require prior knowledge of the vertical distribution of the pollutant, which is usually obtained from models. Using aircraft-measured vertical NO2 profiles over the North Sea in summer 2021, we evaluate the Transport Model 5 profiles used in the TROPOMI NO2 retrieval. We conclude that driven by the low horizontal resolution and the overestimated vertical mixing, resulting NO2 columns are 20 % too low. This has important implications for emission estimates.
Matthew J. McGrath, Ana Maria Roxana Petrescu, Philippe Peylin, Robbie M. Andrew, Bradley Matthews, Frank Dentener, Juraj Balkovič, Vladislav Bastrikov, Meike Becker, Gregoire Broquet, Philippe Ciais, Audrey Fortems-Cheiney, Raphael Ganzenmüller, Giacomo Grassi, Ian Harris, Matthew Jones, Jürgen Knauer, Matthias Kuhnert, Guillaume Monteil, Saqr Munassar, Paul I. Palmer, Glen P. Peters, Chunjing Qiu, Mart-Jan Schelhaas, Oksana Tarasova, Matteo Vizzarri, Karina Winkler, Gianpaolo Balsamo, Antoine Berchet, Peter Briggs, Patrick Brockmann, Frédéric Chevallier, Giulia Conchedda, Monica Crippa, Stijn N. C. Dellaert, Hugo A. C. Denier van der Gon, Sara Filipek, Pierre Friedlingstein, Richard Fuchs, Michael Gauss, Christoph Gerbig, Diego Guizzardi, Dirk Günther, Richard A. Houghton, Greet Janssens-Maenhout, Ronny Lauerwald, Bas Lerink, Ingrid T. Luijkx, Géraud Moulas, Marilena Muntean, Gert-Jan Nabuurs, Aurélie Paquirissamy, Lucia Perugini, Wouter Peters, Roberto Pilli, Julia Pongratz, Pierre Regnier, Marko Scholze, Yusuf Serengil, Pete Smith, Efisio Solazzo, Rona L. Thompson, Francesco N. Tubiello, Timo Vesala, and Sophia Walther
Earth Syst. Sci. Data, 15, 4295–4370, https://doi.org/10.5194/essd-15-4295-2023, https://doi.org/10.5194/essd-15-4295-2023, 2023
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Accurate estimation of fluxes of carbon dioxide from the land surface is essential for understanding future impacts of greenhouse gas emissions on the climate system. A wide variety of methods currently exist to estimate these sources and sinks. We are continuing work to develop annual comparisons of these diverse methods in order to clarify what they all actually calculate and to resolve apparent disagreement, in addition to highlighting opportunities for increased understanding.
Luana S. Basso, Chris Wilson, Martyn P. Chipperfield, Graciela Tejada, Henrique L. G. Cassol, Egídio Arai, Mathew Williams, T. Luke Smallman, Wouter Peters, Stijn Naus, John B. Miller, and Manuel Gloor
Atmos. Chem. Phys., 23, 9685–9723, https://doi.org/10.5194/acp-23-9685-2023, https://doi.org/10.5194/acp-23-9685-2023, 2023
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The Amazon’s carbon balance may have changed due to forest degradation, deforestation and warmer climate. We used an atmospheric model and atmospheric CO2 observations to quantify Amazonian carbon emissions (2010–2018). The region was a small carbon source to the atmosphere, mostly due to fire emissions. Forest uptake compensated for ~ 50 % of the fire emissions, meaning that the remaining forest is still a small carbon sink. We found no clear evidence of weakening carbon uptake over the period.
Ivan Cornut, Nicolas Delpierre, Jean-Paul Laclau, Joannès Guillemot, Yann Nouvellon, Otavio Campoe, Jose Luiz Stape, Vitoria Fernanda Santos, and Guerric le Maire
Biogeosciences, 20, 3093–3117, https://doi.org/10.5194/bg-20-3093-2023, https://doi.org/10.5194/bg-20-3093-2023, 2023
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Potassium is an essential element for living organisms. Trees are dependent upon this element for certain functions that allow them to build their trunks using carbon dioxide. Using data from experiments in eucalypt plantations in Brazil and a simplified computer model of the plantations, we were able to investigate the effect that a lack of potassium can have on the production of wood. Understanding nutrient cycles is useful to understand the response of forests to environmental change.
Ivan Cornut, Guerric le Maire, Jean-Paul Laclau, Joannès Guillemot, Yann Nouvellon, and Nicolas Delpierre
Biogeosciences, 20, 3119–3135, https://doi.org/10.5194/bg-20-3119-2023, https://doi.org/10.5194/bg-20-3119-2023, 2023
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After simulating the effects of low levels of potassium on the canopy of trees and the uptake of carbon dioxide from the atmosphere by leaves in Part 1, here we tried to simulate the way the trees use the carbon they have acquired and the interaction with the potassium cycle in the tree. We show that the effect of low potassium on the efficiency of the trees in acquiring carbon is enough to explain why they produce less wood when they are in soils with low levels of potassium.
Theertha Kariyathan, Ana Bastos, Julia Marshall, Wouter Peters, Pieter Tans, and Markus Reichstein
Atmos. Meas. Tech., 16, 3299–3312, https://doi.org/10.5194/amt-16-3299-2023, https://doi.org/10.5194/amt-16-3299-2023, 2023
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The timing and duration of the carbon uptake period (CUP) are sensitive to the occurrence of major phenological events, which are influenced by recent climate change. This study presents an ensemble-based approach for quantifying the timing and duration of the CUP and their uncertainty when derived from atmospheric CO2 measurements with noise and gaps. The CUP metrics derived with the approach are more robust and have less uncertainty than when estimated with the conventional methods.
Ida Storm, Ute Karstens, Claudio D'Onofrio, Alex Vermeulen, and Wouter Peters
Atmos. Chem. Phys., 23, 4993–5008, https://doi.org/10.5194/acp-23-4993-2023, https://doi.org/10.5194/acp-23-4993-2023, 2023
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In this study, we evaluate what is in the influence regions of the ICOS atmospheric measurement stations to gain insight into what land cover types and land-cover-associated fluxes the network represents. Subsequently, insights about strengths, weaknesses, and potential gaps can assist in future network expansion decisions. The network is concentrated in central Europe, which leads to a general overrepresentation of coniferous forest and cropland and underrepresentation of grass and shrubland.
Auke M. van der Woude, Remco de Kok, Naomi Smith, Ingrid T. Luijkx, Santiago Botía, Ute Karstens, Linda M. J. Kooijmans, Gerbrand Koren, Harro A. J. Meijer, Gert-Jan Steeneveld, Ida Storm, Ingrid Super, Hubertus A. Scheeren, Alex Vermeulen, and Wouter Peters
Earth Syst. Sci. Data, 15, 579–605, https://doi.org/10.5194/essd-15-579-2023, https://doi.org/10.5194/essd-15-579-2023, 2023
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To monitor the progress towards the CO2 emission goals set out in the Paris Agreement, the European Union requires an independent validation of emitted CO2. For this validation, atmospheric measurements of CO2 can be used, together with first-guess estimates of CO2 emissions and uptake. To quickly inform end users, it is imperative that this happens in near real-time. To aid these efforts, we create estimates of European CO2 exchange at high resolution in near real time.
John Douros, Henk Eskes, Jos van Geffen, K. Folkert Boersma, Steven Compernolle, Gaia Pinardi, Anne-Marlene Blechschmidt, Vincent-Henri Peuch, Augustin Colette, and Pepijn Veefkind
Geosci. Model Dev., 16, 509–534, https://doi.org/10.5194/gmd-16-509-2023, https://doi.org/10.5194/gmd-16-509-2023, 2023
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We focus on the challenges associated with comparing atmospheric composition models with satellite products such as tropospheric NO2 columns. The aim is to highlight the methodological difficulties and propose sound ways of doing such comparisons. Building on the comparisons, a new satellite product is proposed and made available, which takes advantage of higher-resolution, regional atmospheric modelling to improve estimates of troposheric NO2 columns over Europe.
Viral Shah, Daniel J. Jacob, Ruijun Dang, Lok N. Lamsal, Sarah A. Strode, Stephen D. Steenrod, K. Folkert Boersma, Sebastian D. Eastham, Thibaud M. Fritz, Chelsea Thompson, Jeff Peischl, Ilann Bourgeois, Ilana B. Pollack, Benjamin A. Nault, Ronald C. Cohen, Pedro Campuzano-Jost, Jose L. Jimenez, Simone T. Andersen, Lucy J. Carpenter, Tomás Sherwen, and Mat J. Evans
Atmos. Chem. Phys., 23, 1227–1257, https://doi.org/10.5194/acp-23-1227-2023, https://doi.org/10.5194/acp-23-1227-2023, 2023
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NOx in the free troposphere (above 2 km) affects global tropospheric chemistry and the retrieval and interpretation of satellite NO2 measurements. We evaluate free tropospheric NOx in global atmospheric chemistry models and find that recycling NOx from its reservoirs over the oceans is faster than that simulated in the models, resulting in increases in simulated tropospheric ozone and OH. Over the U.S., free tropospheric NO2 contributes the majority of the tropospheric NO2 column in summer.
Kim A. P. Faassen, Linh N. T. Nguyen, Eadin R. Broekema, Bert A. M. Kers, Ivan Mammarella, Timo Vesala, Penelope A. Pickers, Andrew C. Manning, Jordi Vilà-Guerau de Arellano, Harro A. J. Meijer, Wouter Peters, and Ingrid T. Luijkx
Atmos. Chem. Phys., 23, 851–876, https://doi.org/10.5194/acp-23-851-2023, https://doi.org/10.5194/acp-23-851-2023, 2023
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The exchange ratio (ER) between atmospheric O2 and CO2 provides a useful tracer for separately estimating photosynthesis and respiration processes in the forest carbon balance. This is highly relevant to better understand the expected biosphere sink, which determines future atmospheric CO2 levels. We therefore measured O2, CO2, and their ER above a boreal forest in Finland and investigated their diurnal behaviour for a representative day, and we show the most suitable way to determine the ER.
Qianqian Zhang, K. Folkert Boersma, Bin Zhao, Henk Eskes, Cuihong Chen, Haotian Zheng, and Xingying Zhang
Atmos. Chem. Phys., 23, 551–563, https://doi.org/10.5194/acp-23-551-2023, https://doi.org/10.5194/acp-23-551-2023, 2023
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We developed an improved superposition column model and used the latest released (v2.3.1) TROPOMI satellite NO2 observations to estimate daily city-scale NOx and CO2 emissions. The results are verified against bottom-up emissions and OCO-2 XCO2 observations. We obtained the day-to-day variation of city NOx and CO2 emissions, allowing policymakers to gain real-time information on spatial–temporal emission patterns and the effectiveness of carbon and nitrogen regulation in urban environments.
Srijana Lama, Sander Houweling, K. Folkert Boersma, Ilse Aben, Hugo A. C. Denier van der Gon, and Maarten C. Krol
Atmos. Chem. Phys., 22, 16053–16071, https://doi.org/10.5194/acp-22-16053-2022, https://doi.org/10.5194/acp-22-16053-2022, 2022
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Hydroxyl radical (OH) is the important chemical species that determines the lifetime of some greenhouse gases and trace gases. OH plays a vital role in air pollution chemistry. OH has a short lifetime and is extremely difficult to measure directly. OH concentrations derived from the chemistry transport model (CTM) have uncertainties of >50 %. Therefore, in this study, OH is derived indirectly using satellite date in urban plumes.
Stijn Naus, Lucas G. Domingues, Maarten Krol, Ingrid T. Luijkx, Luciana V. Gatti, John B. Miller, Emanuel Gloor, Sourish Basu, Caio Correia, Gerbrand Koren, Helen M. Worden, Johannes Flemming, Gabrielle Pétron, and Wouter Peters
Atmos. Chem. Phys., 22, 14735–14750, https://doi.org/10.5194/acp-22-14735-2022, https://doi.org/10.5194/acp-22-14735-2022, 2022
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We assimilate MOPITT CO satellite data in the TM5-4D-Var inverse modelling framework to estimate Amazon fire CO emissions for 2003–2018. We show that fire emissions have decreased over the analysis period, coincident with a decrease in deforestation rates. However, interannual variations in fire emissions are large, and they correlate strongly with soil moisture. Our results reveal an important role for robust, top-down fire CO emissions in quantifying and attributing Amazon fire intensity.
Pierre Friedlingstein, Michael O'Sullivan, Matthew W. Jones, Robbie M. Andrew, Luke Gregor, Judith Hauck, Corinne Le Quéré, Ingrid T. Luijkx, Are Olsen, Glen P. Peters, Wouter Peters, Julia Pongratz, Clemens Schwingshackl, Stephen Sitch, Josep G. Canadell, Philippe Ciais, Robert B. Jackson, Simone R. Alin, Ramdane Alkama, Almut Arneth, Vivek K. Arora, Nicholas R. Bates, Meike Becker, Nicolas Bellouin, Henry C. Bittig, Laurent Bopp, Frédéric Chevallier, Louise P. Chini, Margot Cronin, Wiley Evans, Stefanie Falk, Richard A. Feely, Thomas Gasser, Marion Gehlen, Thanos Gkritzalis, Lucas Gloege, Giacomo Grassi, Nicolas Gruber, Özgür Gürses, Ian Harris, Matthew Hefner, Richard A. Houghton, George C. Hurtt, Yosuke Iida, Tatiana Ilyina, Atul K. Jain, Annika Jersild, Koji Kadono, Etsushi Kato, Daniel Kennedy, Kees Klein Goldewijk, Jürgen Knauer, Jan Ivar Korsbakken, Peter Landschützer, Nathalie Lefèvre, Keith Lindsay, Junjie Liu, Zhu Liu, Gregg Marland, Nicolas Mayot, Matthew J. McGrath, Nicolas Metzl, Natalie M. Monacci, David R. Munro, Shin-Ichiro Nakaoka, Yosuke Niwa, Kevin O'Brien, Tsuneo Ono, Paul I. Palmer, Naiqing Pan, Denis Pierrot, Katie Pocock, Benjamin Poulter, Laure Resplandy, Eddy Robertson, Christian Rödenbeck, Carmen Rodriguez, Thais M. Rosan, Jörg Schwinger, Roland Séférian, Jamie D. Shutler, Ingunn Skjelvan, Tobias Steinhoff, Qing Sun, Adrienne J. Sutton, Colm Sweeney, Shintaro Takao, Toste Tanhua, Pieter P. Tans, Xiangjun Tian, Hanqin Tian, Bronte Tilbrook, Hiroyuki Tsujino, Francesco Tubiello, Guido R. van der Werf, Anthony P. Walker, Rik Wanninkhof, Chris Whitehead, Anna Willstrand Wranne, Rebecca Wright, Wenping Yuan, Chao Yue, Xu Yue, Sönke Zaehle, Jiye Zeng, and Bo Zheng
Earth Syst. Sci. Data, 14, 4811–4900, https://doi.org/10.5194/essd-14-4811-2022, https://doi.org/10.5194/essd-14-4811-2022, 2022
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The Global Carbon Budget 2022 describes the datasets and methodology used to quantify the anthropogenic emissions of carbon dioxide (CO2) and their partitioning among the atmosphere, the land ecosystems, and the ocean. These living datasets are updated every year to provide the highest transparency and traceability in the reporting of CO2, the key driver of climate change.
Pierre Friedlingstein, Matthew W. Jones, Michael O'Sullivan, Robbie M. Andrew, Dorothee C. E. Bakker, Judith Hauck, Corinne Le Quéré, Glen P. Peters, Wouter Peters, Julia Pongratz, Stephen Sitch, Josep G. Canadell, Philippe Ciais, Rob B. Jackson, Simone R. Alin, Peter Anthoni, Nicholas R. Bates, Meike Becker, Nicolas Bellouin, Laurent Bopp, Thi Tuyet Trang Chau, Frédéric Chevallier, Louise P. Chini, Margot Cronin, Kim I. Currie, Bertrand Decharme, Laique M. Djeutchouang, Xinyu Dou, Wiley Evans, Richard A. Feely, Liang Feng, Thomas Gasser, Dennis Gilfillan, Thanos Gkritzalis, Giacomo Grassi, Luke Gregor, Nicolas Gruber, Özgür Gürses, Ian Harris, Richard A. Houghton, George C. Hurtt, Yosuke Iida, Tatiana Ilyina, Ingrid T. Luijkx, Atul Jain, Steve D. Jones, Etsushi Kato, Daniel Kennedy, Kees Klein Goldewijk, Jürgen Knauer, Jan Ivar Korsbakken, Arne Körtzinger, Peter Landschützer, Siv K. Lauvset, Nathalie Lefèvre, Sebastian Lienert, Junjie Liu, Gregg Marland, Patrick C. McGuire, Joe R. Melton, David R. Munro, Julia E. M. S. Nabel, Shin-Ichiro Nakaoka, Yosuke Niwa, Tsuneo Ono, Denis Pierrot, Benjamin Poulter, Gregor Rehder, Laure Resplandy, Eddy Robertson, Christian Rödenbeck, Thais M. Rosan, Jörg Schwinger, Clemens Schwingshackl, Roland Séférian, Adrienne J. Sutton, Colm Sweeney, Toste Tanhua, Pieter P. Tans, Hanqin Tian, Bronte Tilbrook, Francesco Tubiello, Guido R. van der Werf, Nicolas Vuichard, Chisato Wada, Rik Wanninkhof, Andrew J. Watson, David Willis, Andrew J. Wiltshire, Wenping Yuan, Chao Yue, Xu Yue, Sönke Zaehle, and Jiye Zeng
Earth Syst. Sci. Data, 14, 1917–2005, https://doi.org/10.5194/essd-14-1917-2022, https://doi.org/10.5194/essd-14-1917-2022, 2022
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The Global Carbon Budget 2021 describes the data sets and methodology used to quantify the emissions of carbon dioxide and their partitioning among the atmosphere, land, and ocean. These living data are updated every year to provide the highest transparency and traceability in the reporting of CO2, the key driver of climate change.
Carlos Alberti, Frank Hase, Matthias Frey, Darko Dubravica, Thomas Blumenstock, Angelika Dehn, Paolo Castracane, Gregor Surawicz, Roland Harig, Bianca C. Baier, Caroline Bès, Jianrong Bi, Hartmut Boesch, André Butz, Zhaonan Cai, Jia Chen, Sean M. Crowell, Nicholas M. Deutscher, Dragos Ene, Jonathan E. Franklin, Omaira García, David Griffith, Bruno Grouiez, Michel Grutter, Abdelhamid Hamdouni, Sander Houweling, Neil Humpage, Nicole Jacobs, Sujong Jeong, Lilian Joly, Nicholas B. Jones, Denis Jouglet, Rigel Kivi, Ralph Kleinschek, Morgan Lopez, Diogo J. Medeiros, Isamu Morino, Nasrin Mostafavipak, Astrid Müller, Hirofumi Ohyama, Paul I. Palmer, Mahesh Pathakoti, David F. Pollard, Uwe Raffalski, Michel Ramonet, Robbie Ramsay, Mahesh Kumar Sha, Kei Shiomi, William Simpson, Wolfgang Stremme, Youwen Sun, Hiroshi Tanimoto, Yao Té, Gizaw Mengistu Tsidu, Voltaire A. Velazco, Felix Vogel, Masataka Watanabe, Chong Wei, Debra Wunch, Marcia Yamasoe, Lu Zhang, and Johannes Orphal
Atmos. Meas. Tech., 15, 2433–2463, https://doi.org/10.5194/amt-15-2433-2022, https://doi.org/10.5194/amt-15-2433-2022, 2022
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Space-borne greenhouse gas missions require ground-based validation networks capable of providing fiducial reference measurements. Here, considerable refinements of the calibration procedures for the COllaborative Carbon Column Observing Network (COCCON) are presented. Laboratory and solar side-by-side procedures for the characterization of the spectrometers have been refined and extended. Revised calibration factors for XCO2, XCO and XCH4 are provided, incorporating 47 new spectrometers.
Zhu Deng, Philippe Ciais, Zitely A. Tzompa-Sosa, Marielle Saunois, Chunjing Qiu, Chang Tan, Taochun Sun, Piyu Ke, Yanan Cui, Katsumasa Tanaka, Xin Lin, Rona L. Thompson, Hanqin Tian, Yuanzhi Yao, Yuanyuan Huang, Ronny Lauerwald, Atul K. Jain, Xiaoming Xu, Ana Bastos, Stephen Sitch, Paul I. Palmer, Thomas Lauvaux, Alexandre d'Aspremont, Clément Giron, Antoine Benoit, Benjamin Poulter, Jinfeng Chang, Ana Maria Roxana Petrescu, Steven J. Davis, Zhu Liu, Giacomo Grassi, Clément Albergel, Francesco N. Tubiello, Lucia Perugini, Wouter Peters, and Frédéric Chevallier
Earth Syst. Sci. Data, 14, 1639–1675, https://doi.org/10.5194/essd-14-1639-2022, https://doi.org/10.5194/essd-14-1639-2022, 2022
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In support of the global stocktake of the Paris Agreement on climate change, we proposed a method for reconciling the results of global atmospheric inversions with data from UNFCCC national greenhouse gas inventories (NGHGIs). Here, based on a new global harmonized database that we compiled from the UNFCCC NGHGIs and a comprehensive framework presented in this study to process the results of inversions, we compared their results of carbon dioxide (CO2), methane (CH4), and nitrous oxide (N2O).
Jos van Geffen, Henk Eskes, Steven Compernolle, Gaia Pinardi, Tijl Verhoelst, Jean-Christopher Lambert, Maarten Sneep, Mark ter Linden, Antje Ludewig, K. Folkert Boersma, and J. Pepijn Veefkind
Atmos. Meas. Tech., 15, 2037–2060, https://doi.org/10.5194/amt-15-2037-2022, https://doi.org/10.5194/amt-15-2037-2022, 2022
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Nitrogen dioxide (NO2) is one of the main data products measured by the Tropospheric Monitoring Instrument (TROPOMI) on the Sentinel-5 Precursor (S5P) satellite. This study describes improvements in the TROPOMI NO2 retrieval leading to version v2.2, operational since 1 July 2021. It compares results with previous versions v1.2–v1.4 and with Ozone Monitoring Instrument (OMI) and ground-based measurements.
Tobias Christoph Valentin Werner Riess, Klaas Folkert Boersma, Jasper van Vliet, Wouter Peters, Maarten Sneep, Henk Eskes, and Jos van Geffen
Atmos. Meas. Tech., 15, 1415–1438, https://doi.org/10.5194/amt-15-1415-2022, https://doi.org/10.5194/amt-15-1415-2022, 2022
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This paper reports on improved monitoring of ship nitrogen oxide emissions by TROPOMI. With its fantastic resolution we can identify lanes of ship nitrogen dioxide (NO2) pollution not detected from space before. The quality of TROPOMI NO2 data over sea is improved further by recent upgrades in cloud retrievals and the use of sun glint scenes. Lastly, we study the impact of COVID-19 on ship NO2 in European seas and compare the found reductions to emission estimates gained from ship-specific data.
Philippe Ciais, Ana Bastos, Frédéric Chevallier, Ronny Lauerwald, Ben Poulter, Josep G. Canadell, Gustaf Hugelius, Robert B. Jackson, Atul Jain, Matthew Jones, Masayuki Kondo, Ingrid T. Luijkx, Prabir K. Patra, Wouter Peters, Julia Pongratz, Ana Maria Roxana Petrescu, Shilong Piao, Chunjing Qiu, Celso Von Randow, Pierre Regnier, Marielle Saunois, Robert Scholes, Anatoly Shvidenko, Hanqin Tian, Hui Yang, Xuhui Wang, and Bo Zheng
Geosci. Model Dev., 15, 1289–1316, https://doi.org/10.5194/gmd-15-1289-2022, https://doi.org/10.5194/gmd-15-1289-2022, 2022
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The second phase of the Regional Carbon Cycle Assessment and Processes (RECCAP) will provide updated quantification and process understanding of CO2, CH4, and N2O emissions and sinks for ten regions of the globe. In this paper, we give definitions, review different methods, and make recommendations for estimating different components of the total land–atmosphere carbon exchange for each region in a consistent and complete approach.
Linda M. J. Kooijmans, Ara Cho, Jin Ma, Aleya Kaushik, Katherine D. Haynes, Ian Baker, Ingrid T. Luijkx, Mathijs Groenink, Wouter Peters, John B. Miller, Joseph A. Berry, Jerome Ogée, Laura K. Meredith, Wu Sun, Kukka-Maaria Kohonen, Timo Vesala, Ivan Mammarella, Huilin Chen, Felix M. Spielmann, Georg Wohlfahrt, Max Berkelhammer, Mary E. Whelan, Kadmiel Maseyk, Ulli Seibt, Roisin Commane, Richard Wehr, and Maarten Krol
Biogeosciences, 18, 6547–6565, https://doi.org/10.5194/bg-18-6547-2021, https://doi.org/10.5194/bg-18-6547-2021, 2021
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The gas carbonyl sulfide (COS) can be used to estimate photosynthesis. To adopt this approach on regional and global scales, we need biosphere models that can simulate COS exchange. So far, such models have not been evaluated against observations. We evaluate the COS biosphere exchange of the SiB4 model against COS flux observations. We find that the model is capable of simulating key processes in COS biosphere exchange. Still, we give recommendations for further improvement of the model.
Auke J. Visser, Laurens N. Ganzeveld, Ignacio Goded, Maarten C. Krol, Ivan Mammarella, Giovanni Manca, and K. Folkert Boersma
Atmos. Chem. Phys., 21, 18393–18411, https://doi.org/10.5194/acp-21-18393-2021, https://doi.org/10.5194/acp-21-18393-2021, 2021
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Dry deposition is an important sink for tropospheric ozone that affects ecosystem carbon uptake, but process understanding remains incomplete. We apply a common deposition representation in atmospheric chemistry models and a multi-layer canopy model to multi-year ozone deposition observations. The multi-layer canopy model performs better on diurnal timescales compared to the common approach, leading to a substantially improved simulation of ozone deposition and vegetation ozone impact metrics.
Thomas Luke Smallman, David Thomas Milodowski, Eráclito Sousa Neto, Gerbrand Koren, Jean Ometto, and Mathew Williams
Earth Syst. Dynam., 12, 1191–1237, https://doi.org/10.5194/esd-12-1191-2021, https://doi.org/10.5194/esd-12-1191-2021, 2021
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Our study provides a novel assessment of model parameter, structure and climate change scenario uncertainty contribution to future predictions of the Brazilian terrestrial carbon stocks to 2100. We calibrated (2001–2017) five models of the terrestrial C cycle of varied structure. The calibrated models were then projected to 2100 under multiple climate change scenarios. Parameter uncertainty dominates overall uncertainty, being ~ 40 times that of either model structure or climate change scenario.
Wouter Dorigo, Irene Himmelbauer, Daniel Aberer, Lukas Schremmer, Ivana Petrakovic, Luca Zappa, Wolfgang Preimesberger, Angelika Xaver, Frank Annor, Jonas Ardö, Dennis Baldocchi, Marco Bitelli, Günter Blöschl, Heye Bogena, Luca Brocca, Jean-Christophe Calvet, J. Julio Camarero, Giorgio Capello, Minha Choi, Michael C. Cosh, Nick van de Giesen, Istvan Hajdu, Jaakko Ikonen, Karsten H. Jensen, Kasturi Devi Kanniah, Ileen de Kat, Gottfried Kirchengast, Pankaj Kumar Rai, Jenni Kyrouac, Kristine Larson, Suxia Liu, Alexander Loew, Mahta Moghaddam, José Martínez Fernández, Cristian Mattar Bader, Renato Morbidelli, Jan P. Musial, Elise Osenga, Michael A. Palecki, Thierry Pellarin, George P. Petropoulos, Isabella Pfeil, Jarrett Powers, Alan Robock, Christoph Rüdiger, Udo Rummel, Michael Strobel, Zhongbo Su, Ryan Sullivan, Torbern Tagesson, Andrej Varlagin, Mariette Vreugdenhil, Jeffrey Walker, Jun Wen, Fred Wenger, Jean Pierre Wigneron, Mel Woods, Kun Yang, Yijian Zeng, Xiang Zhang, Marek Zreda, Stephan Dietrich, Alexander Gruber, Peter van Oevelen, Wolfgang Wagner, Klaus Scipal, Matthias Drusch, and Roberto Sabia
Hydrol. Earth Syst. Sci., 25, 5749–5804, https://doi.org/10.5194/hess-25-5749-2021, https://doi.org/10.5194/hess-25-5749-2021, 2021
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The International Soil Moisture Network (ISMN) is a community-based open-access data portal for soil water measurements taken at the ground and is accessible at https://ismn.earth. Over 1000 scientific publications and thousands of users have made use of the ISMN. The scope of this paper is to inform readers about the data and functionality of the ISMN and to provide a review of the scientific progress facilitated through the ISMN with the scope to shape future research and operations.
Antoine Berchet, Espen Sollum, Rona L. Thompson, Isabelle Pison, Joël Thanwerdas, Grégoire Broquet, Frédéric Chevallier, Tuula Aalto, Adrien Berchet, Peter Bergamaschi, Dominik Brunner, Richard Engelen, Audrey Fortems-Cheiney, Christoph Gerbig, Christine D. Groot Zwaaftink, Jean-Matthieu Haussaire, Stephan Henne, Sander Houweling, Ute Karstens, Werner L. Kutsch, Ingrid T. Luijkx, Guillaume Monteil, Paul I. Palmer, Jacob C. A. van Peet, Wouter Peters, Philippe Peylin, Elise Potier, Christian Rödenbeck, Marielle Saunois, Marko Scholze, Aki Tsuruta, and Yuanhong Zhao
Geosci. Model Dev., 14, 5331–5354, https://doi.org/10.5194/gmd-14-5331-2021, https://doi.org/10.5194/gmd-14-5331-2021, 2021
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We present here the Community Inversion Framework (CIF) to help rationalize development efforts and leverage the strengths of individual inversion systems into a comprehensive framework. The CIF is a programming protocol to allow various inversion bricks to be exchanged among researchers.
The ensemble of bricks makes a flexible, transparent and open-source Python-based tool. We describe the main structure and functionalities and demonstrate it in a simple academic case.
Isabelle De Smedt, Gaia Pinardi, Corinne Vigouroux, Steven Compernolle, Alkis Bais, Nuria Benavent, Folkert Boersma, Ka-Lok Chan, Sebastian Donner, Kai-Uwe Eichmann, Pascal Hedelt, François Hendrick, Hitoshi Irie, Vinod Kumar, Jean-Christopher Lambert, Bavo Langerock, Christophe Lerot, Cheng Liu, Diego Loyola, Ankie Piters, Andreas Richter, Claudia Rivera Cárdenas, Fabian Romahn, Robert George Ryan, Vinayak Sinha, Nicolas Theys, Jonas Vlietinck, Thomas Wagner, Ting Wang, Huan Yu, and Michel Van Roozendael
Atmos. Chem. Phys., 21, 12561–12593, https://doi.org/10.5194/acp-21-12561-2021, https://doi.org/10.5194/acp-21-12561-2021, 2021
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This paper assess the performances of the TROPOMI formaldehyde observations compared to its predecessor OMI at different spatial and temporal scales. We also use a global network of MAX-DOAS instruments to validate both satellite datasets for a large range of HCHO columns. The precision obtained with daily TROPOMI observations is comparable to monthly OMI observations. We present clear detection of weak HCHO column enhancements related to shipping emissions in the Indian Ocean.
Jianfeng Li, Yuhang Wang, Ruixiong Zhang, Charles Smeltzer, Andrew Weinheimer, Jay Herman, K. Folkert Boersma, Edward A. Celarier, Russell W. Long, James J. Szykman, Ruben Delgado, Anne M. Thompson, Travis N. Knepp, Lok N. Lamsal, Scott J. Janz, Matthew G. Kowalewski, Xiong Liu, and Caroline R. Nowlan
Atmos. Chem. Phys., 21, 11133–11160, https://doi.org/10.5194/acp-21-11133-2021, https://doi.org/10.5194/acp-21-11133-2021, 2021
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Comprehensive evaluations of simulated diurnal cycles of NO2 and NOy concentrations, vertical profiles, and tropospheric vertical column densities at two different resolutions with various measurements during the DISCOVER-AQ 2011 campaign show potential distribution biases of NOx emissions in the National Emissions Inventory 2011 at both 36 and 4 km resolutions, providing another possible explanation for the overestimation of model results.
Jaber Rahimi, Expedit Evariste Ago, Augustine Ayantunde, Sina Berger, Jan Bogaert, Klaus Butterbach-Bahl, Bernard Cappelaere, Jean-Martial Cohard, Jérôme Demarty, Abdoul Aziz Diouf, Ulrike Falk, Edwin Haas, Pierre Hiernaux, David Kraus, Olivier Roupsard, Clemens Scheer, Amit Kumar Srivastava, Torbern Tagesson, and Rüdiger Grote
Geosci. Model Dev., 14, 3789–3812, https://doi.org/10.5194/gmd-14-3789-2021, https://doi.org/10.5194/gmd-14-3789-2021, 2021
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West African Sahelian and Sudanian ecosystems are important regions for global carbon exchange, and they provide valuable food and fodder resources. Therefore, we simulated net ecosystem exchange and aboveground biomass of typical ecosystems in this region with an improved process-based biogeochemical model, LandscapeDNDC. Carbon stocks and exchange rates were particularly correlated with the abundance of trees. Grass and crop yields increased under humid climatic conditions.
Anna B. Harper, Karina E. Williams, Patrick C. McGuire, Maria Carolina Duran Rojas, Debbie Hemming, Anne Verhoef, Chris Huntingford, Lucy Rowland, Toby Marthews, Cleiton Breder Eller, Camilla Mathison, Rodolfo L. B. Nobrega, Nicola Gedney, Pier Luigi Vidale, Fred Otu-Larbi, Divya Pandey, Sebastien Garrigues, Azin Wright, Darren Slevin, Martin G. De Kauwe, Eleanor Blyth, Jonas Ardö, Andrew Black, Damien Bonal, Nina Buchmann, Benoit Burban, Kathrin Fuchs, Agnès de Grandcourt, Ivan Mammarella, Lutz Merbold, Leonardo Montagnani, Yann Nouvellon, Natalia Restrepo-Coupe, and Georg Wohlfahrt
Geosci. Model Dev., 14, 3269–3294, https://doi.org/10.5194/gmd-14-3269-2021, https://doi.org/10.5194/gmd-14-3269-2021, 2021
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We evaluated 10 representations of soil moisture stress in the JULES land surface model against site observations of GPP and latent heat flux. Increasing the soil depth and plant access to deep soil moisture improved many aspects of the simulations, and we recommend these settings in future work using JULES. In addition, using soil matric potential presents the opportunity to include parameters specific to plant functional type to further improve modeled fluxes.
Eloise A. Marais, John F. Roberts, Robert G. Ryan, Henk Eskes, K. Folkert Boersma, Sungyeon Choi, Joanna Joiner, Nader Abuhassan, Alberto Redondas, Michel Grutter, Alexander Cede, Laura Gomez, and Monica Navarro-Comas
Atmos. Meas. Tech., 14, 2389–2408, https://doi.org/10.5194/amt-14-2389-2021, https://doi.org/10.5194/amt-14-2389-2021, 2021
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Nitrogen oxides in the upper troposphere have a profound influence on the global troposphere, but routine reliable observations there are exceedingly rare. We apply cloud-slicing to TROPOMI total columns of nitrogen dioxide (NO2) at high spatial resolution to derive near-global observations of NO2 in the upper troposphere and show consistency with existing datasets. These data offer tremendous potential to address knowledge gaps in this oft underappreciated portion of the atmosphere.
Tijl Verhoelst, Steven Compernolle, Gaia Pinardi, Jean-Christopher Lambert, Henk J. Eskes, Kai-Uwe Eichmann, Ann Mari Fjæraa, José Granville, Sander Niemeijer, Alexander Cede, Martin Tiefengraber, François Hendrick, Andrea Pazmiño, Alkiviadis Bais, Ariane Bazureau, K. Folkert Boersma, Kristof Bognar, Angelika Dehn, Sebastian Donner, Aleksandr Elokhov, Manuel Gebetsberger, Florence Goutail, Michel Grutter de la Mora, Aleksandr Gruzdev, Myrto Gratsea, Georg H. Hansen, Hitoshi Irie, Nis Jepsen, Yugo Kanaya, Dimitris Karagkiozidis, Rigel Kivi, Karin Kreher, Pieternel F. Levelt, Cheng Liu, Moritz Müller, Monica Navarro Comas, Ankie J. M. Piters, Jean-Pierre Pommereau, Thierry Portafaix, Cristina Prados-Roman, Olga Puentedura, Richard Querel, Julia Remmers, Andreas Richter, John Rimmer, Claudia Rivera Cárdenas, Lidia Saavedra de Miguel, Valery P. Sinyakov, Wolfgang Stremme, Kimberly Strong, Michel Van Roozendael, J. Pepijn Veefkind, Thomas Wagner, Folkard Wittrock, Margarita Yela González, and Claus Zehner
Atmos. Meas. Tech., 14, 481–510, https://doi.org/10.5194/amt-14-481-2021, https://doi.org/10.5194/amt-14-481-2021, 2021
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This paper reports on the ground-based validation of the NO2 data produced operationally by the TROPOMI instrument on board the Sentinel-5 Precursor satellite. Tropospheric, stratospheric, and total NO2 columns are compared to measurements collected from MAX-DOAS, ZSL-DOAS, and PGN/Pandora instruments respectively. The products are found to satisfy mission requirements in general, though negative mean differences are found at sites with high pollution levels. Potential causes are discussed.
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Short summary
In this study, we assess the usefulness of Sun-Induced Fluorescence of Terrestrial Ecosystems Retrieval (SIFTER) data from the GOME-2A instrument and near-infrared reflectance of vegetation (NIRv) from MODIS to capture the seasonality and magnitudes of gross primary production (GPP) derived from six eddy-covariance flux towers in Africa in the overlap years between 2007–2014. We also test the robustness of sun-induced fluoresence and NIRv to compare the seasonality of GPP for the major biomes.
In this study, we assess the usefulness of Sun-Induced Fluorescence of Terrestrial Ecosystems...
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