Articles | Volume 13, issue 9
https://doi.org/10.5194/bg-13-2623-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/bg-13-2623-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
03 May 2016
Research article |
| 03 May 2016
Continuous CO2/CH4/CO measurements (2012–2014) at Beromünster tall tower station in Switzerland
Ece Satar
CORRESPONDING AUTHOR
Climate and Environmental Physics, Physics Institute, University of
Bern, Bern, Switzerland
Oeschger Centre for Climate Change Research, University of Bern,
Bern, Switzerland
Tesfaye A. Berhanu
Climate and Environmental Physics, Physics Institute, University of
Bern, Bern, Switzerland
Oeschger Centre for Climate Change Research, University of Bern,
Bern, Switzerland
Dominik Brunner
Empa, Laboratory for Air Pollution/Environmental Technology,
Dübendorf, Switzerland
Stephan Henne
Empa, Laboratory for Air Pollution/Environmental Technology,
Dübendorf, Switzerland
Markus Leuenberger
Climate and Environmental Physics, Physics Institute, University of
Bern, Bern, Switzerland
Oeschger Centre for Climate Change Research, University of Bern,
Bern, Switzerland
Related authors
Ece Satar, Peter Nyfeler, Céline Pascale, Bernhard Niederhauser, and Markus Leuenberger
Atmos. Meas. Tech., 13, 119–130, https://doi.org/10.5194/amt-13-119-2020, https://doi.org/10.5194/amt-13-119-2020, 2020
Short summary
Short summary
To ensure the best preparation and measurement conditions for trace gases, usage of coated materials is in demand in gas metrology and atmospheric measurement communities. In this article, the previously introduced aluminum measurement chamber is used to investigate materials such as glass, aluminum, copper, brass, steel and three different commercially available coatings. Our measurements focus on temperature and pressure dependencies for the species CO2, CO, CH4 and H2O using a CRDS analyzer.
Ece Satar, Peter Nyfeler, Bernhard Bereiter, Céline Pascale, Bernhard Niederhauser, and Markus Leuenberger
Atmos. Meas. Tech., 13, 101–117, https://doi.org/10.5194/amt-13-101-2020, https://doi.org/10.5194/amt-13-101-2020, 2020
Short summary
Short summary
Good-quality measurements of atmospheric trace gases are only possible with regular calibrations and stable measurements from the standard cylinders. This study investigates instabilities due to surface effects on newly built aluminum and steel cylinders. We present measurements over a set of temperature and pressure ranges for the amount fractions of CO2, CO, CH4 and H2O using a commercial and a novel laser spectroscopic analyzer.
Tesfaye A. Berhanu, Sönke Szidat, Dominik Brunner, Ece Satar, Rüdiger Schanda, Peter Nyfeler, Michael Battaglia, Martin Steinbacher, Samuel Hammer, and Markus Leuenberger
Atmos. Chem. Phys., 17, 10753–10766, https://doi.org/10.5194/acp-17-10753-2017, https://doi.org/10.5194/acp-17-10753-2017, 2017
Short summary
Short summary
Fossil fuel CO2 is the major contributor of anthropogenic CO2 in the atmosphere, and accurate quantification is essential to better understand the carbon cycle. Such accurate quantification can be conducted based on radiocarbon measurements. In this study, we present radiocarbon measurements from a tall tower site in Switzerland. From these measurements, we have observed seasonally varying fossil fuel CO2 contributions and a biospheric CO2 component that varies diurnally and seasonally.
Tesfaye Ayalneh Berhanu, Ece Satar, Rudiger Schanda, Peter Nyfeler, Hanspeter Moret, Dominik Brunner, Brian Oney, and Markus Leuenberger
Atmos. Meas. Tech., 9, 2603–2614, https://doi.org/10.5194/amt-9-2603-2016, https://doi.org/10.5194/amt-9-2603-2016, 2016
Short summary
Short summary
In this manuscript, we have presented Co, CO2 and CH4 measurement data from an old radio tower tower (217.5 m) at Beromunster, Switzerland. From about 2 years of continuous CO, CO2 and CH4 measurement at five different heights, we have determined a long-term reproducibility of 2.79 ppb, 0.05 ppm and 0.29 ppb for CO, CO2 and CH4, respectively, compliant with the GAW requirements. We have also observed seasonal and diurnal variation of these species.
Dominik Brunner, Ivo Suter, Leonie Bernet, Lionel Constantin, Stuart K. Grange, Pascal Rubli, Junwei Li, Jia Chen, Alessandro Bigi, and Lukas Emmenegger
EGUsphere, https://doi.org/10.5194/egusphere-2025-640, https://doi.org/10.5194/egusphere-2025-640, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
In order to support the city of Zurich in tracking its path to net-zero greenhouse gas emissions planned to be reached by 2040, a CO2 emission monitoring system was established. The system combines a dense network of CO2 sensors with a high-resolution atmospheric transport model GRAMM/GRAL. This study presents the setup of the model together with its numerous inputs and evaluates its performance in comparison with the observations from the CO2 sensor network.
Rainer Hilland, Josh Hashemi, Stavros Stagakis, Dominik Brunner, Lionel Constantin, Natascha Kljun, Betty Molinier, Samuel Hammer, Lukas Emmenegger, and Andreas Christen
EGUsphere, https://doi.org/10.5194/egusphere-2025-1088, https://doi.org/10.5194/egusphere-2025-1088, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
We present a study of simultaneously measured fluxes of carbon dioxide (CO2) and co-emitted species in the city of Zurich. Flux measurements of CO2 alone can’t be attributed to specific emission sectors, such as road transport or residential heating. We present a model which uses the measured ratios of CO2 to carbon monoxide (CO) and nitrogen oxides (NOx) as well as sector-specific reference ratios, to attribute measured fluxes to their emission sectors.
Joël Thanwerdas, Antoine Berchet, Lionel Constantin, Aki Tsuruta, Michael Steiner, Friedemann Reum, Stephan Henne, and Dominik Brunner
Geosci. Model Dev., 18, 1505–1544, https://doi.org/10.5194/gmd-18-1505-2025, https://doi.org/10.5194/gmd-18-1505-2025, 2025
Short summary
Short summary
The Community Inversion Framework (CIF) brings together methods for estimating greenhouse gas fluxes from atmospheric observations. The initial ensemble method implemented in CIF was found to be incomplete and could hardly be compared to other ensemble methods employed in the inversion community. In this paper, we present and evaluate a new implementation of the ensemble mode, building upon the initial developments.
Stuart K. Grange, Pascal Rubli, Andrea Fischer, Dominik Brunner, Christoph Hueglin, and Lukas Emmenegger
Atmos. Chem. Phys., 25, 2781–2806, https://doi.org/10.5194/acp-25-2781-2025, https://doi.org/10.5194/acp-25-2781-2025, 2025
Short summary
Short summary
Carbon dioxide (CO2) is a very important atmospheric pollutant, and to better understand the gas's source and sink dynamics, a mid-cost sensor network hosting 26 sites was deployed in and around Zurich, Switzerland. The sensor measurement performance was quantified, and natural and anthropogenic CO2 emission sources were explored with a focus on what drives high CO2 levels. The observations will be used further by others to validate what is thought to be known about CO2 emissions in the region.
Fabian Maier, Eva Falge, Maksym Gachkivskyi, Stephan Henne, Ute Karstens, Dafina Kikaj, Ingeborg Levin, Alistair Manning, Christian Rödenbeck, and Christoph Gerbig
EGUsphere, https://doi.org/10.5194/egusphere-2025-477, https://doi.org/10.5194/egusphere-2025-477, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
The radioactive noble gas radon (222Rn) is a suitable natural tracer for atmospheric transport and mixing processes that can be used to validate and calibrate atmospheric transport models. However, this requires accurate estimates of the 222Rn flux from the soil into the atmosphere. In our study, we evaluate the reliability of process-based 222Rn flux maps for Europe using a 222Rn inversion. Our inversion results can give some indications on how to improve the process-based 222Rn flux maps.
Hossein Maazallahi, Foteini Stavropoulou, Samuel Jonson Sutanto, Michael Steiner, Dominik Brunner, Mariano Mertens, Patrick Jöckel, Antoon Visschedijk, Hugo Denier van der Gon, Stijn Dellaert, Nataly Velandia Salinas, Stefan Schwietzke, Daniel Zavala-Araiza, Sorin Ghemulet, Alexandru Pana, Magdalena Ardelean, Marius Corbu, Andreea Calcan, Stephen A. Conley, Mackenzie L. Smith, and Thomas Röckmann
Atmos. Chem. Phys., 25, 1497–1511, https://doi.org/10.5194/acp-25-1497-2025, https://doi.org/10.5194/acp-25-1497-2025, 2025
Short summary
Short summary
This article presents insights from airborne in situ measurements collected during the ROmanian Methane Emissions from Oil and gas (ROMEO) campaign supported by two models. Results reveal Romania's oil and gas methane emissions were significantly under-reported to the United Nations Framework Convention on Climate Change (UNFCCC) in 2019. A large underestimation was also found in the Emissions Database for Global Atmospheric Research (EDGAR) v7.0 for the study domain in the same year.
Diego Santaren, Janne Hakkarainen, Gerrit Kuhlmann, Erik Koene, Frédéric Chevallier, Iolanda Ialongo, Hannakaisa Lindqvist, Janne Nurmela, Johanna Tamminen, Laia Amorós, Dominik Brunner, and Grégoire Broquet
Atmos. Meas. Tech., 18, 211–239, https://doi.org/10.5194/amt-18-211-2025, https://doi.org/10.5194/amt-18-211-2025, 2025
Short summary
Short summary
This study evaluates data-driven inversion methods for estimating CO2 emissions from local sources, such as power plants and cities, using meteorological data and XCO2 and NO2 satellite images rather than atmospheric transport modeling. We assess and compare the performance of five different methods using simulations of 1 year of satellite images, taken from the upcoming Copernicus CO2 Monitoring Mission, covering 15 power plants and the city of Berlin, Germany.
Stephan Räss, Peter Nyfeler, Paul Wheeler, Will Price, and Markus Christian Leuenberger
EGUsphere, https://doi.org/10.5194/egusphere-2024-3572, https://doi.org/10.5194/egusphere-2024-3572, 2025
Short summary
Short summary
Clumped-isotope signals obtained through gas-source mass spectrometry are typically small and require pressure baseline corrections. While such corrections have been developed for square-shaped peaks, we present an approach for correcting peaks with complex shapes. Our method is demonstrated using oxygen clumped isotopes measured in pure oxygen, where the peak tops are linearly increasing and/or negatively curved.
Gerrit Kuhlmann, Foteini Stavropoulou, Stefan Schwietzke, Daniel Zavala-Araiza, Andrew Thorpe, Andreas Hueni, Lukas Emmenegger, Andreea Calcan, Thomas Röckmann, and Dominik Brunner
EGUsphere, https://doi.org/10.5194/egusphere-2024-3494, https://doi.org/10.5194/egusphere-2024-3494, 2024
Short summary
Short summary
A measurement campaign in 2019 found that methane emissions from oil and gas in Romania were significantly higher than reported. In 2021, our follow-up campaign using airborne remote sensing showed a marked decreases in emissions by 20–60 % due to improved infrastructure. The study highlights the importance of measurement-based emission monitoring and illustrates the value of a multi-scale assessment integrating ground-based observations with large-scale airborne remote sensing campaigns.
Jakob Pernov, William Aeberhard, Michele Volpi, Eliza Harris, Benjamin Hohermuth, Sakiko Ishino, Ragnhild Bieltvedt Skeie, Stephan Henne, Ulas Im, Patricia Quinn, Lucia Upchurch, and Julia Schmale
EGUsphere, https://doi.org/10.5194/egusphere-2024-3379, https://doi.org/10.5194/egusphere-2024-3379, 2024
Short summary
Short summary
MSAp is a vital part of the Arctic climate system. Numerical models struggle to reproduce the seasonal cycle of MSAp. We evaluate three numerical models and one reanalysis product’s ability to simulate MSAp. We develop data-driven models for MSAp at four High Arctic stations. The data-driven models outperform the numerical models and reanalysis product and identified precursor source, chemical processing, and removal-related features as being important for modeling MSAp.
Michael Steiner, Luca Cantarello, Stephan Henne, and Dominik Brunner
Atmos. Chem. Phys., 24, 12447–12463, https://doi.org/10.5194/acp-24-12447-2024, https://doi.org/10.5194/acp-24-12447-2024, 2024
Short summary
Short summary
Atmospheric greenhouse gas inversions have great potential to independently check reported bottom-up emissions; however they are subject to large uncertainties. It is paramount to address and reduce the largest source of uncertainty, which stems from the representation of atmospheric transport in the models. In this study, we show that the use of a temporally varying flow-dependent atmospheric transport uncertainty can enhance the accuracy of emission estimation in an idealized experiment.
Lucie Bakels, Daria Tatsii, Anne Tipka, Rona Thompson, Marina Dütsch, Michael Blaschek, Petra Seibert, Katharina Baier, Silvia Bucci, Massimo Cassiani, Sabine Eckhardt, Christine Groot Zwaaftink, Stephan Henne, Pirmin Kaufmann, Vincent Lechner, Christian Maurer, Marie D. Mulder, Ignacio Pisso, Andreas Plach, Rakesh Subramanian, Martin Vojta, and Andreas Stohl
Geosci. Model Dev., 17, 7595–7627, https://doi.org/10.5194/gmd-17-7595-2024, https://doi.org/10.5194/gmd-17-7595-2024, 2024
Short summary
Short summary
Computer models are essential for improving our understanding of how gases and particles move in the atmosphere. We present an update of the atmospheric transport model FLEXPART. FLEXPART 11 is more accurate due to a reduced number of interpolations and a new scheme for wet deposition. It can simulate non-spherical aerosols and includes linear chemical reactions. It is parallelised using OpenMP and includes new user options. A new user manual details how to use FLEXPART 11.
Ana Maria Roxana Petrescu, Glen P. Peters, Richard Engelen, Sander Houweling, Dominik Brunner, Aki Tsuruta, Bradley Matthews, Prabir K. Patra, Dmitry Belikov, Rona L. Thompson, Lena Höglund-Isaksson, Wenxin Zhang, Arjo J. Segers, Giuseppe Etiope, Giancarlo Ciotoli, Philippe Peylin, Frédéric Chevallier, Tuula Aalto, Robbie M. Andrew, David Bastviken, Antoine Berchet, Grégoire Broquet, Giulia Conchedda, Stijn N. C. Dellaert, Hugo Denier van der Gon, Johannes Gütschow, Jean-Matthieu Haussaire, Ronny Lauerwald, Tiina Markkanen, Jacob C. A. van Peet, Isabelle Pison, Pierre Regnier, Espen Solum, Marko Scholze, Maria Tenkanen, Francesco N. Tubiello, Guido R. van der Werf, and John R. Worden
Earth Syst. Sci. Data, 16, 4325–4350, https://doi.org/10.5194/essd-16-4325-2024, https://doi.org/10.5194/essd-16-4325-2024, 2024
Short summary
Short summary
This study provides an overview of data availability from observation- and inventory-based CH4 emission estimates. It systematically compares them and provides recommendations for robust comparisons, aiming to steadily engage more parties in using observational methods to complement their UNFCCC submissions. Anticipating improvements in atmospheric modelling and observations, future developments need to resolve knowledge gaps in both approaches and to better quantify remaining uncertainty.
Stavros Stagakis, Dominik Brunner, Junwei Li, Leif Backman, Anni Karvonen, Lionel Constantin, Leena Järvi, Minttu Havu, Jia Chen, Sophie Emberger, and Liisa Kulmala
EGUsphere, https://doi.org/10.5194/egusphere-2024-2475, https://doi.org/10.5194/egusphere-2024-2475, 2024
Short summary
Short summary
The balance between CO2 uptake and emissions from urban green areas is still not well understood. This study evaluated for the first time the urban park CO2 exchange simulations by four different types of biosphere models by comparing them with observations. Even though some advantages and disadvantages of the different model types were identified, there was no strong evidence that more complex models performed better than simple ones.
Sandro Meier, Erik F. M. Koene, Maarten Krol, Dominik Brunner, Alexander Damm, and Gerrit Kuhlmann
Atmos. Chem. Phys., 24, 7667–7686, https://doi.org/10.5194/acp-24-7667-2024, https://doi.org/10.5194/acp-24-7667-2024, 2024
Short summary
Short summary
Nitrogen oxides (NOx = NO + NO2) are important air pollutants. This study addresses the challenge of accurately estimating NOx emissions from NO2 satellite observations. We develop a realistic model to convert NO2 to NOx by using simulated plumes from various power plants. We apply the model to satellite NO2 observations, significantly reducing biases in estimated NOx emissions. The study highlights the potential for a consistent, high-resolution estimation of NOx emissions using satellite data.
Gerrit Kuhlmann, Erik Koene, Sandro Meier, Diego Santaren, Grégoire Broquet, Frédéric Chevallier, Janne Hakkarainen, Janne Nurmela, Laia Amorós, Johanna Tamminen, and Dominik Brunner
Geosci. Model Dev., 17, 4773–4789, https://doi.org/10.5194/gmd-17-4773-2024, https://doi.org/10.5194/gmd-17-4773-2024, 2024
Short summary
Short summary
We present a Python software library for data-driven emission quantification (ddeq). It can be used to determine the emissions of hot spots (cities, power plants and industry) from remote sensing images using different methods. ddeq can be extended for new datasets and methods, providing a powerful community tool for users and developers. The application of the methods is shown using Jupyter notebooks included in the library.
Michael Steiner, Wouter Peters, Ingrid Luijkx, Stephan Henne, Huilin Chen, Samuel Hammer, and Dominik Brunner
Atmos. Chem. Phys., 24, 2759–2782, https://doi.org/10.5194/acp-24-2759-2024, https://doi.org/10.5194/acp-24-2759-2024, 2024
Short summary
Short summary
The Paris Agreement increased interest in estimating greenhouse gas (GHG) emissions of individual countries, but top-down emission estimation is not yet considered policy-relevant. It is therefore paramount to reduce large errors and to build systems that are based on the newest atmospheric transport models. In this study, we present the first application of ICON-ART in the inverse modeling of GHG fluxes with an ensemble Kalman filter and present our results for European CH4 emissions.
Robert Hanfland, Dominik Brunner, Christiane Voigt, Alina Fiehn, Anke Roiger, and Margit Pattantyús-Ábrahám
Atmos. Chem. Phys., 24, 2511–2534, https://doi.org/10.5194/acp-24-2511-2024, https://doi.org/10.5194/acp-24-2511-2024, 2024
Short summary
Short summary
To show that the three-dimensional dispersion of plumes simulated by the Atmospheric Radionuclide Transport Model within the planetary boundary layer agrees with real plumes, we identify the most important input parameters and analyse the turbulence properties of five different turbulence models in very unstable stratification conditions using their deviation from the well-mixed state. Simulations show that one model agrees slightly better in unstable stratification conditions.
Ioannis Katharopoulos, Dominique Rust, Martin K. Vollmer, Dominik Brunner, Stefan Reimann, Simon J. O'Doherty, Dickon Young, Kieran M. Stanley, Tanja Schuck, Jgor Arduini, Lukas Emmenegger, and Stephan Henne
Atmos. Chem. Phys., 23, 14159–14186, https://doi.org/10.5194/acp-23-14159-2023, https://doi.org/10.5194/acp-23-14159-2023, 2023
Short summary
Short summary
The effectiveness of climate change mitigation needs to be scrutinized by monitoring greenhouse gas (GHG) emissions. Countries report their emissions to the UN in a bottom-up manner. By combining atmospheric observations and transport models someone can independently validate emission estimates in a top-down fashion. We report Swiss emissions of synthetic GHGs based on kilometer-scale transport and inverse modeling, highlighting the role of appropriate resolution in complex terrain.
Marie Bouchet, Amaëlle Landais, Antoine Grisart, Frédéric Parrenin, Frédéric Prié, Roxanne Jacob, Elise Fourré, Emilie Capron, Dominique Raynaud, Vladimir Ya Lipenkov, Marie-France Loutre, Thomas Extier, Anders Svensson, Etienne Legrain, Patricia Martinerie, Markus Leuenberger, Wei Jiang, Florian Ritterbusch, Zheng-Tian Lu, and Guo-Min Yang
Clim. Past, 19, 2257–2286, https://doi.org/10.5194/cp-19-2257-2023, https://doi.org/10.5194/cp-19-2257-2023, 2023
Short summary
Short summary
A new federative chronology for five deep polar ice cores retrieves 800 000 years of past climate variations with improved accuracy. Precise ice core timescales are key to studying the mechanisms linking changes in the Earth’s orbit to the diverse climatic responses (temperature and atmospheric greenhouse gas concentrations). To construct the chronology, new measurements from the oldest continuous ice core as well as glaciological modeling estimates were combined in a statistical model.
Stephan Räss, Peter Nyfeler, Paul Wheeler, Will Price, and Markus Christian Leuenberger
Atmos. Meas. Tech., 16, 4489–4505, https://doi.org/10.5194/amt-16-4489-2023, https://doi.org/10.5194/amt-16-4489-2023, 2023
Short summary
Short summary
Due to technological advances clumped-isotope studies have gained importance in recent years. Typically, these studies are performed with high-resolution isotope ratio mass spectrometers (IRMSs) along with a changeover-valve-based dual-inlet system (DIS). We are taking a different approach, namely performing clumped-isotope measurements with a compact low-resolution IRMS with an open-split-based DIS. Currently, we are working with pure-oxygen gas for which we are providing a proof of concept.
Jenny Maccali, Anna Nele Meckler, Stein-Erik Lauritzen, Torill Brekken, Helen Aase Rokkan, Alvaro Fernandez, Yves Krüger, Jane Adigun, Stéphane Affolter, and Markus Leuenberger
Clim. Past, 19, 1847–1862, https://doi.org/10.5194/cp-19-1847-2023, https://doi.org/10.5194/cp-19-1847-2023, 2023
Short summary
Short summary
The southern coast of South Africa hosts some key archeological sites for the study of early human evolution. Here we present a short but high-resolution record of past changes in the hydroclimate and temperature on the southern coast of South Africa based on the study of a speleothem collected from Bloukrantz Cave. Overall, the paleoclimate indicators suggest stable temperature from 48.3 to 45.2 ka, whereas precipitation was variable, with marked short drier episodes.
Foteini Stavropoulou, Katarina Vinković, Bert Kers, Marcel de Vries, Steven van Heuven, Piotr Korbeń, Martina Schmidt, Julia Wietzel, Pawel Jagoda, Jaroslav M. Necki, Jakub Bartyzel, Hossein Maazallahi, Malika Menoud, Carina van der Veen, Sylvia Walter, Béla Tuzson, Jonas Ravelid, Randulph Paulo Morales, Lukas Emmenegger, Dominik Brunner, Michael Steiner, Arjan Hensen, Ilona Velzeboer, Pim van den Bulk, Hugo Denier van der Gon, Antonio Delre, Maklawe Essonanawe Edjabou, Charlotte Scheutz, Marius Corbu, Sebastian Iancu, Denisa Moaca, Alin Scarlat, Alexandru Tudor, Ioana Vizireanu, Andreea Calcan, Magdalena Ardelean, Sorin Ghemulet, Alexandru Pana, Aurel Constantinescu, Lucian Cusa, Alexandru Nica, Calin Baciu, Cristian Pop, Andrei Radovici, Alexandru Mereuta, Horatiu Stefanie, Alexandru Dandocsi, Bas Hermans, Stefan Schwietzke, Daniel Zavala-Araiza, Huilin Chen, and Thomas Röckmann
Atmos. Chem. Phys., 23, 10399–10412, https://doi.org/10.5194/acp-23-10399-2023, https://doi.org/10.5194/acp-23-10399-2023, 2023
Short summary
Short summary
In this study, we quantify CH4 emissions from onshore oil production sites in Romania at source and facility level using a combination of ground- and drone-based measurement techniques. We show that the total CH4 emissions in our studied areas are much higher than the emissions reported to UNFCCC, and up to three-quarters of the detected emissions are related to operational venting. Our results suggest that oil and gas production infrastructure in Romania holds a massive mitigation potential.
Alison L. Redington, Alistair J. Manning, Stephan Henne, Francesco Graziosi, Luke M. Western, Jgor Arduini, Anita L. Ganesan, Christina M. Harth, Michela Maione, Jens Mühle, Simon O'Doherty, Joseph Pitt, Stefan Reimann, Matthew Rigby, Peter K. Salameh, Peter G. Simmonds, T. Gerard Spain, Kieran Stanley, Martin K. Vollmer, Ray F. Weiss, and Dickon Young
Atmos. Chem. Phys., 23, 7383–7398, https://doi.org/10.5194/acp-23-7383-2023, https://doi.org/10.5194/acp-23-7383-2023, 2023
Short summary
Short summary
Chlorofluorocarbons (CFCs) were used in Europe pre-1990, damaging the stratospheric ozone layer. Legislation has controlled production and use, and global emissions have decreased sharply. The global rate of decline in CFC-11 recently slowed and was partly attributed to illegal emission in eastern China. This study concludes that emissions of CFC-11 in western Europe have not contributed to the unexplained part of the global increase in CFC-11 observed in the last decade.
Ana Maria Roxana Petrescu, Chunjing Qiu, Matthew J. McGrath, Philippe Peylin, Glen P. Peters, Philippe Ciais, Rona L. Thompson, Aki Tsuruta, Dominik Brunner, Matthias Kuhnert, Bradley Matthews, Paul I. Palmer, Oksana Tarasova, Pierre Regnier, Ronny Lauerwald, David Bastviken, Lena Höglund-Isaksson, Wilfried Winiwarter, Giuseppe Etiope, Tuula Aalto, Gianpaolo Balsamo, Vladislav Bastrikov, Antoine Berchet, Patrick Brockmann, Giancarlo Ciotoli, Giulia Conchedda, Monica Crippa, Frank Dentener, Christine D. Groot Zwaaftink, Diego Guizzardi, Dirk Günther, Jean-Matthieu Haussaire, Sander Houweling, Greet Janssens-Maenhout, Massaer Kouyate, Adrian Leip, Antti Leppänen, Emanuele Lugato, Manon Maisonnier, Alistair J. Manning, Tiina Markkanen, Joe McNorton, Marilena Muntean, Gabriel D. Oreggioni, Prabir K. Patra, Lucia Perugini, Isabelle Pison, Maarit T. Raivonen, Marielle Saunois, Arjo J. Segers, Pete Smith, Efisio Solazzo, Hanqin Tian, Francesco N. Tubiello, Timo Vesala, Guido R. van der Werf, Chris Wilson, and Sönke Zaehle
Earth Syst. Sci. Data, 15, 1197–1268, https://doi.org/10.5194/essd-15-1197-2023, https://doi.org/10.5194/essd-15-1197-2023, 2023
Short summary
Short summary
This study updates the state-of-the-art scientific overview of CH4 and N2O emissions in the EU27 and UK in Petrescu et al. (2021a). Yearly updates are needed to improve the different respective approaches and to inform on the development of formal verification systems. It integrates the most recent emission inventories, process-based model and regional/global inversions, comparing them with UNFCCC national GHG inventories, in support to policy to facilitate real-time verification procedures.
Dominik Brunner, Gerrit Kuhlmann, Stephan Henne, Erik Koene, Bastian Kern, Sebastian Wolff, Christiane Voigt, Patrick Jöckel, Christoph Kiemle, Anke Roiger, Alina Fiehn, Sven Krautwurst, Konstantin Gerilowski, Heinrich Bovensmann, Jakob Borchardt, Michal Galkowski, Christoph Gerbig, Julia Marshall, Andrzej Klonecki, Pascal Prunet, Robert Hanfland, Margit Pattantyús-Ábrahám, Andrzej Wyszogrodzki, and Andreas Fix
Atmos. Chem. Phys., 23, 2699–2728, https://doi.org/10.5194/acp-23-2699-2023, https://doi.org/10.5194/acp-23-2699-2023, 2023
Short summary
Short summary
We evaluated six atmospheric transport models for their capability to simulate the CO2 plumes from two of the largest power plants in Europe by comparing the models against aircraft observations collected during the CoMet (Carbon Dioxide and Methane Mission) campaign in 2018. The study analyzed how realistically such plumes can be simulated at different model resolutions and how well the planned European satellite mission CO2M will be able to quantify emissions from power plants.
Andreas Plach, Rolf Rüfenacht, Simone Kotthaus, and Markus Leuenberger
EGUsphere, https://doi.org/10.5194/egusphere-2022-1019, https://doi.org/10.5194/egusphere-2022-1019, 2022
Preprint archived
Short summary
Short summary
Greenhouse gases emissions are contributing to global warming and it is essential to better understand where they originate from and how they are transported. In this study we analyze greenhouse gas observations at a Swiss tall tower where measurements are taken more than 200 m above ground and investigate their origin by looking at the condition of the atmosphere at the time of the observations. We find that most pollution at this site is caused from emissions transported from further away.
Prabhakar Shrestha, Jana Mendrok, and Dominik Brunner
Atmos. Chem. Phys., 22, 14095–14117, https://doi.org/10.5194/acp-22-14095-2022, https://doi.org/10.5194/acp-22-14095-2022, 2022
Short summary
Short summary
The study extends the Terrestrial Systems Modeling Platform with gas-phase chemistry aerosol dynamics and a radar forward operator to enable detailed studies of aerosol–cloud–precipitation interactions. This is demonstrated using a case study of a deep convective storm, which showed that the strong updraft in the convective core of the storm produced aerosol-tower-like features, which affected the size of the hydrometeors and the simulated polarimetric features (e.g., ZDR and KDP columns).
Peter Bergamaschi, Arjo Segers, Dominik Brunner, Jean-Matthieu Haussaire, Stephan Henne, Michel Ramonet, Tim Arnold, Tobias Biermann, Huilin Chen, Sebastien Conil, Marc Delmotte, Grant Forster, Arnoud Frumau, Dagmar Kubistin, Xin Lan, Markus Leuenberger, Matthias Lindauer, Morgan Lopez, Giovanni Manca, Jennifer Müller-Williams, Simon O'Doherty, Bert Scheeren, Martin Steinbacher, Pamela Trisolino, Gabriela Vítková, and Camille Yver Kwok
Atmos. Chem. Phys., 22, 13243–13268, https://doi.org/10.5194/acp-22-13243-2022, https://doi.org/10.5194/acp-22-13243-2022, 2022
Short summary
Short summary
We present a novel high-resolution inverse modelling system, "FLEXVAR", and its application for the inverse modelling of European CH4 emissions in 2018. The new system combines a high spatial resolution of 7 km x 7 km with a variational data assimilation technique, which allows CH4 emissions to be optimized from individual model grid cells. The high resolution allows the observations to be better reproduced, while the derived emissions show overall good consistency with two existing models.
Simone M. Pieber, Béla Tuzson, Stephan Henne, Ute Karstens, Christoph Gerbig, Frank-Thomas Koch, Dominik Brunner, Martin Steinbacher, and Lukas Emmenegger
Atmos. Chem. Phys., 22, 10721–10749, https://doi.org/10.5194/acp-22-10721-2022, https://doi.org/10.5194/acp-22-10721-2022, 2022
Short summary
Short summary
Understanding regional greenhouse gas emissions into the atmosphere is a prerequisite to mitigate climate change. In this study, we investigated the regional contributions of carbon dioxide (CO2) at the location of the high Alpine observatory Jungfraujoch (JFJ, Switzerland, 3580 m a.s.l.). To this purpose, we combined receptor-oriented atmospheric transport simulations for CO2 concentration in the period 2009–2017 with stable carbon isotope (δ13C–CO2) information.
Luke M. Western, Alison L. Redington, Alistair J. Manning, Cathy M. Trudinger, Lei Hu, Stephan Henne, Xuekun Fang, Lambert J. M. Kuijpers, Christina Theodoridi, David S. Godwin, Jgor Arduini, Bronwyn Dunse, Andreas Engel, Paul J. Fraser, Christina M. Harth, Paul B. Krummel, Michela Maione, Jens Mühle, Simon O'Doherty, Hyeri Park, Sunyoung Park, Stefan Reimann, Peter K. Salameh, Daniel Say, Roland Schmidt, Tanja Schuck, Carolina Siso, Kieran M. Stanley, Isaac Vimont, Martin K. Vollmer, Dickon Young, Ronald G. Prinn, Ray F. Weiss, Stephen A. Montzka, and Matthew Rigby
Atmos. Chem. Phys., 22, 9601–9616, https://doi.org/10.5194/acp-22-9601-2022, https://doi.org/10.5194/acp-22-9601-2022, 2022
Short summary
Short summary
The production of ozone-destroying gases is being phased out. Even though production of one of the main ozone-depleting gases, called HCFC-141b, has been declining for many years, the amount that is being released to the atmosphere has been increasing since 2017. We do not know for sure why this is. A possible explanation is that HCFC-141b that was used to make insulating foams many years ago is only now escaping to the atmosphere, or a large part of its production is not being reported.
Horim Kim, Michael Müller, Stephan Henne, and Christoph Hüglin
Atmos. Meas. Tech., 15, 2979–2992, https://doi.org/10.5194/amt-15-2979-2022, https://doi.org/10.5194/amt-15-2979-2022, 2022
Short summary
Short summary
In this study, the performance of electrochemical sensors for NO and NO2 for measuring air quality was determined over a longer operating period. The performance of NO sensors remained reliable for more than 18 months. However, the NO2 sensors showed decreasing performance over time. During deployment, we found that the NO2 sensors can distinguish general pollution levels, but they proved unsuitable for accurate measurements due to significant biases.
Randulph Morales, Jonas Ravelid, Katarina Vinkovic, Piotr Korbeń, Béla Tuzson, Lukas Emmenegger, Huilin Chen, Martina Schmidt, Sebastian Humbel, and Dominik Brunner
Atmos. Meas. Tech., 15, 2177–2198, https://doi.org/10.5194/amt-15-2177-2022, https://doi.org/10.5194/amt-15-2177-2022, 2022
Short summary
Short summary
Mapping trace gas emission plumes using in situ measurements from unmanned aerial vehicles (UAVs) is an emerging and attractive possibility to quantify emissions from localized sources. We performed an extensive controlled-release experiment to develop an optimal quantification method and to determine the related uncertainties under various environmental and sampling conditions. Our approach was successful in quantifying local methane sources from drone-based measurements.
Gerrit Kuhlmann, Ka Lok Chan, Sebastian Donner, Ying Zhu, Marc Schwaerzel, Steffen Dörner, Jia Chen, Andreas Hueni, Duc Hai Nguyen, Alexander Damm, Annette Schütt, Florian Dietrich, Dominik Brunner, Cheng Liu, Brigitte Buchmann, Thomas Wagner, and Mark Wenig
Atmos. Meas. Tech., 15, 1609–1629, https://doi.org/10.5194/amt-15-1609-2022, https://doi.org/10.5194/amt-15-1609-2022, 2022
Short summary
Short summary
Nitrogen dioxide (NO2) is an air pollutant whose concentration often exceeds air quality guideline values, especially in urban areas. To map the spatial distribution of NO2 in Munich, we conducted the Munich NO2 Imaging Campaign (MuNIC), where NO2 was measured with stationary, mobile, and airborne in situ and remote sensing instruments. The campaign provides a unique dataset that has been used to compare the different instruments and to study the spatial variability of NO2 and its sources.
Dominique Rust, Ioannis Katharopoulos, Martin K. Vollmer, Stephan Henne, Simon O'Doherty, Daniel Say, Lukas Emmenegger, Renato Zenobi, and Stefan Reimann
Atmos. Chem. Phys., 22, 2447–2466, https://doi.org/10.5194/acp-22-2447-2022, https://doi.org/10.5194/acp-22-2447-2022, 2022
Short summary
Short summary
Artificial halocarbons contribute to ozone layer depletion and to global warming. We measured the atmospheric concentrations of halocarbons at the Beromünster tower, modelled the Swiss emissions, and compared the results to the internationally reported Swiss emissions inventory. For most of the halocarbons, we found good agreement, whereas one refrigerant might be overestimated in the inventory. In addition, we present first emission estimates of the newest types of halocarbons.
Cyril Brunner, Benjamin T. Brem, Martine Collaud Coen, Franz Conen, Maxime Hervo, Stephan Henne, Martin Steinbacher, Martin Gysel-Beer, and Zamin A. Kanji
Atmos. Chem. Phys., 21, 18029–18053, https://doi.org/10.5194/acp-21-18029-2021, https://doi.org/10.5194/acp-21-18029-2021, 2021
Short summary
Short summary
Special microscopic particles called ice-nucleating particles (INPs) are essential for ice crystals to form in the atmosphere. INPs are sparse and their atmospheric concentration and properties are not well understood. Mineral dust particles make up a significant fraction of INPs but how much remains unknown. Here, we address this knowledge gap by studying periods when mineral particles are present in large quantities at a mountaintop station in central Europe.
Larissa Lacher, Hans-Christian Clemen, Xiaoli Shen, Stephan Mertes, Martin Gysel-Beer, Alireza Moallemi, Martin Steinbacher, Stephan Henne, Harald Saathoff, Ottmar Möhler, Kristina Höhler, Thea Schiebel, Daniel Weber, Jann Schrod, Johannes Schneider, and Zamin A. Kanji
Atmos. Chem. Phys., 21, 16925–16953, https://doi.org/10.5194/acp-21-16925-2021, https://doi.org/10.5194/acp-21-16925-2021, 2021
Short summary
Short summary
We investigate ice-nucleating particle properties at Jungfraujoch during the 2017 joint INUIT/CLACE field campaign, to improve the knowledge about those rare particles in a cloud-relevant environment. By quantifying ice-nucleating particles in parallel to single-particle mass spectrometry measurements, we find that mineral dust and aged sea spray particles are potential candidates for ice-nucleating particles. Our findings are supported by ice residual analysis and source region modeling.
Marc Schwaerzel, Dominik Brunner, Fabian Jakub, Claudia Emde, Brigitte Buchmann, Alexis Berne, and Gerrit Kuhlmann
Atmos. Meas. Tech., 14, 6469–6482, https://doi.org/10.5194/amt-14-6469-2021, https://doi.org/10.5194/amt-14-6469-2021, 2021
Short summary
Short summary
NO2 maps from airborne imaging remote sensing often appear much smoother than one would expect from high-resolution model simulations of NO2 over cities, despite the small ground-pixel size of the sensors. Our case study over Zurich, using the newly implemented building module of the MYSTIC radiative transfer solver, shows that the 3D effect can explain part of the smearing and that building shadows cause a noticeable underestimation and noise in the measured NO2 columns.
Antoine Berchet, Espen Sollum, Rona L. Thompson, Isabelle Pison, Joël Thanwerdas, Grégoire Broquet, Frédéric Chevallier, Tuula Aalto, Adrien Berchet, Peter Bergamaschi, Dominik Brunner, Richard Engelen, Audrey Fortems-Cheiney, Christoph Gerbig, Christine D. Groot Zwaaftink, Jean-Matthieu Haussaire, Stephan Henne, Sander Houweling, Ute Karstens, Werner L. Kutsch, Ingrid T. Luijkx, Guillaume Monteil, Paul I. Palmer, Jacob C. A. van Peet, Wouter Peters, Philippe Peylin, Elise Potier, Christian Rödenbeck, Marielle Saunois, Marko Scholze, Aki Tsuruta, and Yuanhong Zhao
Geosci. Model Dev., 14, 5331–5354, https://doi.org/10.5194/gmd-14-5331-2021, https://doi.org/10.5194/gmd-14-5331-2021, 2021
Short summary
Short summary
We present here the Community Inversion Framework (CIF) to help rationalize development efforts and leverage the strengths of individual inversion systems into a comprehensive framework. The CIF is a programming protocol to allow various inversion bricks to be exchanged among researchers.
The ensemble of bricks makes a flexible, transparent and open-source Python-based tool. We describe the main structure and functionalities and demonstrate it in a simple academic case.
Dac-Loc Nguyen, Hendryk Czech, Simone M. Pieber, Jürgen Schnelle-Kreis, Martin Steinbacher, Jürgen Orasche, Stephan Henne, Olga B. Popovicheva, Gülcin Abbaszade, Guenter Engling, Nicolas Bukowiecki, Nhat-Anh Nguyen, Xuan-Anh Nguyen, and Ralf Zimmermann
Atmos. Chem. Phys., 21, 8293–8312, https://doi.org/10.5194/acp-21-8293-2021, https://doi.org/10.5194/acp-21-8293-2021, 2021
Short summary
Short summary
Southeast Asia is well-known for emission-intense and recurring wildfires and after-harvest crop residue burning during the pre-monsoon season from February to April. We describe a biomass burning (BB) plume arriving at remote Pha Din meteorological station, outline its carbonaceous particulate matter (PM) constituents based on more than 50 target compounds and discuss possible BB sources. This study adds valuable information on chemical PM composition for a region with scarce data availability.
Ana Maria Roxana Petrescu, Chunjing Qiu, Philippe Ciais, Rona L. Thompson, Philippe Peylin, Matthew J. McGrath, Efisio Solazzo, Greet Janssens-Maenhout, Francesco N. Tubiello, Peter Bergamaschi, Dominik Brunner, Glen P. Peters, Lena Höglund-Isaksson, Pierre Regnier, Ronny Lauerwald, David Bastviken, Aki Tsuruta, Wilfried Winiwarter, Prabir K. Patra, Matthias Kuhnert, Gabriel D. Oreggioni, Monica Crippa, Marielle Saunois, Lucia Perugini, Tiina Markkanen, Tuula Aalto, Christine D. Groot Zwaaftink, Hanqin Tian, Yuanzhi Yao, Chris Wilson, Giulia Conchedda, Dirk Günther, Adrian Leip, Pete Smith, Jean-Matthieu Haussaire, Antti Leppänen, Alistair J. Manning, Joe McNorton, Patrick Brockmann, and Albertus Johannes Dolman
Earth Syst. Sci. Data, 13, 2307–2362, https://doi.org/10.5194/essd-13-2307-2021, https://doi.org/10.5194/essd-13-2307-2021, 2021
Short summary
Short summary
This study is topical and provides a state-of-the-art scientific overview of data availability from bottom-up and top-down CH4 and N2O emissions in the EU27 and UK. The data integrate recent emission inventories with process-based model data and regional/global inversions for the European domain, aiming at reconciling them with official country-level UNFCCC national GHG inventories in support to policy and to facilitate real-time verification procedures.
Gerrit Kuhlmann, Dominik Brunner, Grégoire Broquet, and Yasjka Meijer
Atmos. Meas. Tech., 13, 6733–6754, https://doi.org/10.5194/amt-13-6733-2020, https://doi.org/10.5194/amt-13-6733-2020, 2020
Short summary
Short summary
The European CO2M mission is a proposed constellation of CO2 imaging satellites expected to monitor CO2 emissions of large cities. Using synthetic observations, we show that a constellation of two or more satellites should be able to quantify Berlin's annual emissions with 10–20 % accuracy, even when considering atmospheric transport model errors. We therefore expect that CO2M will make an important contribution to the monitoring and verification of CO2 emissions from cities worldwide.
Tito Arosio, Malin M. Ziehmer-Wenz, Kurt Nicolussi, Christian Schlüchter, and Markus Leuenberger
Biogeosciences Discuss., https://doi.org/10.5194/bg-2020-406, https://doi.org/10.5194/bg-2020-406, 2020
Revised manuscript not accepted
Short summary
Short summary
A recent analysis of stable isotopes of samples from larch and cembran trees, revealed that δD and δ18O exhibit no trends in adult trees, but trends in the juvenile period. In this work we applied a correlation analysis on different cambial age to verify if these changes were correlated with tree-ring width values. The results prove a significant correlation between tree-ring-width and both hydrogen and oxygen stable isotopes before 100 year of cambial age, but not afterwards, in both species.
Ying Zhu, Jia Chen, Xiao Bi, Gerrit Kuhlmann, Ka Lok Chan, Florian Dietrich, Dominik Brunner, Sheng Ye, and Mark Wenig
Atmos. Chem. Phys., 20, 13241–13251, https://doi.org/10.5194/acp-20-13241-2020, https://doi.org/10.5194/acp-20-13241-2020, 2020
Short summary
Short summary
Average NO2 concentration of on-street mobile measurements (MMs) near the monitoring stations (MSs) was found to be considerably higher than the MSs data. The common measurement height (H) and distance (D) of the MSs result in 27 % lower average concentrations in total than the concentration of our MMs. Another 21 % difference remained after correcting the influence of the measuring H and D. This result makes our city-wide measurements for capturing the full range of concentrations necessary.
Rachel L. Tunnicliffe, Anita L. Ganesan, Robert J. Parker, Hartmut Boesch, Nicola Gedney, Benjamin Poulter, Zhen Zhang, Jošt V. Lavrič, David Walter, Matthew Rigby, Stephan Henne, Dickon Young, and Simon O'Doherty
Atmos. Chem. Phys., 20, 13041–13067, https://doi.org/10.5194/acp-20-13041-2020, https://doi.org/10.5194/acp-20-13041-2020, 2020
Short summary
Short summary
This study quantifies Brazil’s emissions of a potent atmospheric greenhouse gas, methane. This is in the field of atmospheric modelling and uses remotely sensed data and surface measurements of methane concentrations as well as an atmospheric transport model to interpret the data. Because of Brazil’s large emissions from wetlands, agriculture and biomass burning, these emissions affect global methane concentrations and thus are of global significance.
Tito Arosio, Malin M. Ziehmer, Kurt Nicolussi, Christian Schlüchter, and Markus Leuenberger
Biogeosciences, 17, 4871–4882, https://doi.org/10.5194/bg-17-4871-2020, https://doi.org/10.5194/bg-17-4871-2020, 2020
Short summary
Short summary
Stable isotopes in tree-ring cellulose are tools for climatic reconstructions, but interpretation is challenging due to nonclimate trends. We analyzed the tree-age trends in tree-ring isotopes of deciduous larch and evergreen cembran pine. Samples covering the whole Holocene were collected at the tree line in the Alps. For cambial ages over 100 years, we prove the absence of age trends in δD, δ18O, and δ13C for both species. For lower cambial ages, trends differ for each isotope and species.
Michael Döring and Markus Christian Leuenberger
Clim. Past Discuss., https://doi.org/10.5194/cp-2020-132, https://doi.org/10.5194/cp-2020-132, 2020
Manuscript not accepted for further review
Short summary
Short summary
We analyze Holocene temperatures reconstructed from gas-stable-isotope species measured on ancient air extracted from a Greenland ice core. Also, we compare two state of the art firn-models which are needed for the inversion of the gas-isotope data to paleo-temperature and provide detailed uncertainty estimations for the reconstructed temperature estimates. Finally, we compare our reconstructed temperatures to two recent reconstructions based on the same gas-isotope data as used here.
Marc Schwaerzel, Claudia Emde, Dominik Brunner, Randulph Morales, Thomas Wagner, Alexis Berne, Brigitte Buchmann, and Gerrit Kuhlmann
Atmos. Meas. Tech., 13, 4277–4293, https://doi.org/10.5194/amt-13-4277-2020, https://doi.org/10.5194/amt-13-4277-2020, 2020
Short summary
Short summary
Horizontal homogeneity is often assumed for trace gases remote sensing, although it is not valid where trace gas concentrations have high spatial variability, e.g., in cities. We show the importance of 3D effects for MAX-DOAS and airborne imaging spectrometers using 3D-box air mass factors implemented in the MYSTIC radiative transfer solver. In both cases, 3D information is invaluable for interpreting the measurements, as not considering 3D effects can lead to misinterpretation of measurements.
Michael Müller, Peter Graf, Jonas Meyer, Anastasia Pentina, Dominik Brunner, Fernando Perez-Cruz, Christoph Hüglin, and Lukas Emmenegger
Atmos. Meas. Tech., 13, 3815–3834, https://doi.org/10.5194/amt-13-3815-2020, https://doi.org/10.5194/amt-13-3815-2020, 2020
Peter G. Simmonds, Matthew Rigby, Alistair J. Manning, Sunyoung Park, Kieran M. Stanley, Archie McCulloch, Stephan Henne, Francesco Graziosi, Michela Maione, Jgor Arduini, Stefan Reimann, Martin K. Vollmer, Jens Mühle, Simon O'Doherty, Dickon Young, Paul B. Krummel, Paul J. Fraser, Ray F. Weiss, Peter K. Salameh, Christina M. Harth, Mi-Kyung Park, Hyeri Park, Tim Arnold, Chris Rennick, L. Paul Steele, Blagoj Mitrevski, Ray H. J. Wang, and Ronald G. Prinn
Atmos. Chem. Phys., 20, 7271–7290, https://doi.org/10.5194/acp-20-7271-2020, https://doi.org/10.5194/acp-20-7271-2020, 2020
Short summary
Short summary
Sulfur hexafluoride (SF6) is a potent greenhouse gas which is regulated under the Kyoto Protocol. From a 40-year record of measurements, collected at five global monitoring sites and archived air samples, we show that its concentration in the atmosphere has steadily increased. Using modelling techniques, we estimate that global emissions have increased by about 24 % over the past decade. We find that this increase is driven by the demand for SF6-insulated switchgear in developing countries.
Longfei Yu, Eliza Harris, Stephan Henne, Sarah Eggleston, Martin Steinbacher, Lukas Emmenegger, Christoph Zellweger, and Joachim Mohn
Atmos. Chem. Phys., 20, 6495–6519, https://doi.org/10.5194/acp-20-6495-2020, https://doi.org/10.5194/acp-20-6495-2020, 2020
Short summary
Short summary
We observed the isotopic composition of nitrous oxide in the unpolluted air at Jungfraujoch for 5 years. Our results indicate a clear seasonal pattern in the isotopic composition, corresponding with that in atmospheric nitrous oxide levels. This is most likely due to temporal variations in both emission processes and air mass sources for Jungfraujoch. Our findings are of importance to global nitrous oxide modelling and to better understanding of long-term trends in atmospheric nitrous oxide.
Michael Jähn, Gerrit Kuhlmann, Qing Mu, Jean-Matthieu Haussaire, David Ochsner, Katherine Osterried, Valentin Clément, and Dominik Brunner
Geosci. Model Dev., 13, 2379–2392, https://doi.org/10.5194/gmd-13-2379-2020, https://doi.org/10.5194/gmd-13-2379-2020, 2020
Short summary
Short summary
Emission inventories of air pollutants and greenhouse gases are widely used as input for atmospheric chemistry transport models. However, the pre-processing of these data is both time-consuming and requires a large amount of disk storage. To overcome this issue, a Python package has been developed and tested for two different models. There, the inventory is projected to the model grid and scaling factors are provided. This approach saves computational time while remaining numerically equivalent.
Gianluca Mussetti, Dominik Brunner, Stephan Henne, Jonas Allegrini, E. Scott Krayenhoff, Sebastian Schubert, Christian Feigenwinter, Roland Vogt, Andreas Wicki, and Jan Carmeliet
Geosci. Model Dev., 13, 1685–1710, https://doi.org/10.5194/gmd-13-1685-2020, https://doi.org/10.5194/gmd-13-1685-2020, 2020
Short summary
Short summary
Street trees are regarded as a powerful measure to reduce excessive heat in cities. To enable city-wide studies of the cooling effect of street trees, we developed a coupled urban climate model with explicit representation of street trees (COSMO-BEP-Tree). The model compares well with surface, flux and satellite observations and responds realistically to changes in tree characteristics. Street trees largely impact energy fluxes and wind speed, while air temperatures are only slightly reduced.
Ece Satar, Peter Nyfeler, Céline Pascale, Bernhard Niederhauser, and Markus Leuenberger
Atmos. Meas. Tech., 13, 119–130, https://doi.org/10.5194/amt-13-119-2020, https://doi.org/10.5194/amt-13-119-2020, 2020
Short summary
Short summary
To ensure the best preparation and measurement conditions for trace gases, usage of coated materials is in demand in gas metrology and atmospheric measurement communities. In this article, the previously introduced aluminum measurement chamber is used to investigate materials such as glass, aluminum, copper, brass, steel and three different commercially available coatings. Our measurements focus on temperature and pressure dependencies for the species CO2, CO, CH4 and H2O using a CRDS analyzer.
Ece Satar, Peter Nyfeler, Bernhard Bereiter, Céline Pascale, Bernhard Niederhauser, and Markus Leuenberger
Atmos. Meas. Tech., 13, 101–117, https://doi.org/10.5194/amt-13-101-2020, https://doi.org/10.5194/amt-13-101-2020, 2020
Short summary
Short summary
Good-quality measurements of atmospheric trace gases are only possible with regular calibrations and stable measurements from the standard cylinders. This study investigates instabilities due to surface effects on newly built aluminum and steel cylinders. We present measurements over a set of temperature and pressure ranges for the amount fractions of CO2, CO, CH4 and H2O using a commercial and a novel laser spectroscopic analyzer.
Tesfaye A. Berhanu, John Hoffnagle, Chris Rella, David Kimhak, Peter Nyfeler, and Markus Leuenberger
Atmos. Meas. Tech., 12, 6803–6826, https://doi.org/10.5194/amt-12-6803-2019, https://doi.org/10.5194/amt-12-6803-2019, 2019
Short summary
Short summary
Accurate measurement of variations in atmospheric O2 can provide useful information about atmospheric, biospheric, and oceanic processes, which is a challenge for existing measurement techniques. Here, we introduce a newly built high-precision, stable CRDS analyzer (Picarro G2207) that can measure O2 mixing ratios with a short-term precision of < 1 ppm and only requires calibration every 12 h. Measurements from tower and mountain sites are also presented.
Gerrit Kuhlmann, Grégoire Broquet, Julia Marshall, Valentin Clément, Armin Löscher, Yasjka Meijer, and Dominik Brunner
Atmos. Meas. Tech., 12, 6695–6719, https://doi.org/10.5194/amt-12-6695-2019, https://doi.org/10.5194/amt-12-6695-2019, 2019
Short summary
Short summary
The Copernicus Anthropogenic CO2 Monitoring (CO2M) mission is a proposed constellation of imaging satellites with a CO2 instrument as main payload and optionally instruments for NO2, CO and aerosols. This study demonstrates the huge benefit of an NO2 instrument for detecting city plumes and weak point sources. Its main advantages are the higher signal-to-noise ratio and the lower sensitivity to clouds that significantly increases the number of observations available for quantifying CO2 emission.
Ignacio Pisso, Espen Sollum, Henrik Grythe, Nina I. Kristiansen, Massimo Cassiani, Sabine Eckhardt, Delia Arnold, Don Morton, Rona L. Thompson, Christine D. Groot Zwaaftink, Nikolaos Evangeliou, Harald Sodemann, Leopold Haimberger, Stephan Henne, Dominik Brunner, John F. Burkhart, Anne Fouilloux, Jerome Brioude, Anne Philipp, Petra Seibert, and Andreas Stohl
Geosci. Model Dev., 12, 4955–4997, https://doi.org/10.5194/gmd-12-4955-2019, https://doi.org/10.5194/gmd-12-4955-2019, 2019
Short summary
Short summary
We present the latest release of the Lagrangian transport model FLEXPART, which simulates the transport, diffusion, dry and wet deposition, radioactive decay, and 1st-order chemical reactions of atmospheric tracers. The model has been recently updated both technically and in the representation of physicochemical processes. We describe the changes, document the most recent input and output files, provide working examples, and introduce testing capabilities.
Michael Döring and Markus Christian Leuenberger
Clim. Past Discuss., https://doi.org/10.5194/cp-2019-132, https://doi.org/10.5194/cp-2019-132, 2019
Manuscript not accepted for further review
Short summary
Short summary
We analyse Holocen temperatures reconstructed from gas-stable-isotope species measured on ancient air extracted from a Greenland ice core. Also, we compare two state of the art firn-models which are needed for the inversion of the gas-isotope data to paleo-temperature and provide detailed uncertainty estimations for the reconstructed temperature estimates. Finally, we compare our reconstructed temperatures to two recent reconstructions based on the same gas-isotope data as used here.
Erkan Ibraim, Benjamin Wolf, Eliza Harris, Rainer Gasche, Jing Wei, Longfei Yu, Ralf Kiese, Sarah Eggleston, Klaus Butterbach-Bahl, Matthias Zeeman, Béla Tuzson, Lukas Emmenegger, Johan Six, Stephan Henne, and Joachim Mohn
Biogeosciences, 16, 3247–3266, https://doi.org/10.5194/bg-16-3247-2019, https://doi.org/10.5194/bg-16-3247-2019, 2019
Short summary
Short summary
Nitrous oxide (N2O) is an important greenhouse gas and the major stratospheric ozone-depleting substance; therefore, mitigation of anthropogenic N2O emissions is needed. To trace N2O-emitting source processes, in this study, we observed N2O isotopocules above an intensively managed grassland research site with a recently developed laser spectroscopy method. Our results indicate that the domain of denitrification or nitrifier denitrification was the major N2O source.
Dominik Brunner, Gerrit Kuhlmann, Julia Marshall, Valentin Clément, Oliver Fuhrer, Grégoire Broquet, Armin Löscher, and Yasjka Meijer
Atmos. Chem. Phys., 19, 4541–4559, https://doi.org/10.5194/acp-19-4541-2019, https://doi.org/10.5194/acp-19-4541-2019, 2019
Short summary
Short summary
Atmospheric transport models are increasingly being used to estimate CO2 emissions from atmospheric CO2 measurements. This study demonstrates the importance of distributing CO2 emissions vertically in the model according to realistic profiles, since a major proportion of CO2 is emitted through tall stacks from power plants and industrial sources. With the traditional approach of emitting all CO2 at the surface, models may significantly overestimate the atmospheric CO2 levels.
Christine D. Groot Zwaaftink, Stephan Henne, Rona L. Thompson, Edward J. Dlugokencky, Toshinobu Machida, Jean-Daniel Paris, Motoki Sasakawa, Arjo Segers, Colm Sweeney, and Andreas Stohl
Geosci. Model Dev., 11, 4469–4487, https://doi.org/10.5194/gmd-11-4469-2018, https://doi.org/10.5194/gmd-11-4469-2018, 2018
Short summary
Short summary
A Lagrangian particle dispersion model is used to simulate global fields of methane, constrained by observations through nudging. We show that this rather simple and computationally inexpensive method can give results similar to or as good as a computationally expensive Eulerian chemistry transport model with a data assimilation scheme. The three-dimensional methane fields are of interest to applications such as inverse modelling and satellite retrievals.
Rocío Baró, Pedro Jiménez-Guerrero, Martin Stengel, Dominik Brunner, Gabriele Curci, Renate Forkel, Lucy Neal, Laura Palacios-Peña, Nicholas Savage, Martijn Schaap, Paolo Tuccella, Hugo Denier van der Gon, and Stefano Galmarini
Atmos. Chem. Phys., 18, 15183–15199, https://doi.org/10.5194/acp-18-15183-2018, https://doi.org/10.5194/acp-18-15183-2018, 2018
Short summary
Short summary
Particles in the atmosphere, such as pollution, desert dust, and volcanic ash, have an impact on meteorology. They interact with incoming radiation resulting in a cooling effect of the atmosphere. Today, the use of meteorology and chemistry models help us to understand these processes, but there are a lot of uncertainties. The goal of this work is to evaluate how these interactions are represented in the models by comparing them to satellite data to see how close they are to reality.
Michael Döring and Markus C. Leuenberger
Clim. Past, 14, 763–788, https://doi.org/10.5194/cp-14-763-2018, https://doi.org/10.5194/cp-14-763-2018, 2018
Short summary
Short summary
We present a novel approach for ice-core-based temperature reconstructions, which is based on gas-isotope data measured on enclosed air bubbles in ice cores. The processes of air movement and enclosure are highly temperature dependent due to heat diffusion in and densification of the snow and ice. Our method inverts a model, which describes these processes, to desired temperature histories. This paper examines the performance of our novel approach on different synthetic isotope-data scenarios.
Laura Palacios-Peña, Rocío Baró, Alexander Baklanov, Alessandra Balzarini, Dominik Brunner, Renate Forkel, Marcus Hirtl, Luka Honzak, José María López-Romero, Juan Pedro Montávez, Juan Luis Pérez, Guido Pirovano, Roberto San José, Wolfram Schröder, Johannes Werhahn, Ralf Wolke, Rahela Žabkar, and Pedro Jiménez-Guerrero
Atmos. Chem. Phys., 18, 5021–5043, https://doi.org/10.5194/acp-18-5021-2018, https://doi.org/10.5194/acp-18-5021-2018, 2018
Short summary
Short summary
Atmospheric aerosols modify the radiative budget of the Earth, and it is therefore mandatory to have an accurate representation of their optical properties for understanding their climatic role. This work therefore evaluates the skill in the representation of optical properties by different remote-sensing sensors and regional online coupled chemistry–climate models over Europe.
Peter G. Simmonds, Matthew Rigby, Archie McCulloch, Martin K. Vollmer, Stephan Henne, Jens Mühle, Simon O'Doherty, Alistair J. Manning, Paul B. Krummel, Paul J. Fraser, Dickon Young, Ray F. Weiss, Peter K. Salameh, Christina M. Harth, Stefan Reimann, Cathy M. Trudinger, L. Paul Steele, Ray H. J. Wang, Diane J. Ivy, Ronald G. Prinn, Blagoj Mitrevski, and David M. Etheridge
Atmos. Chem. Phys., 18, 4153–4169, https://doi.org/10.5194/acp-18-4153-2018, https://doi.org/10.5194/acp-18-4153-2018, 2018
Short summary
Short summary
Recent measurements of the potent greenhouse gas HFC-23, a by-product of HCFC-22 production, show a 28 % increase in the atmospheric mole fraction from 2009 to 2016. A minimum in the atmospheric abundance of HFC-23 in 2009 was attributed to abatement of HFC-23 emissions by incineration under the Clean Development Mechanism (CDM). Our results indicate that the recent increase in HFC-23 emissions is driven by failure of mitigation under the CDM to keep pace with increased HCFC-22 production.
Fabian Schoenenberger, Stephan Henne, Matthias Hill, Martin K. Vollmer, Giorgos Kouvarakis, Nikolaos Mihalopoulos, Simon O'Doherty, Michela Maione, Lukas Emmenegger, Thomas Peter, and Stefan Reimann
Atmos. Chem. Phys., 18, 4069–4092, https://doi.org/10.5194/acp-18-4069-2018, https://doi.org/10.5194/acp-18-4069-2018, 2018
Short summary
Short summary
Anthropogenic halocarbon emissions contribute to stratospheric ozone depletion and global warming. We measured atmospheric halocarbons for 6 months on Crete to extend the coverage of the existing observation network to the Eastern Mediterranean. The derived emission estimates showed a contribution of 16.8 % (13.6–23.3 %) and 53.2 % (38.1–84.2 %) of this region to the total HFC and HCFC emissions of the analyzed European domain and a reduction of the underlying uncertainties by 40–80 %.
Abdelhadi El Yazidi, Michel Ramonet, Philippe Ciais, Gregoire Broquet, Isabelle Pison, Amara Abbaris, Dominik Brunner, Sebastien Conil, Marc Delmotte, Francois Gheusi, Frederic Guerin, Lynn Hazan, Nesrine Kachroudi, Giorgos Kouvarakis, Nikolaos Mihalopoulos, Leonard Rivier, and Dominique Serça
Atmos. Meas. Tech., 11, 1599–1614, https://doi.org/10.5194/amt-11-1599-2018, https://doi.org/10.5194/amt-11-1599-2018, 2018
Ye Yuan, Ludwig Ries, Hannes Petermeier, Martin Steinbacher, Angel J. Gómez-Peláez, Markus C. Leuenberger, Marcus Schumacher, Thomas Trickl, Cedric Couret, Frank Meinhardt, and Annette Menzel
Atmos. Meas. Tech., 11, 1501–1514, https://doi.org/10.5194/amt-11-1501-2018, https://doi.org/10.5194/amt-11-1501-2018, 2018
Short summary
Short summary
This paper presents a novel statistical method, ADVS, for baseline selection of representative CO2 data at elevated mountain measurement stations. It provides insights on how data processing techniques are critical for measurements and data analyses. Compared with other statistical methods, our method appears to be a good option as a generalized approach with improved comparability, which is important for research on measurement site characteristics and comparisons between stations.
Malin M. Ziehmer, Kurt Nicolussi, Christian Schlüchter, and Markus Leuenberger
Biogeosciences, 15, 1047–1064, https://doi.org/10.5194/bg-15-1047-2018, https://doi.org/10.5194/bg-15-1047-2018, 2018
Short summary
Short summary
Cellulose content (CC (%)) series from two high-Alpine species, Larix decidua Mill. (European larch, LADE) and Pinus cembra L. (Swiss stone pine, PICE) are investigated in modern wood samples and Holocene wood remains from the Early and mid-Holocene. Trends in modern and Holocene time series as well as climate–cellulose relationships for modern trees in the Alps show high potential for CC (%) to be established as novel supplementary proxy in dendroclimatology.
Martin K. Vollmer, Dickon Young, Cathy M. Trudinger, Jens Mühle, Stephan Henne, Matthew Rigby, Sunyoung Park, Shanlan Li, Myriam Guillevic, Blagoj Mitrevski, Christina M. Harth, Benjamin R. Miller, Stefan Reimann, Bo Yao, L. Paul Steele, Simon A. Wyss, Chris R. Lunder, Jgor Arduini, Archie McCulloch, Songhao Wu, Tae Siek Rhee, Ray H. J. Wang, Peter K. Salameh, Ove Hermansen, Matthias Hill, Ray L. Langenfelds, Diane Ivy, Simon O'Doherty, Paul B. Krummel, Michela Maione, David M. Etheridge, Lingxi Zhou, Paul J. Fraser, Ronald G. Prinn, Ray F. Weiss, and Peter G. Simmonds
Atmos. Chem. Phys., 18, 979–1002, https://doi.org/10.5194/acp-18-979-2018, https://doi.org/10.5194/acp-18-979-2018, 2018
Short summary
Short summary
We measured the three chlorofluorocarbons (CFCs) CFC-13, CFC-114, and CFC-115 in the atmosphere because they are important in stratospheric ozone depletion. These compounds should have decreased in the atmosphere because they are banned by the Montreal Protocol but we find the opposite. Emissions over the last decade have not declined on a global scale. We use inverse modeling and our observations to find that a large part of the emissions originate in the Asian region.
Yu Liu, Nicolas Gruber, and Dominik Brunner
Atmos. Chem. Phys., 17, 14145–14169, https://doi.org/10.5194/acp-17-14145-2017, https://doi.org/10.5194/acp-17-14145-2017, 2017
Short summary
Short summary
We analyze fossil fuel signals in atmospheric CO2 over Europe using a high-resolution atmospheric transport model and diurnal emission data. We find that fossil fuel CO2 accounts for more than half of the atmospheric CO2 variations, mainly at diurnal timescales. The covariance of diurnal emission and transport also leads to a substantial rectification effect. Thus, the consideration of diurnal emissions and high-resolution transport is paramount for accurately modeling the fossil fuel signal.
Antoine Berchet, Katrin Zink, Dietmar Oettl, Jürg Brunner, Lukas Emmenegger, and Dominik Brunner
Geosci. Model Dev., 10, 3441–3459, https://doi.org/10.5194/gmd-10-3441-2017, https://doi.org/10.5194/gmd-10-3441-2017, 2017
Short summary
Short summary
We evaluate a new cost-effective method to simulate pollutant dispersion at high resolution on a city-wide domain. The method is based on a catalogue of reference simulations matched to weather observations to produce a sequence of hourly pollution maps. A total of 2 years of simulations are compared with continuous measurements and passive NO2 samplers in the city of Zurich. Spatial and temporal variability proved to be very well reproduced by the method.
Tesfaye A. Berhanu, Sönke Szidat, Dominik Brunner, Ece Satar, Rüdiger Schanda, Peter Nyfeler, Michael Battaglia, Martin Steinbacher, Samuel Hammer, and Markus Leuenberger
Atmos. Chem. Phys., 17, 10753–10766, https://doi.org/10.5194/acp-17-10753-2017, https://doi.org/10.5194/acp-17-10753-2017, 2017
Short summary
Short summary
Fossil fuel CO2 is the major contributor of anthropogenic CO2 in the atmosphere, and accurate quantification is essential to better understand the carbon cycle. Such accurate quantification can be conducted based on radiocarbon measurements. In this study, we present radiocarbon measurements from a tall tower site in Switzerland. From these measurements, we have observed seasonally varying fossil fuel CO2 contributions and a biospheric CO2 component that varies diurnally and seasonally.
Dominik Brunner, Tim Arnold, Stephan Henne, Alistair Manning, Rona L. Thompson, Michela Maione, Simon O'Doherty, and Stefan Reimann
Atmos. Chem. Phys., 17, 10651–10674, https://doi.org/10.5194/acp-17-10651-2017, https://doi.org/10.5194/acp-17-10651-2017, 2017
Short summary
Short summary
Hydrofluorocarbons (HFCs) and SF6 are industrially produced gases with a large greenhouse-gas warming potential. In this study, we estimated the emissions of HFCs and SF6 over Europe by combining measurements at three background stations with four different model systems. We identified significant differences between our estimates and nationally reported numbers, but also found that the network of only three sites in Europe is insufficient to reliably attribute emissions to individual countries.
Eleni Athanasopoulou, Orestis Speyer, Dominik Brunner, Heike Vogel, Bernhard Vogel, Nikolaos Mihalopoulos, and Evangelos Gerasopoulos
Atmos. Chem. Phys., 17, 10597–10618, https://doi.org/10.5194/acp-17-10597-2017, https://doi.org/10.5194/acp-17-10597-2017, 2017
Short summary
Short summary
This work focuses on the impact of residential wood burning on aerosol levels, composition and radiation under the ongoing economic crisis in Greece. The atmospheric model COSMO-ART performed a series of runs during the winter of 2013–2014. Emission inputs were revised according to the detailed aerosol characterization by local measurements. Aerosol levels were found to be elevated and mostly composed of organics, yet the timing of the plume justifies the minor radiative cooling and feedbacks.
Yann Poltera, Giovanni Martucci, Martine Collaud Coen, Maxime Hervo, Lukas Emmenegger, Stephan Henne, Dominik Brunner, and Alexander Haefele
Atmos. Chem. Phys., 17, 10051–10070, https://doi.org/10.5194/acp-17-10051-2017, https://doi.org/10.5194/acp-17-10051-2017, 2017
Short summary
Short summary
We present the PathfinderTURB algorithm for the analysis of ceilometer backscatter data and the real-time detection of the vertical structure of the planetary boundary layer. PathfinderTURB has been applied to 1 year of data measured by two ceilometers operated at two Swiss stations: the Aerological Observatory of Payerne on the Swiss plateau, and the Alpine Jungfraujoch observatory. The study shows that aerosols from the boundary layer significantly influence the air measured at Jungfraujoch.
Rocío Baró, Laura Palacios-Peña, Alexander Baklanov, Alessandra Balzarini, Dominik Brunner, Renate Forkel, Marcus Hirtl, Luka Honzak, Juan Luis Pérez, Guido Pirovano, Roberto San José, Wolfram Schröder, Johannes Werhahn, Ralf Wolke, Rahela Žabkar, and Pedro Jiménez-Guerrero
Atmos. Chem. Phys., 17, 9677–9696, https://doi.org/10.5194/acp-17-9677-2017, https://doi.org/10.5194/acp-17-9677-2017, 2017
Short summary
Short summary
The influence on modeled max., mean and min. temperature over Europe of including aerosol–radiation–cloud interactions has been assessed for two case studies in 2010. Data were taken from an ensemble of online regional chemistry–climate models from EuMetChem COST Action. The results indicate that including these interactions clearly improves the spatiotemporal variability in the temperature signal simulated by the models, with implications for reducing the uncertainty in climate projections.
Kathrin M. Keller, Sebastian Lienert, Anil Bozbiyik, Thomas F. Stocker, Olga V. Churakova (Sidorova), David C. Frank, Stefan Klesse, Charles D. Koven, Markus Leuenberger, William J. Riley, Matthias Saurer, Rolf Siegwolf, Rosemarie B. Weigt, and Fortunat Joos
Biogeosciences, 14, 2641–2673, https://doi.org/10.5194/bg-14-2641-2017, https://doi.org/10.5194/bg-14-2641-2017, 2017
Carla Frege, Federico Bianchi, Ugo Molteni, Jasmin Tröstl, Heikki Junninen, Stephan Henne, Mikko Sipilä, Erik Herrmann, Michel J. Rossi, Markku Kulmala, Christopher R. Hoyle, Urs Baltensperger, and Josef Dommen
Atmos. Chem. Phys., 17, 2613–2629, https://doi.org/10.5194/acp-17-2613-2017, https://doi.org/10.5194/acp-17-2613-2017, 2017
Short summary
Short summary
We present measurements of the chemical composition of atmospheric ions at high altitude (3450 m a.s.l.) during a 9-month campaign. We detected remarkably high correlation between methanesulfonic acid (MSA) and SO5−. Halogenated species were also detected frequently at this continental location. New-particle formation events occurred via the condensation of highly oxygenated molecules (HOMs) at very low sulfuric acid concentration or, less frequently, due to ammonia–sulfuric acid clusters.
Laura Palacios-Peña, Rocío Baró, Juan Luis Guerrero-Rascado, Lucas Alados-Arboledas, Dominik Brunner, and Pedro Jiménez-Guerrero
Atmos. Chem. Phys., 17, 277–296, https://doi.org/10.5194/acp-17-277-2017, https://doi.org/10.5194/acp-17-277-2017, 2017
Short summary
Short summary
The effects of atmospheric aerosols over the Earth’s climate mainly depend on their optical, microphysical and chemical properties, which modify the Earth's radiative budget, the main source of uncertainty in climate change. In this work we have studied the representation of aerosol optical properties using an online coupled model (WRF-Chem) when aerosol–radiation interactions (ARIs) and aerosol–clouds interactions (ACIs) are taken into account over the Iberian Peninsula.
Ioannis Kioutsioukis, Ulas Im, Efisio Solazzo, Roberto Bianconi, Alba Badia, Alessandra Balzarini, Rocío Baró, Roberto Bellasio, Dominik Brunner, Charles Chemel, Gabriele Curci, Hugo Denier van der Gon, Johannes Flemming, Renate Forkel, Lea Giordano, Pedro Jiménez-Guerrero, Marcus Hirtl, Oriol Jorba, Astrid Manders-Groot, Lucy Neal, Juan L. Pérez, Guidio Pirovano, Roberto San Jose, Nicholas Savage, Wolfram Schroder, Ranjeet S. Sokhi, Dimiter Syrakov, Paolo Tuccella, Johannes Werhahn, Ralf Wolke, Christian Hogrefe, and Stefano Galmarini
Atmos. Chem. Phys., 16, 15629–15652, https://doi.org/10.5194/acp-16-15629-2016, https://doi.org/10.5194/acp-16-15629-2016, 2016
Short summary
Short summary
Four ensemble methods are applied to two annual AQMEII datasets and their performance is compared for O3, NO2 and PM10. The goal of the study is to quantify to what extent we can extract predictable signals from an ensemble with superior skill at each station over the single models and the ensemble mean. The promotion of the right amount of accuracy and diversity within the ensemble results in an average additional skill of up to 31 % compared to using the full ensemble in an unconditional way.
Thomas Röckmann, Simon Eyer, Carina van der Veen, Maria E. Popa, Béla Tuzson, Guillaume Monteil, Sander Houweling, Eliza Harris, Dominik Brunner, Hubertus Fischer, Giulia Zazzeri, David Lowry, Euan G. Nisbet, Willi A. Brand, Jaroslav M. Necki, Lukas Emmenegger, and Joachim Mohn
Atmos. Chem. Phys., 16, 10469–10487, https://doi.org/10.5194/acp-16-10469-2016, https://doi.org/10.5194/acp-16-10469-2016, 2016
Short summary
Short summary
A dual isotope ratio mass spectrometric system (IRMS) and a quantum cascade laser absorption spectroscopy (QCLAS)-based technique were deployed at the Cabauw experimental site for atmospheric research (CESAR) in the Netherlands and performed in situ, high-frequency (approx. hourly) measurements for a period of more than 5 months, yielding a combined dataset with more than 2500 measurements of both δ13C and δD.
Michael F. Schibig, Emmanuel Mahieu, Stephan Henne, Bernard Lejeune, and Markus C. Leuenberger
Atmos. Chem. Phys., 16, 9935–9949, https://doi.org/10.5194/acp-16-9935-2016, https://doi.org/10.5194/acp-16-9935-2016, 2016
Short summary
Short summary
Two CO2 time series measured at the High Alpine Research Station Jungfraujoch, Switzerland (3580 m a.s.l.), in the period from 2005 to 2013 were compared. One data set was measured in situ whereas the other data set was measured in the column above Jungfraujoch. The trends of the column integrated and the in situ data set are in good agreement, the amplitude of the in situ data set is ca. two times the amplitude of the column integrated data set, because it is closer to the sources and sinks.
Emiliano Stopelli, Franz Conen, Cindy E. Morris, Erik Herrmann, Stephan Henne, Martin Steinbacher, and Christine Alewell
Atmos. Chem. Phys., 16, 8341–8351, https://doi.org/10.5194/acp-16-8341-2016, https://doi.org/10.5194/acp-16-8341-2016, 2016
Short summary
Short summary
Knowing the variability of ice nucleating particles (INPs) helps determining their role in the formation of precipitation. Here we describe and predict the concentrations of INPs active at −8 °C in precipitation samples collected at Jungfraujoch (CH, 3580 m a.s.l.). A high abundance of these INPs can be expected whenever a coincidence of high wind speed and first precipitation from an air mass occurs. This expands the set of conditions where such INPs could affect the onset of precipitation.
Tesfaye Ayalneh Berhanu, Ece Satar, Rudiger Schanda, Peter Nyfeler, Hanspeter Moret, Dominik Brunner, Brian Oney, and Markus Leuenberger
Atmos. Meas. Tech., 9, 2603–2614, https://doi.org/10.5194/amt-9-2603-2016, https://doi.org/10.5194/amt-9-2603-2016, 2016
Short summary
Short summary
In this manuscript, we have presented Co, CO2 and CH4 measurement data from an old radio tower tower (217.5 m) at Beromunster, Switzerland. From about 2 years of continuous CO, CO2 and CH4 measurement at five different heights, we have determined a long-term reproducibility of 2.79 ppb, 0.05 ppm and 0.29 ppb for CO, CO2 and CH4, respectively, compliant with the GAW requirements. We have also observed seasonal and diurnal variation of these species.
Florian Berkes, Peter Hoor, Heiko Bozem, Daniel Kunkel, Michael Sprenger, and Stephan Henne
Atmos. Chem. Phys., 16, 6011–6025, https://doi.org/10.5194/acp-16-6011-2016, https://doi.org/10.5194/acp-16-6011-2016, 2016
Short summary
Short summary
We presented airborne measurements of CO2 and O3 across the entrainment zone over a semi-remote environment in southwestern Germany in late summer 2011 .
For the first time CO2 and O3 were used as tracer to identify mixing through this transport barrier. We demonstrated that the tracer--tracer correlation of CO2 and O3 is a powerful tool to identify entrainment and mixing.
Lucie Bazin, Amaelle Landais, Emilie Capron, Valérie Masson-Delmotte, Catherine Ritz, Ghislain Picard, Jean Jouzel, Marie Dumont, Markus Leuenberger, and Frédéric Prié
Clim. Past, 12, 729–748, https://doi.org/10.5194/cp-12-729-2016, https://doi.org/10.5194/cp-12-729-2016, 2016
Short summary
Short summary
We present new measurements of δO2⁄N2 and δ18Oatm performed on well-conserved ice from EDC covering MIS5 and between 380 and 800 ka. The combination of the observation of a 100 ka periodicity in the new δO2⁄N2 record with a MIS5 multi-site multi-proxy study has revealed a potential influence of local climatic parameters on δO2⁄N2. Moreover, we propose that the varying delay between d18Oatm and precession for the last 800 ka is affected by the occurrence of ice sheet discharge events.
Stephan Henne, Dominik Brunner, Brian Oney, Markus Leuenberger, Werner Eugster, Ines Bamberger, Frank Meinhardt, Martin Steinbacher, and Lukas Emmenegger
Atmos. Chem. Phys., 16, 3683–3710, https://doi.org/10.5194/acp-16-3683-2016, https://doi.org/10.5194/acp-16-3683-2016, 2016
Short summary
Short summary
Greenhouse gas emissions can be assessed by "top-down" methods that combine atmospheric observations, a transport model and a mathematical optimisation framework. Here, we apply such a top-down method to the methane emissions of Switzerland, utilising observations from the recently installed CarboCount-CH network. Our Swiss total emissions largely agree with those of the national "bottom-up" inventory, whereas regional differences suggest lower than reported emissions from manure handling.
P. G. Simmonds, M. Rigby, A. J. Manning, M. F. Lunt, S. O'Doherty, A. McCulloch, P. J. Fraser, S. Henne, M. K. Vollmer, J. Mühle, R. F. Weiss, P. K. Salameh, D. Young, S. Reimann, A. Wenger, T. Arnold, C. M. Harth, P. B. Krummel, L. P. Steele, B. L. Dunse, B. R. Miller, C. R. Lunder, O. Hermansen, N. Schmidbauer, T. Saito, Y. Yokouchi, S. Park, S. Li, B. Yao, L. X. Zhou, J. Arduini, M. Maione, R. H. J. Wang, D. Ivy, and R. G. Prinn
Atmos. Chem. Phys., 16, 365–382, https://doi.org/10.5194/acp-16-365-2016, https://doi.org/10.5194/acp-16-365-2016, 2016
Short summary
Short summary
We report regional and global emissions estimates of HFC-152a using high frequency measurements from 11 observing sites and archived air samples dating back to 1978 together with atmospheric transport models. The "bottom-up" emissions of HFC-152a reported to the UNFCCC appear to significantly underestimate those reported here from observations. This discrepancy we suggest arises from largely underestimated USA and undeclared Asian emissions.
M. C. Leuenberger, M. F. Schibig, and P. Nyfeler
Atmos. Meas. Tech., 8, 5289–5299, https://doi.org/10.5194/amt-8-5289-2015, https://doi.org/10.5194/amt-8-5289-2015, 2015
Short summary
Short summary
Adsorption/desorption effects of trace gases in gas cylinders were investigated. Our measurements indicate a rather strong effect on steel cylinders for CO2 that becomes easily visible through enhanced concentrations for low (<20 bars) gas pressure. Much smaller effects are observed for CO and CH4. Significantly smaller effects are measured for all gas species investigated on aluminium cylinders. Careful selection of gas cylinders for high-precision calibration purposes is recommended.
T. Kobashi, T. Ikeda-Fukazawa, M. Suwa, J. Schwander, T. Kameda, J. Lundin, A. Hori, H. Motoyama, M. Döring, and M. Leuenberger
Atmos. Chem. Phys., 15, 13895–13914, https://doi.org/10.5194/acp-15-13895-2015, https://doi.org/10.5194/acp-15-13895-2015, 2015
Short summary
Short summary
We find that argon/nitrogen ratios of trapped air in the GISP2 ice core on “gas ages” are significantly negatively correlated with accumulation rate changes over the past 6000 years. Lines of evidence indicate that changes in overloading pressure at bubble closeoff depths induced the gas fractionation in closed bubbles. Further understanding of the fractionation processes may lead to a new proxy for the past temperature and accumulation rate.
R. Fröhlich, M. J. Cubison, J. G. Slowik, N. Bukowiecki, F. Canonaco, P. L. Croteau, M. Gysel, S. Henne, E. Herrmann, J. T. Jayne, M. Steinbacher, D. R. Worsnop, U. Baltensperger, and A. S. H. Prévôt
Atmos. Chem. Phys., 15, 11373–11398, https://doi.org/10.5194/acp-15-11373-2015, https://doi.org/10.5194/acp-15-11373-2015, 2015
Short summary
Short summary
This manuscript presents the first long-term (14-month) and highly time-resolved (10 min) measurements of NR-PM1 aerosol chemical composition at a high-altitude site (JFJ, Switzerland, 3580m a.s.l.). The elevated location allowed the investigation of free tropospheric aerosol year round. Total and relative mass loadings, diurnal variations as well as seasonal variations are discussed together with geographical origin, organic aerosol sources and the influence of the planetary boundary layer.
T. A. Berhanu, J. Savarino, J. Erbland, W. C. Vicars, S. Preunkert, J. F. Martins, and M. S. Johnson
Atmos. Chem. Phys., 15, 11243–11256, https://doi.org/10.5194/acp-15-11243-2015, https://doi.org/10.5194/acp-15-11243-2015, 2015
Short summary
Short summary
In this field study at Dome C, Antarctica, we investigated the effect of solar UV photolysis on the stable isotopes of nitrate in snow via comparison of two identical snow pits while exposing only one to solar UV. From the difference between the average isotopic fractionations calculated for each pit, we determined a purely photolytic nitrogen isotopic fractionation of -55.8‰, in good agreement with what has been recently determined in a laboratory study.
B. Oney, S. Henne, N. Gruber, M. Leuenberger, I. Bamberger, W. Eugster, and D. Brunner
Atmos. Chem. Phys., 15, 11147–11164, https://doi.org/10.5194/acp-15-11147-2015, https://doi.org/10.5194/acp-15-11147-2015, 2015
Short summary
Short summary
We present a detailed analysis of a new greenhouse gas measurement network
in the Swiss Plateau, situated between the Jura mountains and the Alps. We
find the network's measurements to be information rich and suitable
for studying surface carbon fluxes of the study region. However, we are
limited by the high-resolution (2km) atmospheric transport model's ability
to simulate meteorology at the individual measurement stations, especially
at those situated in rough terrain.
M. S. Studer, R. T. W. Siegwolf, M. Leuenberger, and S. Abiven
Biogeosciences, 12, 1865–1879, https://doi.org/10.5194/bg-12-1865-2015, https://doi.org/10.5194/bg-12-1865-2015, 2015
Short summary
Short summary
We present a new technique to label organic matter (OM) at its place of formation by the application of 13C, 18O and 2H through the gaseous phase. The label diffused into leaves was incorporated into assimilates and was detected in plant tissues. This technique can be applied in soil sciences, e.g. to trace the decomposition pathways of soil OM inputs, or in plant physiology and palaeoclimatic reconstruction, e.g. to further investigate the origin of the 18O and 2H signal in tree ring cellulose.
M. F. Schibig, M. Steinbacher, B. Buchmann, I. T. van der Laan-Luijkx, S. van der Laan, S. Ranjan, and M. C. Leuenberger
Atmos. Meas. Tech., 8, 57–68, https://doi.org/10.5194/amt-8-57-2015, https://doi.org/10.5194/amt-8-57-2015, 2015
S. Pandey Deolal, S. Henne, L. Ries, S. Gilge, U. Weers, M. Steinbacher, J. Staehelin, and T. Peter
Atmos. Chem. Phys., 14, 12553–12571, https://doi.org/10.5194/acp-14-12553-2014, https://doi.org/10.5194/acp-14-12553-2014, 2014
Short summary
Short summary
Mixing ratios of Peroxyacetyl nitrate (PAN) at Jungfraujoch (Switzerland) and Zugspitze (Germany) show a seasonal variation with maxima in spring, typical for remote sites in the lower atmosphere in northern mid-latitudes. The detailed analysis of PAN measurements of May 2008 indicates that PAN at these high mountain sites is dominated by photochemical formation in the relatively cold polluted European planetary boundary layer rather than formation in the free troposphere.
M. C. Leuenberger, M. F. Schibig, and P. Nyfeler
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-14-19293-2014, https://doi.org/10.5194/acpd-14-19293-2014, 2014
Revised manuscript not accepted
S. Affolter, D. Fleitmann, and M. Leuenberger
Clim. Past, 10, 1291–1304, https://doi.org/10.5194/cp-10-1291-2014, https://doi.org/10.5194/cp-10-1291-2014, 2014
I. Mariani, A. Eichler, T. M. Jenk, S. Brönnimann, R. Auchmann, M. C. Leuenberger, and M. Schwikowski
Clim. Past, 10, 1093–1108, https://doi.org/10.5194/cp-10-1093-2014, https://doi.org/10.5194/cp-10-1093-2014, 2014
P. Kindler, M. Guillevic, M. Baumgartner, J. Schwander, A. Landais, and M. Leuenberger
Clim. Past, 10, 887–902, https://doi.org/10.5194/cp-10-887-2014, https://doi.org/10.5194/cp-10-887-2014, 2014
M. Baumgartner, P. Kindler, O. Eicher, G. Floch, A. Schilt, J. Schwander, R. Spahni, E. Capron, J. Chappellaz, M. Leuenberger, H. Fischer, and T. F. Stocker
Clim. Past, 10, 903–920, https://doi.org/10.5194/cp-10-903-2014, https://doi.org/10.5194/cp-10-903-2014, 2014
R. V. Hiller, D. Bretscher, T. DelSontro, T. Diem, W. Eugster, R. Henneberger, S. Hobi, E. Hodson, D. Imer, M. Kreuzer, T. Künzle, L. Merbold, P. A. Niklaus, B. Rihm, A. Schellenberger, M. H. Schroth, C. J. Schubert, H. Siegrist, J. Stieger, N. Buchmann, and D. Brunner
Biogeosciences, 11, 1941–1959, https://doi.org/10.5194/bg-11-1941-2014, https://doi.org/10.5194/bg-11-1941-2014, 2014
Z. Kern, B. Kohán, and M. Leuenberger
Atmos. Chem. Phys., 14, 1897–1907, https://doi.org/10.5194/acp-14-1897-2014, https://doi.org/10.5194/acp-14-1897-2014, 2014
A. Baklanov, K. Schlünzen, P. Suppan, J. Baldasano, D. Brunner, S. Aksoyoglu, G. Carmichael, J. Douros, J. Flemming, R. Forkel, S. Galmarini, M. Gauss, G. Grell, M. Hirtl, S. Joffre, O. Jorba, E. Kaas, M. Kaasik, G. Kallos, X. Kong, U. Korsholm, A. Kurganskiy, J. Kushta, U. Lohmann, A. Mahura, A. Manders-Groot, A. Maurizi, N. Moussiopoulos, S. T. Rao, N. Savage, C. Seigneur, R. S. Sokhi, E. Solazzo, S. Solomos, B. Sørensen, G. Tsegas, E. Vignati, B. Vogel, and Y. Zhang
Atmos. Chem. Phys., 14, 317–398, https://doi.org/10.5194/acp-14-317-2014, https://doi.org/10.5194/acp-14-317-2014, 2014
L. Bazin, A. Landais, B. Lemieux-Dudon, H. Toyé Mahamadou Kele, D. Veres, F. Parrenin, P. Martinerie, C. Ritz, E. Capron, V. Lipenkov, M.-F. Loutre, D. Raynaud, B. Vinther, A. Svensson, S. O. Rasmussen, M. Severi, T. Blunier, M. Leuenberger, H. Fischer, V. Masson-Delmotte, J. Chappellaz, and E. Wolff
Clim. Past, 9, 1715–1731, https://doi.org/10.5194/cp-9-1715-2013, https://doi.org/10.5194/cp-9-1715-2013, 2013
I. T. van der Laan-Luijkx, S. van der Laan, C. Uglietti, M. F. Schibig, R. E. M. Neubert, H. A. J. Meijer, W. A. Brand, A. Jordan, J. M. Richter, M. Rothe, and M. C. Leuenberger
Atmos. Meas. Tech., 6, 1805–1815, https://doi.org/10.5194/amt-6-1805-2013, https://doi.org/10.5194/amt-6-1805-2013, 2013
P. Sturm, B. Tuzson, S. Henne, and L. Emmenegger
Atmos. Meas. Tech., 6, 1659–1671, https://doi.org/10.5194/amt-6-1659-2013, https://doi.org/10.5194/amt-6-1659-2013, 2013
M. Guillevic, L. Bazin, A. Landais, P. Kindler, A. Orsi, V. Masson-Delmotte, T. Blunier, S. L. Buchardt, E. Capron, M. Leuenberger, P. Martinerie, F. Prié, and B. M. Vinther
Clim. Past, 9, 1029–1051, https://doi.org/10.5194/cp-9-1029-2013, https://doi.org/10.5194/cp-9-1029-2013, 2013
E. Capron, A. Landais, D. Buiron, A. Cauquoin, J. Chappellaz, M. Debret, J. Jouzel, M. Leuenberger, P. Martinerie, V. Masson-Delmotte, R. Mulvaney, F. Parrenin, and F. Prié
Clim. Past, 9, 983–999, https://doi.org/10.5194/cp-9-983-2013, https://doi.org/10.5194/cp-9-983-2013, 2013
C. Knote and D. Brunner
Atmos. Chem. Phys., 13, 1177–1192, https://doi.org/10.5194/acp-13-1177-2013, https://doi.org/10.5194/acp-13-1177-2013, 2013
Related subject area
Biogeochemistry: Greenhouse Gases
Surface CO2 gradients challenge conventional CO2 emission quantification in lentic water bodies under calm conditions
Spatiotemporal variability of CO2, N2O and CH4 fluxes from a semi-deciduous tropical forest soil in the Congo Basin
Eddy-covariance fluxes of CO2, CH4 and N2O in a drained peatland forest after clear-cutting
Eddy covariance evaluation of ecosystem fluxes at a temperate saltmarsh in Victoria, Australia, shows large CO2 uptake
Interferences caused by the biogeochemical methane cycle in peats during the assessment of abandoned oil wells
Carbon sequestration in different urban vegetation types in Southern Finland
Proglacial methane emissions driven by meltwater and groundwater flushing in a high-Arctic glacial catchment
Seasonal and interannual variability in CO2 fluxes in southern Africa seen by GOSAT
Air temperature and precipitation constraining the modelled wetland methane emissions in a boreal region in northern Europe
Ensemble estimates of global wetland methane emissions over 2000–2020
Seasonal carbon fluxes from vegetation and soil in a Mediterranean non-tidal salt marsh
Explainable machine learning for modeling of net ecosystem exchange in boreal forests
Dynamics of CO2 and CH4 fluxes in Red Sea mangrove soils
Nitrous oxide (N2O) in Macquarie Harbour, Tasmania
Technical note: A low-cost, automatic soil–plant–atmosphere enclosure system to investigate CO2 and evapotranspiration flux dynamics
Tidal influence on carbon dioxide and methane fluxes from tree stems and soils in mangrove forests
Drought conditions disrupt atmospheric carbon uptake in a Mediterranean saline lake
Physicochemical perturbation increases nitrous oxide production from denitrification in soils and sediments
Carbon degradation and mobilisation potentials of thawing permafrost peatlands in northern Norway inferred from laboratory incubations
Seasonal dynamics and regional distribution patterns of CO2 and CH4 in the north-eastern Baltic Sea
Rising Arctic Seas and Thawing Permafrost: Uncovering the Carbon Cycle Impact in a Thermokarst Lagoon System in the outer Mackenzie Delta, Canada
Interannual and seasonal variability of the air–sea CO2 exchange at Utö in the coastal region of the Baltic Sea
Modelling decadal trends and the impact of extreme events on carbon fluxes in a deciduous temperate forest using the QUINCY model
CO2 emissions of drained coastal peatlands in the Netherlands and potential emission reduction by water infiltration systems
Intercomparison of biogenic CO2 flux models in four urban parks in the city of Zurich
Influence of wind strength and direction on diffusive methane fluxes and atmospheric methane concentrations above the North Sea
Using eddy covariance observations to determine the carbon sequestration characteristics of subalpine forests in the Qinghai–Tibet Plateau
Isotopomer labeling and oxygen dependence of hybrid nitrous oxide production
The emission of CO from tropical rainforest soils
CO2 flux characteristics of the grassland ecosystem and its response to environmental factors in the dry-hot valley of Jinsha River, China
Modelling CO2 and N2O emissions from soils in silvopastoral systems of the West African Sahelian band
A case study on topsoil removal and rewetting for paludiculture: effect on biogeochemistry and greenhouse gas emissions from Typha latifolia, Typha angustifolia, and Azolla filiculoides
Observations of methane net sinks in the Arctic tundra
Assessing improvements in global ocean pCO2 machine learning reconstructions with Southern Ocean autonomous sampling
Timescale dependence of airborne fraction and underlying climate–carbon-cycle feedbacks for weak perturbations in CMIP5 models
Technical note: Preventing CO2 overestimation from mercuric or copper(II) chloride preservation of dissolved greenhouse gases in freshwater samples
Exploring temporal and spatial variation of nitrous oxide flux using several years of peatland forest automatic chamber data
Diurnal versus spatial variability of greenhouse gas emissions from an anthropogenically modified lowland river in Germany
Regional assessment and uncertainty analysis of carbon and nitrogen balances at cropland scale using the ecosystem model LandscapeDNDC
Resolving heterogeneous fluxes from tundra halves the growing season carbon budget
Lawns and meadows in urban green space – a comparison from perspectives of greenhouse gases, drought resilience and plant functional types
Large contribution of soil N2O emission to the global warming potential of a large-scale oil palm plantation despite changing from conventional to reduced management practices
Identifying landscape hot and cold spots of soil greenhouse gas fluxes by combining field measurements and remote sensing data
Enhanced Southern Ocean CO2 outgassing as a result of stronger and poleward shifted southern hemispheric westerlies
Spatial and temporal variability of methane emissions and environmental conditions in a hyper-eutrophic fishpond
Optical and radar Earth observation data for upscaling methane emissions linked to permafrost degradation in sub-Arctic peatlands in northern Sweden
Herbivore–shrub interactions influence ecosystem respiration and biogenic volatile organic compound composition in the subarctic
Methane emissions due to reservoir flushing: a significant emission pathway?
Carbon dioxide and methane fluxes from mounds of African fungus-growing termites
Diel and seasonal methane dynamics in the shallow and turbulent Wadden Sea
Patrick Aurich, Uwe Spank, and Matthias Koschorreck
Biogeosciences, 22, 1697–1709, https://doi.org/10.5194/bg-22-1697-2025, https://doi.org/10.5194/bg-22-1697-2025, 2025
Short summary
Short summary
Lakes can be sources and sinks of the greenhouse gas carbon dioxide. The gas exchange between the atmosphere and the water can be measured by taking gas samples from them. However, the depth of water samples is not well defined, which may cause errors. We hypothesized that gradients of CO2 concentrations develop under the surface when wind speeds are very low. Our measurements show that such a gradient can occur on calm nights, potentially shifting lakes from a CO2 sink to a source.
Roxanne Daelman, Marijn Bauters, Matti Barthel, Emmanuel Bulonza, Lodewijk Lefevre, José Mbifo, Johan Six, Klaus Butterbach-Bahl, Benjamin Wolf, Ralf Kiese, and Pascal Boeckx
Biogeosciences, 22, 1529–1542, https://doi.org/10.5194/bg-22-1529-2025, https://doi.org/10.5194/bg-22-1529-2025, 2025
Short summary
Short summary
The increase in atmospheric concentrations of several greenhouse gases (GHGs) since 1750 is attributed to human activity. However, natural ecosystems, such as tropical forests, also contribute to GHG budgets. The Congo Basin hosts the second largest tropical forest and is understudied. In this study, measurements of soil GHG exchange were carried out during 16 months in a tropical forest in the Congo Basin. Overall, the soil acted as a major source of CO2 and N2O and a minor sink of CH4.
Olli-Pekka Tikkasalo, Olli Peltola, Pavel Alekseychik, Juha Heikkinen, Samuli Launiainen, Aleksi Lehtonen, Qian Li, Eduardo Martínez-García, Mikko Peltoniemi, Petri Salovaara, Ville Tuominen, and Raisa Mäkipää
Biogeosciences, 22, 1277–1300, https://doi.org/10.5194/bg-22-1277-2025, https://doi.org/10.5194/bg-22-1277-2025, 2025
Short summary
Short summary
The emissions of greenhouse gases (GHGs) carbon dioxide (CO2), methane (CH4) and nitrous oxide (N2O) were measured from a clear-cut peatland forest site. The measurements covered the whole year of 2022, which was the second growing season after the clear-cut. The site was a strong GHG source, and the highest emissions came from CO2, followed by N2O and CH4. A statistical model that included information on different surfaces at the site was developed to unravel surface-type-specific GHG fluxes.
Ruth Reef, Edoardo Daly, Tivanka Anandappa, Eboni-Jane Vienna-Hallam, Harriet Robertson, Matthew Peck, and Adrien Guyot
Biogeosciences, 22, 1149–1162, https://doi.org/10.5194/bg-22-1149-2025, https://doi.org/10.5194/bg-22-1149-2025, 2025
Short summary
Short summary
Studies show that saltmarshes excel at capturing carbon from the atmosphere. In this study, we measured CO2 flux in an Australian temperate saltmarsh on French Island. The temperate saltmarsh exhibited strong seasonality. During the warmer growing season, the saltmarsh absorbed 10.5 g CO2 m−2 on average daily from the atmosphere. Even in winter, when plants were dormant, it continued to be a CO2 sink, albeit a smaller one. Cool temperatures and high cloud cover inhibit carbon sequestration.
Sebastian F. A. Jordan, Stefan Schloemer, Martin Krüger, Tanja Heffner, Marcus A. Horn, and Martin Blumenberg
Biogeosciences, 22, 809–830, https://doi.org/10.5194/bg-22-809-2025, https://doi.org/10.5194/bg-22-809-2025, 2025
Short summary
Short summary
Using a multilayer approach, we studied the methane flux, soil gas composition, and isotopic signatures of soil methane and carbon dioxide at eight cut and buried abandoned oil wells in a peat-rich area of northern Germany. The detected methane emissions were of biogenic, peat origin and were not associated with the abandoned wells. Additional microbial analysis and methane oxidation rate measurements demonstrated a high methane emission mitigation potential in the studied peat soils.
Laura Thölix, Leif Backman, Minttu Havu, Esko Karvinen, Jesse Soininen, Justine Trémeau, Olli Nevalainen, Joyson Ahongshangbam, Leena Järvi, and Liisa Kulmala
Biogeosciences, 22, 725–749, https://doi.org/10.5194/bg-22-725-2025, https://doi.org/10.5194/bg-22-725-2025, 2025
Short summary
Short summary
Cities aim for carbon neutrality and seek to understand urban vegetation's role as a carbon sink. Direct measurements are challenging, so models are used to estimate the urban carbon cycle. We evaluated model performance at estimating carbon sequestration in lawns, park trees, and urban forests in Helsinki, Finland. Models captured seasonal and annual variations well. Trees had higher sequestration rates than lawns, and irrigation often enhanced carbon sinks.
Gabrielle E. Kleber, Leonard Magerl, Alexandra V. Turchyn, Stefan Schloemer, Mark Trimmer, Yizhu Zhu, and Andrew Hodson
Biogeosciences, 22, 659–674, https://doi.org/10.5194/bg-22-659-2025, https://doi.org/10.5194/bg-22-659-2025, 2025
Short summary
Short summary
Our research on Svalbard shows that glacier melt rivers can transport large amounts of methane, a potent greenhouse gas. By studying a glacier over one summer, we found that its river was highly concentrated in methane, suggesting that rivers could provide a significant source of methane emissions as the Arctic warms and glaciers melt. This is the first time such emissions have been measured on Svalbard, indicating a wider environmental concern as such processes are occurring across the Arctic.
Eva-Marie Metz, Sanam Noreen Vardag, Sourish Basu, Martin Jung, and André Butz
Biogeosciences, 22, 555–584, https://doi.org/10.5194/bg-22-555-2025, https://doi.org/10.5194/bg-22-555-2025, 2025
Short summary
Short summary
We estimate CO2 fluxes in semiarid southern Africa from 2009 to 2018 based on satellite CO2 measurements and atmospheric inverse modeling. By selecting process-based vegetation models, which agree with the satellite CO2 fluxes, we find that soil respiration mainly drives the seasonality, whereas photosynthesis substantially influences the interannual variability. Our study emphasizes the need for better representation of the response of semiarid ecosystems to soil rewetting in vegetation models.
Tuula Aalto, Aki Tsuruta, Jarmo Mäkelä, Jurek Müller, Maria Tenkanen, Eleanor Burke, Sarah Chadburn, Yao Gao, Vilma Mannisenaho, Thomas Kleinen, Hanna Lee, Antti Leppänen, Tiina Markkanen, Stefano Materia, Paul A. Miller, Daniele Peano, Olli Peltola, Benjamin Poulter, Maarit Raivonen, Marielle Saunois, David Wårlind, and Sönke Zaehle
Biogeosciences, 22, 323–340, https://doi.org/10.5194/bg-22-323-2025, https://doi.org/10.5194/bg-22-323-2025, 2025
Short summary
Short summary
Wetland methane responses to temperature and precipitation were studied in a boreal wetland-rich region in northern Europe using ecosystem models, atmospheric inversions, and upscaled flux observations. The ecosystem models differed in their responses to temperature and precipitation and in their seasonality. However, multi-model means, inversions, and upscaled fluxes had similar seasonality, and they suggested co-limitation by temperature and precipitation.
Zhen Zhang, Benjamin Poulter, Joe R. Melton, William J. Riley, George H. Allen, David J. Beerling, Philippe Bousquet, Josep G. Canadell, Etienne Fluet-Chouinard, Philippe Ciais, Nicola Gedney, Peter O. Hopcroft, Akihiko Ito, Robert B. Jackson, Atul K. Jain, Katherine Jensen, Fortunat Joos, Thomas Kleinen, Sara H. Knox, Tingting Li, Xin Li, Xiangyu Liu, Kyle McDonald, Gavin McNicol, Paul A. Miller, Jurek Müller, Prabir K. Patra, Changhui Peng, Shushi Peng, Zhangcai Qin, Ryan M. Riggs, Marielle Saunois, Qing Sun, Hanqin Tian, Xiaoming Xu, Yuanzhi Yao, Yi Xi, Wenxin Zhang, Qing Zhu, Qiuan Zhu, and Qianlai Zhuang
Biogeosciences, 22, 305–321, https://doi.org/10.5194/bg-22-305-2025, https://doi.org/10.5194/bg-22-305-2025, 2025
Short summary
Short summary
This study assesses global methane emissions from wetlands between 2000 and 2020 using multiple models. We found that wetland emissions increased by 6–7 Tg CH4 yr-1 in the 2010s compared to the 2000s. Rising temperatures primarily drove this increase, while changes in precipitation and CO2 levels also played roles. Our findings highlight the importance of wetlands in the global methane budget and the need for continuous monitoring to understand their impact on climate change.
Lorena Carrasco-Barea, Dolors Verdaguer, Maria Gispert, Xavier D. Quintana, Hélène Bourhis, and Laura Llorens
Biogeosciences, 22, 289–304, https://doi.org/10.5194/bg-22-289-2025, https://doi.org/10.5194/bg-22-289-2025, 2025
Short summary
Short summary
Carbon dioxide fluxes have been measured seasonally in four plant species in a Mediterranean non-tidal salt marsh, highlighting the high carbon removal potential that these species have. Carbon dioxide and methane emissions from soil showed high variability among the habitats studied, and they were generally higher than those observed in tidal salt marshes. Our results are important for making more accurate predictions regarding carbon emissions from these ecosystems.
Ekaterina Ezhova, Topi Laanti, Anna Lintunen, Pasi Kolari, Tuomo Nieminen, Ivan Mammarella, Keijo Heljanko, and Markku Kulmala
Biogeosciences, 22, 257–288, https://doi.org/10.5194/bg-22-257-2025, https://doi.org/10.5194/bg-22-257-2025, 2025
Short summary
Short summary
Machine learning (ML) models are gaining popularity in biogeosciences. They are applied as gap-filling methods and used to upscale carbon fluxes to larger areas. Here we use explainable artificial intelligence (XAI) methods to elucidate the performance of machine learning models for carbon dioxide fluxes in boreal forests. We show that statistically equal models treat input variables differently. XAI methods can help scientists make informed decisions when applying ML models in their research.
Jessica Breavington, Alexandra Steckbauer, Chuancheng Fu, Mongi Ennasri, and Carlos M. Duarte
Biogeosciences, 22, 117–134, https://doi.org/10.5194/bg-22-117-2025, https://doi.org/10.5194/bg-22-117-2025, 2025
Short summary
Short summary
Mangrove carbon storage in the Red Sea is lower than average due to challenging growth conditions. We collected mangrove soil cores over multiple seasons to measure greenhouse gas (GHG) flux of carbon dioxide and methane. GHG emissions are a small offset to mangrove carbon storage overall but punctuated by periods of high emission. This variation is linked to environmental and soil properties, which were also measured. The findings aid understanding of GHG dynamics in arid mangrove ecosystems.
Johnathan Daniel Maxey, Neil D. Hartstein, Hermann W. Bange, and Moritz Müller
Biogeosciences, 21, 5613–5637, https://doi.org/10.5194/bg-21-5613-2024, https://doi.org/10.5194/bg-21-5613-2024, 2024
Short summary
Short summary
The distribution of N2O in fjord-like estuaries is poorly described in the Southern Hemisphere. Our study describes N2O distribution and its drivers in one such system in Macquarie Harbour, Tasmania. Water samples were collected seasonally in 2022 and 2023. Results show the system removes atmospheric N2O when river flow is high, whereas the system emits N2O when the river flow is low. N2O generated in basins is intercepted by the surface water and exported to the ocean during high river flow.
Wael Al Hamwi, Maren Dubbert, Jörg Schaller, Matthias Lück, Marten Schmidt, and Mathias Hoffmann
Biogeosciences, 21, 5639–5651, https://doi.org/10.5194/bg-21-5639-2024, https://doi.org/10.5194/bg-21-5639-2024, 2024
Short summary
Short summary
We present a fully automatic, low-cost soil–plant enclosure system to monitor CO2 and evapotranspiration fluxes within greenhouse experiments. It operates in two modes: independent, using low-cost sensors, and dependent, where multiple chambers connect to a single gas analyzer via a low-cost multiplexer. This system provides precise, accurate measurements and high temporal resolution, enabling comprehensive monitoring of plant–soil responses to various treatments and conditions.
Zhao-Jun Yong, Wei-Jen Lin, Chiao-Wen Lin, and Hsing-Juh Lin
Biogeosciences, 21, 5247–5260, https://doi.org/10.5194/bg-21-5247-2024, https://doi.org/10.5194/bg-21-5247-2024, 2024
Short summary
Short summary
We measured CO2 and CH4 fluxes from mangrove stems and soils of Avicennia marina and Kandelia obovata during tidal cycles. Both stem types served as CO2 and CH4 sources, emitting less CH4 than soils, with no difference in CO2 flux. While A. marina stems showed increased CO2 fluxes from low to high tides, they acted as a CH4 sink before flooding and as a source after ebbing. However, K. obovata stems showed no flux pattern. This study highlights the need to consider tidal influence and species.
Ihab Alfadhel, Ignacio Peralta-Maraver, Isabel Reche, Enrique P. Sánchez-Cañete, Sergio Aranda-Barranco, Eva Rodríguez-Velasco, Andrew S. Kowalski, and Penélope Serrano-Ortiz
Biogeosciences, 21, 5117–5129, https://doi.org/10.5194/bg-21-5117-2024, https://doi.org/10.5194/bg-21-5117-2024, 2024
Short summary
Short summary
Inland saline lakes are crucial in the global carbon cycle, but increased droughts may alter their carbon exchange capacity. We measured CO2 and CH4 fluxes in a Mediterranean saline lake using the eddy covariance method under dry and wet conditions. We found the lake acts as a carbon sink during wet periods but not during droughts. These results highlight the importance of saline lakes in carbon sequestration and their vulnerability to climate-change-induced droughts.
Nathaniel B. Weston, Cynthia Troy, Patrick J. Kearns, Jennifer L. Bowen, William Porubsky, Christelle Hyacinthe, Christof Meile, Philippe Van Cappellen, and Samantha B. Joye
Biogeosciences, 21, 4837–4851, https://doi.org/10.5194/bg-21-4837-2024, https://doi.org/10.5194/bg-21-4837-2024, 2024
Short summary
Short summary
Nitrous oxide (N2O) is a potent greenhouse and ozone-depleting gas produced largely from microbial nitrogen cycling processes, and human activities have resulted in increases in atmospheric N2O. We investigate the role of physical and chemical disturbances to soils and sediments in N2O production. We demonstrate that physicochemical perturbation increases N2O production, microbial community adapts over time, and initial perturbation appears to confer resilience to subsequent disturbance.
Sigrid Trier Kjær, Sebastian Westermann, Nora Nedkvitne, and Peter Dörsch
Biogeosciences, 21, 4723–4737, https://doi.org/10.5194/bg-21-4723-2024, https://doi.org/10.5194/bg-21-4723-2024, 2024
Short summary
Short summary
Permafrost peatlands are thawing due to climate change, releasing large quantities of carbon that degrades upon thawing and is released as CO2, CH4 or dissolved organic carbon (DOC). We incubated thawed Norwegian permafrost peat plateaus and thermokarst pond sediment found next to permafrost for up to 350 d to measure carbon loss. CO2 production was initially the highest, whereas CH4 production increased over time. The largest carbon loss was measured at the top of the peat plateau core as DOC.
Silvie Lainela, Erik Jacobs, Stella-Theresa Luik, Gregor Rehder, and Urmas Lips
Biogeosciences, 21, 4495–4519, https://doi.org/10.5194/bg-21-4495-2024, https://doi.org/10.5194/bg-21-4495-2024, 2024
Short summary
Short summary
We evaluate the variability of carbon dioxide and methane in the surface layer of the north-eastern basins of the Baltic Sea in 2018. We show that the shallower coastal areas have considerably higher spatial variability and seasonal amplitude of surface layer pCO2 and cCH4 than measured in the offshore areas of the Baltic Sea. Despite this high variability, caused mostly by coastal physical processes, the average annual air–sea CO2 fluxes differed only marginally between the sub-basins.
Maren Jenrich, Juliane Wolter, Susanne Liebner, Christian Knoblauch, Guido Grosse, Fiona Giebeler, Dustin Whalen, and Jens Strauss
EGUsphere, https://doi.org/10.5194/egusphere-2024-2891, https://doi.org/10.5194/egusphere-2024-2891, 2024
Short summary
Short summary
Climate warming in the Arctic is causing the erosion of permafrost coasts and the transformation of permafrost lakes into lagoons. To understand how this affects greenhouse gas (GHG) emissions, we studied carbon dioxide (CO₂) and methane (CH₄) production in lagoons with varying sea connections. Younger lagoons produce more CH₄, while CO₂ increases in more marine conditions. Flooding of permafrost lowlands due to rising sea levels may lead to higher GHG emissions from Arctic coasts in the future.
Martti Honkanen, Mika Aurela, Juha Hatakka, Lumi Haraguchi, Sami Kielosto, Timo Mäkelä, Jukka Seppälä, Simo-Matti Siiriä, Ken Stenbäck, Juha-Pekka Tuovinen, Pasi Ylöstalo, and Lauri Laakso
Biogeosciences, 21, 4341–4359, https://doi.org/10.5194/bg-21-4341-2024, https://doi.org/10.5194/bg-21-4341-2024, 2024
Short summary
Short summary
The exchange of CO2 between the sea and the atmosphere was studied in the Archipelago Sea, Baltic Sea, in 2017–2021, using an eddy covariance technique. The sea acted as a net source of CO2 with an average yearly emission of 27.1 gC m-2 yr-1, indicating that the marine ecosystem respired carbon that originated elsewhere. The yearly CO2 emission varied between 18.2–39.2 gC m-2 yr-1, mostly due to the yearly variation of ecosystem carbon uptake.
Tea Thum, Tuuli Miinalainen, Outi Seppälä, Holly Croft, Cheryl Rogers, Ralf Staebler, Silvia Caldararu, and Sönke Zaehle
EGUsphere, https://doi.org/10.5194/egusphere-2024-2802, https://doi.org/10.5194/egusphere-2024-2802, 2024
Short summary
Short summary
Climate change has potential to influence the carbon sequestration potential of terrestrial ecosystems and here also nitrogen cycle is important. We used a terrestrial biosphere model QUINCY at mixed deciduous forest in Canada. We investigated the usefulness of using leaf area index and leaf chlorophyll content to improve the parameterization of the model. This work paves way for using spaceborn observations in the model parameterization, also including information on the nitrogen cycle.
Ralf C. H. Aben, Daniël van de Craats, Jim Boonman, Stijn H. Peeters, Bart Vriend, Coline C. F. Boonman, Ype van der Velde, Gilles Erkens, and Merit van den Berg
Biogeosciences, 21, 4099–4118, https://doi.org/10.5194/bg-21-4099-2024, https://doi.org/10.5194/bg-21-4099-2024, 2024
Short summary
Short summary
Drained peatlands cause high CO2 emissions. We assessed the effectiveness of subsurface water infiltration systems (WISs) in reducing CO2 emissions related to increases in water table depth (WTD) on 12 sites for up to 4 years. Results show WISs markedly reduced emissions by 2.1 t CO2-C ha-1 yr-1. The relationship between the amount of carbon above the WTD and CO2 emission was stronger than the relationship between WTD and emission. Long-term monitoring is crucial for accurate emission estimates.
Stavros Stagakis, Dominik Brunner, Junwei Li, Leif Backman, Anni Karvonen, Lionel Constantin, Leena Järvi, Minttu Havu, Jia Chen, Sophie Emberger, and Liisa Kulmala
EGUsphere, https://doi.org/10.5194/egusphere-2024-2475, https://doi.org/10.5194/egusphere-2024-2475, 2024
Short summary
Short summary
The balance between CO2 uptake and emissions from urban green areas is still not well understood. This study evaluated for the first time the urban park CO2 exchange simulations by four different types of biosphere models by comparing them with observations. Even though some advantages and disadvantages of the different model types were identified, there was no strong evidence that more complex models performed better than simple ones.
Ingeborg Bussmann, Eric P. Achterberg, Holger Brix, Nicolas Brüggemann, Götz Flöser, Claudia Schütze, and Philipp Fischer
Biogeosciences, 21, 3819–3838, https://doi.org/10.5194/bg-21-3819-2024, https://doi.org/10.5194/bg-21-3819-2024, 2024
Short summary
Short summary
Methane (CH4) is an important greenhouse gas and contributes to climate warming. However, the input of CH4 from coastal areas to the atmosphere is not well defined. Dissolved and atmospheric CH4 was determined at high spatial resolution in or above the North Sea. The atmospheric CH4 concentration was mainly influenced by wind direction. With our detailed study on the spatial distribution of CH4 fluxes we were able to provide a detailed and more realistic estimation of coastal CH4 fluxes.
Niu Zhu, Jinniu Wang, Dongliang Luo, Xufeng Wang, Cheng Shen, and Ning Wu
Biogeosciences, 21, 3509–3522, https://doi.org/10.5194/bg-21-3509-2024, https://doi.org/10.5194/bg-21-3509-2024, 2024
Short summary
Short summary
Our study delves into the vital role of subalpine forests in the Qinghai–Tibet Plateau as carbon sinks in the context of climate change. Utilizing advanced eddy covariance systems, we uncover their significant carbon sequestration potential, observing distinct seasonal patterns influenced by temperature, humidity, and radiation. Notably, these forests exhibit robust carbon absorption, with potential implications for global carbon balance.
Colette L. Kelly, Nicole M. Travis, Pascale Anabelle Baya, Claudia Frey, Xin Sun, Bess B. Ward, and Karen L. Casciotti
Biogeosciences, 21, 3215–3238, https://doi.org/10.5194/bg-21-3215-2024, https://doi.org/10.5194/bg-21-3215-2024, 2024
Short summary
Short summary
Nitrous oxide, a potent greenhouse gas, accumulates in regions of the ocean that are low in dissolved oxygen. We used a novel combination of chemical tracers to determine how nitrous oxide is produced in one of these regions, the eastern tropical North Pacific Ocean. Our experiments showed that the two most important sources of nitrous oxide under low-oxygen conditions are denitrification, an anaerobic process, and a novel “hybrid” process performed by ammonia-oxidizing archaea.
Hella van Asperen, Thorsten Warneke, Alessandro Carioca de Araújo, Bruce Forsberg, Sávio José Filgueiras Ferreira, Thomas Röckmann, Carina van der Veen, Sipko Bulthuis, Leonardo Ramos de Oliveira, Thiago de Lima Xavier, Jailson da Mata, Marta de Oliveira Sá, Paulo Ricardo Teixeira, Julie Andrews de França e Silva, Susan Trumbore, and Justus Notholt
Biogeosciences, 21, 3183–3199, https://doi.org/10.5194/bg-21-3183-2024, https://doi.org/10.5194/bg-21-3183-2024, 2024
Short summary
Short summary
Carbon monoxide (CO) is regarded as an important indirect greenhouse gas. Soils can emit and take up CO, but, until now, uncertainty remains as to which process dominates in tropical rainforests. We present the first soil CO flux measurements from a tropical rainforest. Based on our observations, we report that tropical rainforest soils are a net source of CO. In addition, we show that valley streams and inundated areas are likely additional hot spots of CO in the ecosystem.
Chaolei Yang, Yufeng Tian, Jingqi Cui, Guangxiong He, Jingyuan Li, Canfeng Li, Haichuang Duan, Zong Wei, Liu Yan, Xin Xia, Yong Huang, and Aihua Jiang
EGUsphere, https://doi.org/10.5194/egusphere-2024-1226, https://doi.org/10.5194/egusphere-2024-1226, 2024
Short summary
Short summary
The environmental factors and CO2 flux of the grassland ecosystem in the dry-hot valley of the Jinsha River exhibited highly seasonal characteristics. During the rainy season, the grassland showed a carbon sink feature, while during the dry season, it exhibited carbon emission status. Throughout the entire year, the grassland ecosystem acted as a weak carbon source, exhibiting a carbon-neutral. The CO2 flux was most influenced by vapor pressure deficit, relative humidity, and soil water content.
Yélognissè Agbohessou, Claire Delon, Manuela Grippa, Eric Mougin, Daouda Ngom, Espoir Koudjo Gaglo, Ousmane Ndiaye, Paulo Salgado, and Olivier Roupsard
Biogeosciences, 21, 2811–2837, https://doi.org/10.5194/bg-21-2811-2024, https://doi.org/10.5194/bg-21-2811-2024, 2024
Short summary
Short summary
Emissions of greenhouse gases in the Sahel are not well represented because they are considered weak compared to the rest of the world. However, natural areas in the Sahel emit carbon dioxide and nitrous oxides, which need to be assessed because of extended surfaces. We propose an assessment of such emissions in Sahelian silvopastoral systems and of how they are influenced by environmental characteristics. These results are essential to inform climate change strategies in the region.
Merit van den Berg, Thomas M. Gremmen, Renske J. E. Vroom, Jacobus van Huissteden, Jim Boonman, Corine J. A. van Huissteden, Ype van der Velde, Alfons J. P. Smolders, and Bas P. van de Riet
Biogeosciences, 21, 2669–2690, https://doi.org/10.5194/bg-21-2669-2024, https://doi.org/10.5194/bg-21-2669-2024, 2024
Short summary
Short summary
Drained peatlands emit 3 % of the global greenhouse gas emissions. Paludiculture is a way to reduce CO2 emissions while at the same time generating an income for landowners. The side effect is the potentially high methane emissions. We found very high methane emissions for broadleaf cattail compared with narrowleaf cattail and water fern. The rewetting was, however, effective to stop CO2 emissions for all species. The highest potential to reduce greenhouse gas emissions had narrowleaf cattail.
Antonio Donateo, Daniela Famulari, Donato Giovannelli, Arturo Mariani, Mauro Mazzola, Stefano Decesari, and Gianluca Pappaccogli
EGUsphere, https://doi.org/10.5194/egusphere-2024-1440, https://doi.org/10.5194/egusphere-2024-1440, 2024
Short summary
Short summary
This study focuses on direct measurements of CO2 and CH4 turbulent eddy covariance fluxes in tundra ecosystems in the Svalbard Islands over a two-year period. Our results reveal dynamic interactions between climatic conditions and ecosystem activities such as photosynthesis and microbial activity. The observed net summertime methane uptake is correlated with the activation and aeration of soil microorganisms. High temperature anomalies increase CO2 and CH4 emissions.
Thea H. Heimdal, Galen A. McKinley, Adrienne J. Sutton, Amanda R. Fay, and Lucas Gloege
Biogeosciences, 21, 2159–2176, https://doi.org/10.5194/bg-21-2159-2024, https://doi.org/10.5194/bg-21-2159-2024, 2024
Short summary
Short summary
Measurements of ocean carbon are limited in time and space. Machine learning algorithms are therefore used to reconstruct ocean carbon where observations do not exist. Improving these reconstructions is important in order to accurately estimate how much carbon the ocean absorbs from the atmosphere. In this study, we find that a small addition of observations from the Southern Ocean, obtained by autonomous sampling platforms, could significantly improve the reconstructions.
Guilherme L. Torres Mendonça, Julia Pongratz, and Christian H. Reick
Biogeosciences, 21, 1923–1960, https://doi.org/10.5194/bg-21-1923-2024, https://doi.org/10.5194/bg-21-1923-2024, 2024
Short summary
Short summary
We study the timescale dependence of airborne fraction and underlying feedbacks by a theory of the climate–carbon system. Using simulations we show the predictive power of this theory and find that (1) this fraction generally decreases for increasing timescales and (2) at all timescales the total feedback is negative and the model spread in a single feedback causes the spread in the airborne fraction. Our study indicates that those are properties of the system, independently of the scenario.
François Clayer, Jan Erik Thrane, Kuria Ndungu, Andrew King, Peter Dörsch, and Thomas Rohrlack
Biogeosciences, 21, 1903–1921, https://doi.org/10.5194/bg-21-1903-2024, https://doi.org/10.5194/bg-21-1903-2024, 2024
Short summary
Short summary
Determination of dissolved greenhouse gas (GHG) in freshwater allows us to estimate GHG fluxes. Mercuric chloride (HgCl2) is used to preserve water samples prior to GHG analysis despite its environmental and health impacts and interferences with water chemistry in freshwater. Here, we tested the effects of HgCl2, two substitutes and storage time on GHG in water from two boreal lakes. Preservation with HgCl2 caused overestimation of CO2 concentration with consequences for GHG flux estimation.
Helena Rautakoski, Mika Korkiakoski, Jarmo Mäkelä, Markku Koskinen, Kari Minkkinen, Mika Aurela, Paavo Ojanen, and Annalea Lohila
Biogeosciences, 21, 1867–1886, https://doi.org/10.5194/bg-21-1867-2024, https://doi.org/10.5194/bg-21-1867-2024, 2024
Short summary
Short summary
Current and future nitrous oxide (N2O) emissions are difficult to estimate due to their high variability in space and time. Several years of N2O fluxes from drained boreal peatland forest indicate high importance of summer precipitation, winter temperature, and snow conditions in controlling annual N2O emissions. The results indicate increasing year-to-year variation in N2O emissions in changing climate with more extreme seasonal weather conditions.
Matthias Koschorreck, Norbert Kamjunke, Uta Koedel, Michael Rode, Claudia Schuetze, and Ingeborg Bussmann
Biogeosciences, 21, 1613–1628, https://doi.org/10.5194/bg-21-1613-2024, https://doi.org/10.5194/bg-21-1613-2024, 2024
Short summary
Short summary
We measured the emission of carbon dioxide (CO2) and methane (CH4) from different sites at the river Elbe in Germany over 3 days to find out what is more important for quantification: small-scale spatial variability or diurnal temporal variability. We found that CO2 emissions were very different between day and night, while CH4 emissions were more different between sites. Dried out river sediments contributed to CO2 emissions, while the side areas of the river were important CH4 sources.
Odysseas Sifounakis, Edwin Haas, Klaus Butterbach-Bahl, and Maria P. Papadopoulou
Biogeosciences, 21, 1563–1581, https://doi.org/10.5194/bg-21-1563-2024, https://doi.org/10.5194/bg-21-1563-2024, 2024
Short summary
Short summary
We performed a full assessment of the carbon and nitrogen cycles of a cropland ecosystem. An uncertainty analysis and quantification of all carbon and nitrogen fluxes were deployed. The inventory simulations include greenhouse gas emissions of N2O, NH3 volatilization and NO3 leaching from arable land cultivation in Greece. The inventory also reports changes in soil organic carbon and nitrogen stocks in arable soils.
Sarah M. Ludwig, Luke Schiferl, Jacqueline Hung, Susan M. Natali, and Roisin Commane
Biogeosciences, 21, 1301–1321, https://doi.org/10.5194/bg-21-1301-2024, https://doi.org/10.5194/bg-21-1301-2024, 2024
Short summary
Short summary
Landscapes are often assumed to be homogeneous when using eddy covariance fluxes, which can lead to biases when calculating carbon budgets. In this study we report eddy covariance carbon fluxes from heterogeneous tundra. We used the footprints of each flux observation to unmix the fluxes coming from components of the landscape. We identified and quantified hot spots of carbon emissions in the landscape. Accurately scaling with landscape heterogeneity yielded half as much regional carbon uptake.
Justine Trémeau, Beñat Olascoaga, Leif Backman, Esko Karvinen, Henriikka Vekuri, and Liisa Kulmala
Biogeosciences, 21, 949–972, https://doi.org/10.5194/bg-21-949-2024, https://doi.org/10.5194/bg-21-949-2024, 2024
Short summary
Short summary
We studied urban lawns and meadows in the Helsinki metropolitan area, Finland. We found that meadows are more resistant to drought events but that they do not increase carbon sequestration compared with lawns. Moreover, the transformation from lawns to meadows did not demonstrate any negative climate effects in terms of greenhouse gas emissions. Even though social and economic aspects also steer urban development, these results can guide planning to consider carbon-smart options.
Guantao Chen, Edzo Veldkamp, Muhammad Damris, Bambang Irawan, Aiyen Tjoa, and Marife D. Corre
Biogeosciences, 21, 513–529, https://doi.org/10.5194/bg-21-513-2024, https://doi.org/10.5194/bg-21-513-2024, 2024
Short summary
Short summary
We established an oil palm management experiment in a large-scale oil palm plantation in Jambi, Indonesia. We recorded oil palm fruit yield and measured soil CO2, N2O, and CH4 fluxes. After 4 years of treatment, compared with conventional fertilization with herbicide weeding, reduced fertilization with mechanical weeding did not reduce yield and soil greenhouse gas emissions, which highlights the legacy effects of over a decade of conventional management prior to the start of the experiment.
Elizabeth Gachibu Wangari, Ricky Mwangada Mwanake, Tobias Houska, David Kraus, Gretchen Maria Gettel, Ralf Kiese, Lutz Breuer, and Klaus Butterbach-Bahl
Biogeosciences, 20, 5029–5067, https://doi.org/10.5194/bg-20-5029-2023, https://doi.org/10.5194/bg-20-5029-2023, 2023
Short summary
Short summary
Agricultural landscapes act as sinks or sources of the greenhouse gases (GHGs) CO2, CH4, or N2O. Various physicochemical and biological processes control the fluxes of these GHGs between ecosystems and the atmosphere. Therefore, fluxes depend on environmental conditions such as soil moisture, soil temperature, or soil parameters, which result in large spatial and temporal variations of GHG fluxes. Here, we describe an example of how this variation may be studied and analyzed.
Laurie C. Menviel, Paul Spence, Andrew E. Kiss, Matthew A. Chamberlain, Hakase Hayashida, Matthew H. England, and Darryn Waugh
Biogeosciences, 20, 4413–4431, https://doi.org/10.5194/bg-20-4413-2023, https://doi.org/10.5194/bg-20-4413-2023, 2023
Short summary
Short summary
As the ocean absorbs 25% of the anthropogenic emissions of carbon, it is important to understand the impact of climate change on the flux of carbon between the ocean and the atmosphere. Here, we use a very high-resolution ocean, sea-ice, carbon cycle model to show that the capability of the Southern Ocean to uptake CO2 has decreased over the last 40 years due to a strengthening and poleward shift of the southern hemispheric westerlies. This trend is expected to continue over the coming century.
Petr Znachor, Jiří Nedoma, Vojtech Kolar, and Anna Matoušů
Biogeosciences, 20, 4273–4288, https://doi.org/10.5194/bg-20-4273-2023, https://doi.org/10.5194/bg-20-4273-2023, 2023
Short summary
Short summary
We conducted intensive spatial sampling of the hypertrophic fishpond to better understand the spatial dynamics of methane fluxes and environmental heterogeneity in fishponds. The diffusive fluxes of methane accounted for only a minor fraction of the total fluxes and both varied pronouncedly within the pond and over the studied summer season. This could be explained only by the water depth. Wind substantially affected temperature, oxygen and chlorophyll a distribution in the pond.
Sofie Sjögersten, Martha Ledger, Matthias Siewert, Betsabé de la Barreda-Bautista, Andrew Sowter, David Gee, Giles Foody, and Doreen S. Boyd
Biogeosciences, 20, 4221–4239, https://doi.org/10.5194/bg-20-4221-2023, https://doi.org/10.5194/bg-20-4221-2023, 2023
Short summary
Short summary
Permafrost thaw in Arctic regions is increasing methane emissions, but quantification is difficult given the large and remote areas impacted. We show that UAV data together with satellite data can be used to extrapolate emissions across the wider landscape as well as detect areas at risk of higher emissions. A transition of currently degrading areas to fen type vegetation can increase emission by several orders of magnitude, highlighting the importance of quantifying areas at risk.
Cole G. Brachmann, Tage Vowles, Riikka Rinnan, Mats P. Björkman, Anna Ekberg, and Robert G. Björk
Biogeosciences, 20, 4069–4086, https://doi.org/10.5194/bg-20-4069-2023, https://doi.org/10.5194/bg-20-4069-2023, 2023
Short summary
Short summary
Herbivores change plant communities through grazing, altering the amount of CO2 and plant-specific chemicals (termed VOCs) emitted. We tested this effect by excluding herbivores and studying the CO2 and VOC emissions. Herbivores reduced CO2 emissions from a meadow community and altered VOC composition; however, community type had the strongest effect on the amount of CO2 and VOCs released. Herbivores can mediate greenhouse gas emissions, but the effect is marginal and community dependent.
Ole Lessmann, Jorge Encinas Fernández, Karla Martínez-Cruz, and Frank Peeters
Biogeosciences, 20, 4057–4068, https://doi.org/10.5194/bg-20-4057-2023, https://doi.org/10.5194/bg-20-4057-2023, 2023
Short summary
Short summary
Based on a large dataset of seasonally resolved methane (CH4) pore water concentrations in a reservoir's sediment, we assess the significance of CH4 emissions due to reservoir flushing. In the studied reservoir, CH4 emissions caused by one flushing operation can represent 7 %–14 % of the annual CH4 emissions and depend on the timing of the flushing operation. In reservoirs with high sediment loadings, regular flushing may substantially contribute to the overall CH4 emissions.
Matti Räsänen, Risto Vesala, Petri Rönnholm, Laura Arppe, Petra Manninen, Markus Jylhä, Jouko Rikkinen, Petri Pellikka, and Janne Rinne
Biogeosciences, 20, 4029–4042, https://doi.org/10.5194/bg-20-4029-2023, https://doi.org/10.5194/bg-20-4029-2023, 2023
Short summary
Short summary
Fungus-growing termites recycle large parts of dead plant material in African savannas and are significant sources of greenhouse gases. We measured CO2 and CH4 fluxes from their mounds and surrounding soils in open and closed habitats. The fluxes scale with mound volume. The results show that emissions from mounds of fungus-growing termites are more stable than those from other termites. The soil fluxes around the mound are affected by the termite colonies at up to 2 m distance from the mound.
Tim René de Groot, Anne Margriet Mol, Katherine Mesdag, Pierre Ramond, Rachel Ndhlovu, Julia Catherine Engelmann, Thomas Röckmann, and Helge Niemann
Biogeosciences, 20, 3857–3872, https://doi.org/10.5194/bg-20-3857-2023, https://doi.org/10.5194/bg-20-3857-2023, 2023
Short summary
Short summary
This study investigates methane dynamics in the Wadden Sea. Our measurements revealed distinct variations triggered by seasonality and tidal forcing. The methane budget was higher in warmer seasons but surprisingly high in colder seasons. Methane dynamics were amplified during low tides, flushing the majority of methane into the North Sea or releasing it to the atmosphere. Methanotrophic activity was also elevated during low tide but mitigated only a small fraction of the methane efflux.
Cited articles
Aubinet, M., Berbigier, P., Bernhofer, C., Cescatti, A., Feigenwinter, C., Granier, A., Grünwald, T., Havrankova, K., Heinesch, B., Longdoz, B., Marcolla, B., Montagnani, L., and Sedlak, P.: Comparing CO2 Storage and Advection Conditions at Night at Different Carboeuroflux Sites, Bound.-Lay. Meteorol., 116, 63–93, https://doi.org/10.1007/s10546-004-7091-8, 2005.
Bakwin, P. S., Tans, P. P., Zhao, C., Ussler, W., and Quesnell, E.: Measurements of carbon dioxide on a very tall tower, Tellus B, 47, 535–549, https://doi.org/10.1034/j.1600-0889.47.issue5.2.x, 1995.
Bakwin, P. S., Tans, P. P., Hurst, D. F., and Zhao, C.: Measurements of carbon dioxide on very tall towers: results of the NOAA/CMDL program, Tellus B, 50, 401–415, https://doi.org/10.1034/j.1600-0889.1998.t01-4-00001.x, 1998.
Bakwin, P. S., Davis, K. J., Yi, C., Wofsy, S. C., Munger, J. W., Haszpra, L., and Barcza, Z.: Regional carbon dioxide fluxes from mixing ratio data, Tellus B, 56, 301–311, https://doi.org/10.3402/tellusb.v56i4.16446, 2004.
Berhanu, T. A., Satar, E., Schanda, R., Nyfeler, P., Moret, H., Brunner, D., Oney, B., and Leuenberger, M.: Measurements of greenhouse gases at Beromünster tall tower station in Switzerland, Atmos. Meas. Tech. Discuss., 8, 10793–10822, https://doi.org/10.5194/amtd-8-10793-2015, 2015.
Berhanu, T. A., Satar, E., Szidat S., Brunner D., Schanda R., Nyfeler, P., Leuenberger, M., Steinbacher, M., Hammer, S., and Levin, I.: Quantification of fossil fuel associated CO2 emissions based on radiocarbon measurements at Beromünster tall tower, Switzerland, in preparation, 2016.
Broquet, G., Chevallier, F., Bréon, F.-M., Kadygrov, N., Alemanno, M., Apadula, F., Hammer, S., Haszpra, L., Meinhardt, F., Morguí, J. A., Necki, J., Piacentino, S., Ramonet, M., Schmidt, M., Thompson, R. L., Vermeulen, A. T., Yver, C., and Ciais, P.: Regional inversion of CO2 ecosystem fluxes from atmospheric measurements: reliability of the uncertainty estimates, Atmos. Chem. Phys., 13, 9039–9056, https://doi.org/10.5194/acp-13-9039-2013, 2013.
Ciais, P., Sabine, C., Bala, G., Bopp, L., Brovkin, V., Canadell, J., Chhabra, A., DeFries, R., Galloway, J., Heimann, M., Jones, C., Le Quèrè, C., Myneni, R. B., Piao, S., and Thornton, P.: Carbon and Other Biogeochemical Cycles, in: Climate Change 2013: The Physical Science Basis. Contribution of Working Group I to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Stocker, T. F., Qin, D., Plattner, G.-K., Tignor, M., Allen, S. K., Boschung, J., Nauels, A., Xia, Y., Bex, V., and Midgley, P. M., Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, 465–570, 2013.
Denning, A. S., Takahashi, T., and Friedlingstein, P.: Can a strong atmospheric CO2 rectifier effect be reconciled with a “reasonable” carbon budget?, Tellus B, 51, 249–253, https://doi.org/10.1034/j.1600-0889.1999.t01-1-00010.x, 1999.
Dlugokencky, E. J., Steele, L. P., Lang, P. M., and Masarie, K. A.: The growth rate and distribution of atmospheric methane, J. Geophys. Res.-Atmos., 99, 17021–17043, https://doi.org/10.1029/94JD01245, 1994.
Ehhalt, D. H.: Photooxidation of trace gases in the troposphere Plenary Lecture, Phys. Chem. Chem. Phys., 1, 5401–5408, https://doi.org/10.1039/A905097C, 1999.
European Environment Agency EEA: European Union emission inventory report 1990–2012 under the UNECE Convention on Long-range Transboundary Air Pollution (LRTAP), 2014.
Fan, S., Gloor, M., Mahlman, J., Pacala, S., Sarmiento, J., Takahashi, T., and Tans, P.: A Large Terrestrial Carbon Sink in North America Implied by Atmospheric and Oceanic Carbon Dioxide Data and Models, Science, 282, 442–446, https://doi.org/10.1126/science.282.5388.442, 1998.
Feigenwinter, C., Bernhofer, C., and Vogt, R.: The Influence of Advection on the Short Term CO2-Budget in and Above a Forest Canopy, Bound.-Lay. Meteorol., 113, 201–224, https://doi.org/10.1023/B:BOUN.0000039372.86053.ff, 2004.
Feigenwinter, C., Bernhofer, C., Eichelmann, U., Heinesch, B., Hertel, M., Janous, D., Kolle, O., Lagergren, F., Lindroth, A., Minerbi, S., Moderow, U., Mölder, M., Montagnani, L., Queck, R., Rebmann, C., Vestin, P., Yernaux, M., Zeri, M., Ziegler, W., and Aubinet, M.: Comparison of horizontal and vertical advective CO2 fluxes at three forest sites, Agr. Forest Meteorol., 148, 12–24, https://doi.org/10.1016/j.agrformet.2007.08.013, 2008.
Felber, R., Münger, A., Neftel, A., and Ammann, C.: Eddy covariance methane flux measurements over a grazed pasture: effect of cows as moving point sources, Biogeosciences, 12, 3925–3940, https://doi.org/10.5194/bg-12-3925-2015, 2015.
Finnigan, J.: A comment on the paper by Lee (1998): On micrometeorological observations of surface-air exchange over tall vegetation, Agr. Forest Meteorol., 97, 55–64, https://doi.org/10.1016/S0168-1923(99)00049-0, 1999.
Gamnitzer, U., Karstens, U., Kromer, B., Neubert, R. E. M., Meijer, H. A. J., Schroeder, H., and Levin, I.: Carbon monoxide: A quantitative tracer for fossil fuel CO2?, J. Geophys. Res.-Atmos., 111, D22302, https://doi.org/10.1029/2005JD006966, 2006.
Gloor, M., Fan, S.-M., Pacala, S., and Sarmiento, J.: Optimal sampling of the atmosphere for purpose of inverse modeling: A model study, Global Biogeochem. Cy., 14, 407–428, https://doi.org/10.1029/1999GB900052, 2000.
Granier, C., Pétron, G., Müller, J.-F., and Brasseur, G.: The impact of natural and anthropogenic hydrocarbons on the tropospheric budget of carbon monoxide, Atmos. Environ., 34, 5255–5270, https://doi.org/10.1016/S1352-2310(00)00299-5, 2000.
Gurney, K. R., Law, R. M., Denning, A. S., Rayner, P. J., Baker, D., Bousquet, P., Bruhwiler, L., Chen, Y.-H., Ciais, P., Fan, S., Fung, I. Y., Gloor, M., Heimann, M., Higuchi, K., John, J., Maki, T., Maksyutov, S., Masarie, K., Peylin, P., Prather, M., Pak, B. C., Randerson, J., Sarmiento, J., Taguchi, S., Takahashi, T., and Yuen, C.-W.: Towards robust regional estimates of CO2 sources and sinks using atmospheric transport models, Nature, 415, 626–630, 2002.
Haszpra, L., Barcza, Z., Davis, K. J., and Tarczay, K.: Long-term tall tower carbon dioxide flux monitoring over an area of mixed vegetation, Agr. Forest Meteorol., 132, 58–77, https://doi.org/10.1016/j.agrformet.2005.07.002, 2005.
Henne, S., Brunner, D., Oney, B., Leuenberger, M., Eugster, W., Bamberger, I., Meinhardt, F., Steinbacher, M., and Emmenegger, L.: Validation of the Swiss methane emission inventory by atmospheric observations and inverse modelling, Atmos. Chem. Phys., 16, 3683–3710, https://doi.org/10.5194/acp-16-3683-2016, 2016.
Hiller, R. V., Bretscher, D., DelSontro, T., Diem, T., Eugster, W., Henneberger, R., Hobi, S., Hodson, E., Imer, D., Kreuzer, M., Künzle, T., Merbold, L., Niklaus, P. A., Rihm, B., Schellenberger, A., Schroth, M. H., Schubert, C. J., Siegrist, H., Stieger, J., Buchmann, N., and Brunner, D.: Anthropogenic and natural methane fluxes in Switzerland synthesized within a spatially explicit inventory, Biogeosciences, 11, 1941–1959, https://doi.org/10.5194/bg-11-1941-2014, 2014.
IPCC: Climate Change 2013: The Physical Science Basis. Contribution of Working Group I to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change, Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, 1535 pp., 2013.
Kirschke, S., Bousquet, P., Ciais, P., Saunois, M., Canadell, J. G., Dlugokencky, E. J., Bergamaschi, P., Bergmann, D., Blake, D. R., Bruhwiler, L., Cameron-Smith, P., Castaldi, S., Chevallier, F., Feng, L., Fraser, A., Heimann, M., Hodson, E. L., Houweling, S., Josse, B., Fraser, P. J., Krummel, P. B., Lamarque, J.-F., Langenfelds, R. L., Le Quere, C., Naik, V., O'Doherty, S., Palmer, P. I., Pison, I., Plummer, D., Poulter, B., Prinn, R. G., Rigby, M., Ringeval, B., Santini, M., Schmidt, M., Shindell, D. T., Simpson, I. J., Spahni, R., Steele, L. P., Strode, S. A., Sudo, K., Szopa, S., van der Werf, G. R., Voulgarakis, A., van Weele, M., Weiss, R. F., Williams, J. E., and Zeng, G.: Three decades of global methane sources and sinks, Nat. Geosci., 6, 813–823, https://doi.org/10.1038/ngeo1955, 2013.
Le Quéré, C., Moriarty, R., Andrew, R. M., Peters, G. P., Ciais, P., Friedlingstein, P., Jones, S. D., Sitch, S., Tans, P., Arneth, A., Boden, T. A., Bopp, L., Bozec, Y., Canadell, J. G., Chini, L. P., Chevallier, F., Cosca, C. E., Harris, I., Hoppema, M., Houghton, R. A., House, J. I., Jain, A. K., Johannessen, T., Kato, E., Keeling, R. F., Kitidis, V., Klein Goldewijk, K., Koven, C., Landa, C. S., Landschützer, P., Lenton, A., Lima, I. D., Marland, G., Mathis, J. T., Metzl, N., Nojiri, Y., Olsen, A., Ono, T., Peng, S., Peters, W., Pfeil, B., Poulter, B., Raupach, M. R., Regnier, P., Rödenbeck, C., Saito, S., Salisbury, J. E., Schuster, U., Schwinger, J., Séférian, R., Segschneider, J., Steinhoff, T., Stocker, B. D., Sutton, A. J., Takahashi, T., Tilbrook, B., van der Werf, G. R., Viovy, N., Wang, Y.-P., Wanninkhof, R., Wiltshire, A., and Zeng, N.: Global carbon budget 2014, Earth Syst. Sci. Data, 7, 47–85, https://doi.org/10.5194/essd-7-47-2015, 2015.
Lee, X.: On micrometeorological observations of surface-air exchange over tall vegetation, Agr. Forest Meteorol., 91, 39–49, https://doi.org/10.1016/S0168-1923(98)00071-9, 1998.
Legendre, P. and Legendre, L.: Chapter 10 – Interpretation of ecological structures, in: Developments in Environmental Modelling, edited by: Pierre, L. and Louis, L., Elsevier, 521–624, 2012.
Masarie, K. A. and Tans, P. P.: Extension and integration of atmospheric carbon dioxide data into a globally consistent measurement record, J. Geophys. Res.-Atmos., 100, 11593–11610, https://doi.org/10.1029/95JD00859, 1995.
Oney, B., Henne, S., Gruber, N., Leuenberger, M., Bamberger, I., Eugster, W., and Brunner, D.: The CarboCount CH sites: characterization of a dense greenhouse gas observation network, Atmos. Chem. Phys., 15, 11147–11164, https://doi.org/10.5194/acp-15-11147-2015, 2015.
Pales, J. C. and Keeling, C. D.: The concentration of atmospheric carbon dioxide in Hawaii, J. Geophys. Res., 70, 6053–6076, https://doi.org/10.1029/JZ070i024p06053, 1965.
Peylin, P., Rayner, P. J., Bousquet, P., Carouge, C., Hourdin, F., Heinrich, P., Ciais, P., and AEROCARB contributors: Daily CO2 flux estimates over Europe from continuous atmospheric measurements: 1, inverse methodology, Atmos. Chem. Phys., 5, 3173–3186, https://doi.org/10.5194/acp-5-3173-2005, 2005.
Popa, M. E., Gloor, M., Manning, A. C., Jordan, A., Schultz, U., Haensel, F., Seifert, T., and Heimann, M.: Measurements of greenhouse gases and related tracers at Bialystok tall tower station in Poland, Atmos. Meas. Tech., 3, 407–427, https://doi.org/10.5194/amt-3-407-2010, 2010.
Randerson, J. T., Thompson, M. V., Conway, T. J., Fung, I. Y., and Field, C. B.: The contribution of terrestrial sources and sinks to trends in the seasonal cycle of atmospheric carbon dioxide, Global Biogeochem. Cy., 11, 535–560, https://doi.org/10.1029/97GB02268, 1997.
Rödenbeck, C., Houweling, S., Gloor, M., and Heimann, M.: CO2 flux history 1982–2001 inferred from atmospheric data using a global inversion of atmospheric transport, Atmos. Chem. Phys., 3, 1919–1964, https://doi.org/10.5194/acp-3-1919-2003, 2003.
Ruckstuhl, A. F., Henne, S., Reimann, S., Steinbacher, M., Vollmer, M. K., O'Doherty, S., Buchmann, B., and Hueglin, C.: Robust extraction of baseline signal of atmospheric trace species using local regression, Atmos. Meas. Tech., 5, 2613–2624, https://doi.org/10.5194/amt-5-2613-2012, 2012.
Schmidt, M., Lopez, M., Yver Kwok, C., Messager, C., Ramonet, M., Wastine, B., Vuillemin, C., Truong, F., Gal, B., Parmentier, E., Cloué, O., and Ciais, P.: High-precision quasi-continuous atmospheric greenhouse gas measurements at Trainou tower (Orléans forest, France), Atmos. Meas. Tech., 7, 2283–2296, https://doi.org/10.5194/amt-7-2283-2014, 2014.
Seinfeld, J. H.: Atmospheric chemistry and physics: from air pollution to climate change, 2nd Edn., edited by: Pandis, S. N. and Hoboken, N. J., J. Wiley, Hoboken, 2006.
Swiss Federal Office for the Environment FOEN: NABEL – Luftbelastung 2013, Messresultate des Nationalen Beobachtungsnetzes für Luftfremdstoffe (NABEL), Bundesamt für Umwelt, Bern, 130 pp., 2014.
Swiss Federal Office for the Environment FOEN: Switzerland's Greenhouse Gas Inventory 1990–2013, National Inventory Report 2015, 2015a.
Swiss Federal Office for the Environment FOEN: Switzerland's Informative Inventory Report 2015, 2015b.
Tans, P. P.: 11 – Observational Strategy for Assessing the Role of Terrestrial Ecosystems in the Global Carbon Cycle: Scaling Down to Regional Levels, in: Scaling Physiological Processes, edited by: Field, J. R. E. B., Academic Press, San Diego, 179–190, 1993.
Thompson, R. L., Manning, A. C., Gloor, E., Schultz, U., Seifert, T., Hänsel, F., Jordan, A., and Heimann, M.: In-situ measurements of oxygen, carbon monoxide and greenhouse gases from Ochsenkopf tall tower in Germany, Atmos. Meas. Tech., 2, 573–591, https://doi.org/10.5194/amt-2-573-2009, 2009.
Thoning, K. W., Tans, P. P., and Komhyr, W. D.: Atmospheric carbon dioxide at Mauna Loa Observatory: 2. Analysis of the NOAA GMCC data, 1974–1985, J. Geophys. Res.-Atmos., 94, 8549–8565, https://doi.org/10.1029/JD094iD06p08549, 1989.
Vermeulen, A. T., Hensen, A., Popa, M. E., van den Bulk, W. C. M., and Jongejan, P. A. C.: Greenhouse gas observations from Cabauw Tall Tower (1992–2010), Atmos. Meas. Tech., 4, 617–644, https://doi.org/10.5194/amt-4-617-2011, 2011.
Warwick, N. J., Bekki, S., Law, K. S., Nisbet, E. G., and Pyle, J. A.: The impact of meteorology on the interannual growth rate of atmospheric methane, Geophys. Res. Lett., 29, 8-1–8-4, https://doi.org/10.1029/2002GL015282, 2002.
Winderlich, J., Chen, H., Gerbig, C., Seifert, T., Kolle, O., Lavric, J. V., Kaiser, C., Höfer, A., and Heimann, M.: Continuous low-maintenance CO2/CH4/H2O measurements at the Zotino Tall Tower Observatory (ZOTTO) in Central Siberia, Atmos. Meas. Tech., 3, 1113–1128, https://doi.org/10.5194/amt-3-1113-2010, 2010.
Winderlich, J., Gerbig, C., Kolle, O., and Heimann, M.: Inferences from CO2 and CH4 concentration profiles at the Zotino Tall Tower Observatory (ZOTTO) on regional summertime ecosystem fluxes, Biogeosciences, 11, 2055–2068, https://doi.org/10.5194/bg-11-2055-2014, 2014.
World Meteorological Organization: WMO Global Atmosphere Watch GAW: WMO GREENHOUSE GAS BULLETIN The State of Greenhouse Gases in the Atmosphere Based on Global Observations through 2013, 2014.
Yi, C., Davis, K. J., Bakwin, P. S., Berger, B. W., and Marr, L. C.: Influence of advection on measurements of the net ecosystem-atmosphere exchange of CO2 from a very tall tower, J. Geophys. Res.-Atmos., 105, 9991–9999, https://doi.org/10.1029/2000jd900080, 2000.
Zeeman, M. J., Hiller, R., Gilgen, A. K., Michna, P., Plüss, P., Buchmann, N., and Eugster, W.: Management and climate impacts on net CO2 fluxes and carbon budgets of three grasslands along an elevational gradient in Switzerland, Agr. Forest Meteorol., 150, 519–530, https://doi.org/10.1016/j.agrformet.2010.01.011, 2010.
Zellweger, C., Hüglin, C., Klausen, J., Steinbacher, M., Vollmer, M., and Buchmann, B.: Inter-comparison of four different carbon monoxide measurement techniques and evaluation of the long-term carbon monoxide time series of Jungfraujoch, Atmos. Chem. Phys., 9, 3491–3503, https://doi.org/10.5194/acp-9-3491-2009, 2009.
Short summary
Beromünster tall tower is the flagship of the densely placed Swiss greenhouse gas observation network (CarboCount CH). In this research article we report the first 2 years of the continuous greenhouse gas measurements using cavity ring down spectroscopy analyzer from this tall tower. We have adopted a purely observation based, multi-species and multi-level approach to characterize the site with respect to sources and sinks of natural and anthropogenic origin at diurnal to annual timescales.
Beromünster tall tower is the flagship of the densely placed Swiss greenhouse gas observation...
Altmetrics
Final-revised paper
Preprint